垃圾填埋场周边地下水和土壤污染物分布特征及健康风险——以广西12个垃圾填埋场为例

IF 6.2 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES
Fengping Liu , Hailin Zhu , Qiongqiong Lu , Yinan Zheng , Zhenyu Ding , Han Wang , Yuhu Chang
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引用次数: 0

摘要

垃圾填埋场处理了大量的城市垃圾,垃圾中的有害物质对填埋场及其周围的生态环境造成了严重的影响。为了系统地调查垃圾填埋场的污染机制和相关的健康风险,我们在中国广西进行了一项综合研究,收集了12个运行中的垃圾填埋场的水、土壤和渗滤液样本。使用电感耦合等离子体质谱法和紫外可见光谱法对这些样品进行分析,以量化18种重点污染物的浓度,包括重金属和营养物质。地统计学分析表明,土壤和地下水中污染物存在适度的空间聚类,Mn、Cd和Pb在渗滤液-土壤-地下水系统中呈显著正相关。值得注意的是,砷的致癌风险值是镉的2.3倍,而锌的非致癌风险系数在所有被研究的污染物中最高。通过相关模型评价了污染物的迁移途径,发现渗滤液中的Cu和Hg显著影响垃圾填埋场周围的地下水质量。这些发现为在受垃圾填埋场影响的地区实施特定地点的污染控制策略和优化健康风险管理方案提供了重要见解。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
The pollutants distribution profiles and health risks of groundwater and soil around the waste landfills: A study of 12 waste landfills in Guangxi province, China
The waste landfill disposes of a large amount of urban garbage, and the harmful substances in the waste have serious impacts on the ecological environment of the landfill and its surroundings. To systematically investigate the pollution mechanisms and associated health risks posed by landfills, we conducted a comprehensive study in Guangxi Province, China by collecting water, soil, and leachate samples from 12 operational landfill sites. These samples were analyzed using inductively coupled plasma mass spectrometry and ultraviolet-visible spectroscopy to quantify concentrations of 18 priority pollutants, including heavy metals and nutrients. Geostatistical analysis revealed moderate spatial clustering of pollutants in soils and groundwater, with significant positive correlations observed between Mn, Cd, and Pb concentrations across leachate-soil-groundwater systems. Notably, as exhibited 2.3-fold higher carcinogenic risk values compared to Cd, while Zn demonstrated the highest non-carcinogenic hazard quotient among all studied pollutants. Contaminant transport pathways were evaluated through correlation models, revealing that Cu and Hg in leachate significantly influenced groundwater quality around landfills. These findings provide critical insights for implementing site-specific pollution control strategies and optimizing health risk management protocols in landfill-impacted regions.
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来源期刊
CiteScore
12.10
自引率
5.90%
发文量
1234
审稿时长
88 days
期刊介绍: Ecotoxicology and Environmental Safety is a multi-disciplinary journal that focuses on understanding the exposure and effects of environmental contamination on organisms including human health. The scope of the journal covers three main themes. The topics within these themes, indicated below, include (but are not limited to) the following: Ecotoxicology、Environmental Chemistry、Environmental Safety etc.
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