小流域细粒沉积物地球化学特征揭示了青藏高原硅酸盐风化强度和空间差异

IF 5.4 1区 农林科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY
Tong Zhao , Qi Feng , Tengfei Yu , Wen Liu , Baofeng Li
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引用次数: 0

摘要

青藏高原硅酸盐风化对长期碳循环具有深远的影响。高原气候和地形的空间变异性对硅酸盐风化过程、通量和强度的研究提出了挑战。在此,我们提出了一套新的数据集,收集了来自青藏高原小流域的细沉积物的主要和微量元素组成。微量元素揭示了沉积物的再循环,尽管这对蚀变化学指数(CIA)只有微弱的影响。沉积物物源以中长英质岩为特征。青藏高原风化强度从北向南呈增加趋势。在高原内部,硅酸盐风化强度主要受气候因素控制。例如,在唐古拉北部,降水是控制风化强度的关键,而在唐古拉以南地区和雅鲁藏布江缝合带,温度是主要的控制因素。有趣的是,河流水化学和沉积物地球化学揭示了不同时间尺度的硅酸盐风化强度。短期风化强度主要受降水和冻融循环影响,长期风化强度受温度控制。在青藏高原东南缘,地形起伏对硅酸盐风化强度的影响较大。该研究为流域尺度上的硅酸盐风化强度评价提供了一个地球化学框架,并突出了青藏高原内部气候控制的风化强度。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Geochemistry of fine sediment from small catchments reveals silicate weathering intensity and spatial variation across the Tibetan Plateau
Silicate weathering on the Tibetan Plateau holds profound implications for long-term carbon cycle. The spatial variability in climate and topography on the plateau poses challenges in investigating silicate weathering processes, fluxes, and intensities. Here, we present a new data set on the major and trace element compositions of fine sediments collected from small catchments across the Tibetan Plateau. Trace elements reveal sediment recycling, though this has only a marginal influence on the chemical index of alteration (CIA). The provenance of sediments is characterized by intermediate and felsic rocks. There is an increasing trend of weathering intensity from north to south across the Tibetan Plateau. In the plateau’s interior, silicate weathering intensity is mainly controlled by climatic factors. For instance, to the north of the Tanggula, precipitation is pivotal in governing weathering intensity, while in regions to the south of the Tanggula and in the Yarlung Zangbo suture zone, temperature emerges as the dominant control. Intriguingly, the river water chemistry and sediment geochemistry reveal different temporal scales of silicate weathering intensity. Short-term weathering intensity is mainly influenced by precipitation and freeze–thaw cycles, and long-term weathering intensity is controlled by temperature. In contrast, relief exerts a strong impact on silicate weathering intensity in the southeastern margin of the Tibetan Plateau. This study provides a geochemical framework for evaluating silicate weathering intensity at the catchment scale and highlights a climate-controlled weathering intensity in the interior of the Tibetan Plateau.
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来源期刊
Catena
Catena 环境科学-地球科学综合
CiteScore
10.50
自引率
9.70%
发文量
816
审稿时长
54 days
期刊介绍: Catena publishes papers describing original field and laboratory investigations and reviews on geoecology and landscape evolution with emphasis on interdisciplinary aspects of soil science, hydrology and geomorphology. It aims to disseminate new knowledge and foster better understanding of the physical environment, of evolutionary sequences that have resulted in past and current landscapes, and of the natural processes that are likely to determine the fate of our terrestrial environment. Papers within any one of the above topics are welcome provided they are of sufficiently wide interest and relevance.
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