{"title":"通过连续体中的双束缚态实现聚焦可调谐放大光致发光的混合超表面","authors":"Omar A. M. Abdelraouf, Mengfei Wu, Hong Liu","doi":"10.1002/adfm.202505165","DOIUrl":null,"url":null,"abstract":"Miniaturized, tunable light sources are essential for integrated photonic devices in quantum computing, communications, and sensing. However, achieving tunable emission post-fabrication remains challenging, especially for efficient amplification. Hybrid metasurfaces that combine multiple nanostructured materials offer a promising solution, enabling enhanced control and amplification of light emission. Here, tunable amplified photoluminescence (PL) is demonstrated in nanocrystalline silicon (nc-Si) quantum dots (QDs) embedded in a hybrid metasurface of amorphous silicon (a-Si) and antimony trisulfide (Sb2S3), a low-loss phase change material (PCM). The nc-Si QDs exhibit stable, efficient PL at high temperatures, while the PCM enables tunable phase transitions. The metasurface supports dual quasi-bound states in the continuum (BICs), achieving Q-factors up to 225 and amplifying PL by a factor of 15 with a wavelength shift of 105 nm via dimensional modulation. Additionally, all-optical PL tunability across a 24 nm range is attained through PCM phase modulation. Furthermore, a high Q-factor metalens is proposed to focus the tunable amplified PL, extending the focused PL tunability into the near-infrared (NIR). This work advances reconfigurable nanophotonic devices for efficient quantum light sources in photonic systems.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"14 1","pages":""},"PeriodicalIF":18.5000,"publicationDate":"2025-04-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Hybrid Metasurfaces Enabling Focused Tunable Amplified Photoluminescence Through Dual Bound States in the Continuum\",\"authors\":\"Omar A. M. Abdelraouf, Mengfei Wu, Hong Liu\",\"doi\":\"10.1002/adfm.202505165\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Miniaturized, tunable light sources are essential for integrated photonic devices in quantum computing, communications, and sensing. However, achieving tunable emission post-fabrication remains challenging, especially for efficient amplification. Hybrid metasurfaces that combine multiple nanostructured materials offer a promising solution, enabling enhanced control and amplification of light emission. Here, tunable amplified photoluminescence (PL) is demonstrated in nanocrystalline silicon (nc-Si) quantum dots (QDs) embedded in a hybrid metasurface of amorphous silicon (a-Si) and antimony trisulfide (Sb2S3), a low-loss phase change material (PCM). The nc-Si QDs exhibit stable, efficient PL at high temperatures, while the PCM enables tunable phase transitions. The metasurface supports dual quasi-bound states in the continuum (BICs), achieving Q-factors up to 225 and amplifying PL by a factor of 15 with a wavelength shift of 105 nm via dimensional modulation. Additionally, all-optical PL tunability across a 24 nm range is attained through PCM phase modulation. Furthermore, a high Q-factor metalens is proposed to focus the tunable amplified PL, extending the focused PL tunability into the near-infrared (NIR). This work advances reconfigurable nanophotonic devices for efficient quantum light sources in photonic systems.\",\"PeriodicalId\":112,\"journal\":{\"name\":\"Advanced Functional Materials\",\"volume\":\"14 1\",\"pages\":\"\"},\"PeriodicalIF\":18.5000,\"publicationDate\":\"2025-04-24\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advanced Functional Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1002/adfm.202505165\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Functional Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1002/adfm.202505165","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Hybrid Metasurfaces Enabling Focused Tunable Amplified Photoluminescence Through Dual Bound States in the Continuum
Miniaturized, tunable light sources are essential for integrated photonic devices in quantum computing, communications, and sensing. However, achieving tunable emission post-fabrication remains challenging, especially for efficient amplification. Hybrid metasurfaces that combine multiple nanostructured materials offer a promising solution, enabling enhanced control and amplification of light emission. Here, tunable amplified photoluminescence (PL) is demonstrated in nanocrystalline silicon (nc-Si) quantum dots (QDs) embedded in a hybrid metasurface of amorphous silicon (a-Si) and antimony trisulfide (Sb2S3), a low-loss phase change material (PCM). The nc-Si QDs exhibit stable, efficient PL at high temperatures, while the PCM enables tunable phase transitions. The metasurface supports dual quasi-bound states in the continuum (BICs), achieving Q-factors up to 225 and amplifying PL by a factor of 15 with a wavelength shift of 105 nm via dimensional modulation. Additionally, all-optical PL tunability across a 24 nm range is attained through PCM phase modulation. Furthermore, a high Q-factor metalens is proposed to focus the tunable amplified PL, extending the focused PL tunability into the near-infrared (NIR). This work advances reconfigurable nanophotonic devices for efficient quantum light sources in photonic systems.
期刊介绍:
Firmly established as a top-tier materials science journal, Advanced Functional Materials reports breakthrough research in all aspects of materials science, including nanotechnology, chemistry, physics, and biology every week.
Advanced Functional Materials is known for its rapid and fair peer review, quality content, and high impact, making it the first choice of the international materials science community.