基于GBFS的甲烷蒸汽催化重整动态温度效应CFD-DEM模拟

IF 8.1 2区 工程技术 Q1 CHEMISTRY, PHYSICAL
Shen Li , Hanwen Kou , Yanzhuo Hu, Shaohui Han, Zisheng Li, Junguo Li, Xing Huang, Yan Lin, Xin Yao
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引用次数: 0

摘要

采用CFD-DEM模拟研究了颗粒化高炉渣(GBFS)催化甲烷蒸汽重整过程,并对颗粒温度波动进行了跟踪研究。探讨了混合气速度、颗粒大小、颗粒温度、汽碳比和压力对反应过程的影响。结果表明,较高的S/C比和GBFS颗粒温度可提高反应速率和产氢率,而气体速度和压力对反应速率和产氢率的影响较小。GBFS粒径的增大导致反应速率的降低和温度波动的减小。此外,还提出了甲烷蒸汽重整的反应途径。这些发现为GBFS废热的化学回收提供了有价值的见解。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
CFD-DEM simulation of dynamic temperature effects on catalytic methane steam reforming using GBFS
This study employs CFD-DEM simulations to investigate the methane steam reforming process catalyzed by Granulated Blast Furnace Slag (GBFS) and tracks the temperature fluctuations of GBFS particles. The effects of mixed gas velocity, particle size, particle temperature, steam-to-carbon (S/C) ratio, and pressure on the reaction process are explored. The results show that higher S/C ratios and GBFS particle temperatures enhance the reaction rate and hydrogen production, while gas velocity and pressure have minimal effects. An increase in GBFS particle size leads to a decrease in reaction rate and reduces temperature fluctuations. Additionally, a reaction pathway for methane steam reforming is proposed. These findings provide valuable insights into the chemical recovery of waste heat from GBFS.
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来源期刊
International Journal of Hydrogen Energy
International Journal of Hydrogen Energy 工程技术-环境科学
CiteScore
13.50
自引率
25.00%
发文量
3502
审稿时长
60 days
期刊介绍: The objective of the International Journal of Hydrogen Energy is to facilitate the exchange of new ideas, technological advancements, and research findings in the field of Hydrogen Energy among scientists and engineers worldwide. This journal showcases original research, both analytical and experimental, covering various aspects of Hydrogen Energy. These include production, storage, transmission, utilization, enabling technologies, environmental impact, economic considerations, and global perspectives on hydrogen and its carriers such as NH3, CH4, alcohols, etc. The utilization aspect encompasses various methods such as thermochemical (combustion), photochemical, electrochemical (fuel cells), and nuclear conversion of hydrogen, hydrogen isotopes, and hydrogen carriers into thermal, mechanical, and electrical energies. The applications of these energies can be found in transportation (including aerospace), industrial, commercial, and residential sectors.
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