{"title":"1,3-二烯与光的可控自由基反应","authors":"Shiwei Lü, Jin Xie","doi":"10.1021/acscatal.5c01867","DOIUrl":null,"url":null,"abstract":"The direct conversion of feedstock chemicals into value-added products is a popular theme in synthetic chemistry. Since 1,3-dienes are some of the most ubiquitous and readily synthesizable starting materials, there is great interest in developing synthetic methods for their functionalization. However, due to the existence of multiple reactive sites on the 1,3-diene, achieving high regio- and enantioselectivity remains elusive. Traditional synthetic processes for 1,3-diene transformations often face challenges, such as low selectivity, high energy consumption, and the generation of undesirable byproducts. Driven by advances in synthetic technologies, synthesis methods utilizing radicals have emerged as a powerful platform for creating valuable chemical motifs. Photocatalytic approaches harness light energy to facilitate radical reactions under mild conditions, offering enhanced control over the reaction pathways and improved selectivity. In this review, we provide an insightful mechanistic overview of these radical-based photocatalytic innovations used in the controllable divergent radical reactions of 1,3-dienes. The reactions are categorized into 1,2- and 1,4-hydrofunctionalization and 1,2- and 1,4-difunctionalization. Perspectives on the future development of this emerging field are also given.","PeriodicalId":9,"journal":{"name":"ACS Catalysis ","volume":"41 1","pages":""},"PeriodicalIF":13.1000,"publicationDate":"2025-04-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Controllable Radical Reactions of 1,3-Dienes with Light\",\"authors\":\"Shiwei Lü, Jin Xie\",\"doi\":\"10.1021/acscatal.5c01867\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The direct conversion of feedstock chemicals into value-added products is a popular theme in synthetic chemistry. Since 1,3-dienes are some of the most ubiquitous and readily synthesizable starting materials, there is great interest in developing synthetic methods for their functionalization. However, due to the existence of multiple reactive sites on the 1,3-diene, achieving high regio- and enantioselectivity remains elusive. Traditional synthetic processes for 1,3-diene transformations often face challenges, such as low selectivity, high energy consumption, and the generation of undesirable byproducts. Driven by advances in synthetic technologies, synthesis methods utilizing radicals have emerged as a powerful platform for creating valuable chemical motifs. Photocatalytic approaches harness light energy to facilitate radical reactions under mild conditions, offering enhanced control over the reaction pathways and improved selectivity. In this review, we provide an insightful mechanistic overview of these radical-based photocatalytic innovations used in the controllable divergent radical reactions of 1,3-dienes. The reactions are categorized into 1,2- and 1,4-hydrofunctionalization and 1,2- and 1,4-difunctionalization. Perspectives on the future development of this emerging field are also given.\",\"PeriodicalId\":9,\"journal\":{\"name\":\"ACS Catalysis \",\"volume\":\"41 1\",\"pages\":\"\"},\"PeriodicalIF\":13.1000,\"publicationDate\":\"2025-04-25\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Catalysis \",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://doi.org/10.1021/acscatal.5c01867\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Catalysis ","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1021/acscatal.5c01867","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Controllable Radical Reactions of 1,3-Dienes with Light
The direct conversion of feedstock chemicals into value-added products is a popular theme in synthetic chemistry. Since 1,3-dienes are some of the most ubiquitous and readily synthesizable starting materials, there is great interest in developing synthetic methods for their functionalization. However, due to the existence of multiple reactive sites on the 1,3-diene, achieving high regio- and enantioselectivity remains elusive. Traditional synthetic processes for 1,3-diene transformations often face challenges, such as low selectivity, high energy consumption, and the generation of undesirable byproducts. Driven by advances in synthetic technologies, synthesis methods utilizing radicals have emerged as a powerful platform for creating valuable chemical motifs. Photocatalytic approaches harness light energy to facilitate radical reactions under mild conditions, offering enhanced control over the reaction pathways and improved selectivity. In this review, we provide an insightful mechanistic overview of these radical-based photocatalytic innovations used in the controllable divergent radical reactions of 1,3-dienes. The reactions are categorized into 1,2- and 1,4-hydrofunctionalization and 1,2- and 1,4-difunctionalization. Perspectives on the future development of this emerging field are also given.
期刊介绍:
ACS Catalysis is an esteemed journal that publishes original research in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. It offers broad coverage across diverse areas such as life sciences, organometallics and synthesis, photochemistry and electrochemistry, drug discovery and synthesis, materials science, environmental protection, polymer discovery and synthesis, and energy and fuels.
The scope of the journal is to showcase innovative work in various aspects of catalysis. This includes new reactions and novel synthetic approaches utilizing known catalysts, the discovery or modification of new catalysts, elucidation of catalytic mechanisms through cutting-edge investigations, practical enhancements of existing processes, as well as conceptual advances in the field. Contributions to ACS Catalysis can encompass both experimental and theoretical research focused on catalytic molecules, macromolecules, and materials that exhibit catalytic turnover.