Hanson Appiah-Twum, Tim Van Winckel, Julia Santolin, Jolien De Paepe, Stefanie Hellweg, Tove A. Larsen, Kai M. Udert, Siegfried E. Vlaeminck, Marc Spiller
{"title":"将分散式尿液处理纳入城市污水管理系统对环境的影响:生命周期比较评估","authors":"Hanson Appiah-Twum, Tim Van Winckel, Julia Santolin, Jolien De Paepe, Stefanie Hellweg, Tove A. Larsen, Kai M. Udert, Siegfried E. Vlaeminck, Marc Spiller","doi":"10.1016/j.watres.2025.123630","DOIUrl":null,"url":null,"abstract":"As municipal wastewater treatment regulations become more stringent, integrating source-separated urine treatment into centralized urban wastewater management offers a ‘hybrid’ solution. However, it is not clear how the environmental impacts of such hybrid systems compare to highly efficient centralized wastewater treatment plants (WWTPs) with low N<sub>2</sub>O emissions and electricity use. In this study, a consequential life cycle assessment was used to compare the environmental impact of three urine separation hybrid wastewater treatment systems – which combine decentralized urine treatment with a highly efficient central WWTP– to a centralized WWTP treating mixed wastewater (baseline). The studied urine treatment systems include partial nitrification & distillation, struvite precipitation & stripping/scrubbing, and partial nitritation/anammox. Additionally, the environmental impact of urine pre-treatment by calcium hydroxide and electrochemical alkalinization methods on the partial nitrification & distillation system was evaluated. The results show that all hybrid scenarios have a lower environmental impact in the freshwater ecotoxicity, marine toxicity, freshwater eutrophication and marine eutrophication categories compared to the baseline. However, all hybrid scenarios resulted in higher impacts on global warming compared to the baseline, with direct N<sub>2</sub>O emissions being a key variable. Additionally, it was identified that urine alkalinization increased the environmental impact of the treatment system in 7 out of the 10 impact categories. A Pareto frontier analysis was developed to guide decision makers on where hybrid solutions could be used as a strategy to reduce global warming impacts of conventional WWTPs. Using N<sub>2</sub>O emission factors of 75 WWTPs, 87% of centralized WWTPs had lower global warming impact compared to partial nitrification & distillation, and 91% compared to partial nitritation/anammox hybrid solutions. However, at energy demands of 1 kWh/PE and 1.5 kWh/PE, both hybrid solutions showed lower global warming impact than all the studied WWTPs. The study highlights the potential of hybrid wastewater treatment solutions as a strategy to reduce global warming impacts in WWTPs with high N<sub>2</sub>O emissions and electricity use as well as a mean to reduce marine eutrophication (i.e. nitrogen pollution).","PeriodicalId":443,"journal":{"name":"Water Research","volume":"35 1","pages":""},"PeriodicalIF":11.4000,"publicationDate":"2025-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Environmental impact of integrating decentralized urine treatment in the urban wastewater management system: A comparative life cycle assessment\",\"authors\":\"Hanson Appiah-Twum, Tim Van Winckel, Julia Santolin, Jolien De Paepe, Stefanie Hellweg, Tove A. Larsen, Kai M. Udert, Siegfried E. Vlaeminck, Marc Spiller\",\"doi\":\"10.1016/j.watres.2025.123630\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"As municipal wastewater treatment regulations become more stringent, integrating source-separated urine treatment into centralized urban wastewater management offers a ‘hybrid’ solution. However, it is not clear how the environmental impacts of such hybrid systems compare to highly efficient centralized wastewater treatment plants (WWTPs) with low N<sub>2</sub>O emissions and electricity use. In this study, a consequential life cycle assessment was used to compare the environmental impact of three urine separation hybrid wastewater treatment systems – which combine decentralized urine treatment with a highly efficient central WWTP– to a centralized WWTP treating mixed wastewater (baseline). The studied urine treatment systems include partial nitrification & distillation, struvite precipitation & stripping/scrubbing, and partial nitritation/anammox. Additionally, the environmental impact of urine pre-treatment by calcium hydroxide and electrochemical alkalinization methods on the partial nitrification & distillation system was evaluated. The results show that all hybrid scenarios have a lower environmental impact in the freshwater ecotoxicity, marine toxicity, freshwater eutrophication and marine eutrophication categories compared to the baseline. However, all hybrid scenarios resulted in higher impacts on global warming compared to the baseline, with direct N<sub>2</sub>O emissions being a key variable. Additionally, it was identified that urine alkalinization increased the environmental impact of the treatment system in 7 out of the 10 impact categories. A Pareto frontier analysis was developed to guide decision makers on where hybrid solutions could be used as a strategy to reduce global warming impacts of conventional WWTPs. 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Environmental impact of integrating decentralized urine treatment in the urban wastewater management system: A comparative life cycle assessment
As municipal wastewater treatment regulations become more stringent, integrating source-separated urine treatment into centralized urban wastewater management offers a ‘hybrid’ solution. However, it is not clear how the environmental impacts of such hybrid systems compare to highly efficient centralized wastewater treatment plants (WWTPs) with low N2O emissions and electricity use. In this study, a consequential life cycle assessment was used to compare the environmental impact of three urine separation hybrid wastewater treatment systems – which combine decentralized urine treatment with a highly efficient central WWTP– to a centralized WWTP treating mixed wastewater (baseline). The studied urine treatment systems include partial nitrification & distillation, struvite precipitation & stripping/scrubbing, and partial nitritation/anammox. Additionally, the environmental impact of urine pre-treatment by calcium hydroxide and electrochemical alkalinization methods on the partial nitrification & distillation system was evaluated. The results show that all hybrid scenarios have a lower environmental impact in the freshwater ecotoxicity, marine toxicity, freshwater eutrophication and marine eutrophication categories compared to the baseline. However, all hybrid scenarios resulted in higher impacts on global warming compared to the baseline, with direct N2O emissions being a key variable. Additionally, it was identified that urine alkalinization increased the environmental impact of the treatment system in 7 out of the 10 impact categories. A Pareto frontier analysis was developed to guide decision makers on where hybrid solutions could be used as a strategy to reduce global warming impacts of conventional WWTPs. Using N2O emission factors of 75 WWTPs, 87% of centralized WWTPs had lower global warming impact compared to partial nitrification & distillation, and 91% compared to partial nitritation/anammox hybrid solutions. However, at energy demands of 1 kWh/PE and 1.5 kWh/PE, both hybrid solutions showed lower global warming impact than all the studied WWTPs. The study highlights the potential of hybrid wastewater treatment solutions as a strategy to reduce global warming impacts in WWTPs with high N2O emissions and electricity use as well as a mean to reduce marine eutrophication (i.e. nitrogen pollution).
期刊介绍:
Water Research, along with its open access companion journal Water Research X, serves as a platform for publishing original research papers covering various aspects of the science and technology related to the anthropogenic water cycle, water quality, and its management worldwide. The audience targeted by the journal comprises biologists, chemical engineers, chemists, civil engineers, environmental engineers, limnologists, and microbiologists. The scope of the journal include:
•Treatment processes for water and wastewaters (municipal, agricultural, industrial, and on-site treatment), including resource recovery and residuals management;
•Urban hydrology including sewer systems, stormwater management, and green infrastructure;
•Drinking water treatment and distribution;
•Potable and non-potable water reuse;
•Sanitation, public health, and risk assessment;
•Anaerobic digestion, solid and hazardous waste management, including source characterization and the effects and control of leachates and gaseous emissions;
•Contaminants (chemical, microbial, anthropogenic particles such as nanoparticles or microplastics) and related water quality sensing, monitoring, fate, and assessment;
•Anthropogenic impacts on inland, tidal, coastal and urban waters, focusing on surface and ground waters, and point and non-point sources of pollution;
•Environmental restoration, linked to surface water, groundwater and groundwater remediation;
•Analysis of the interfaces between sediments and water, and between water and atmosphere, focusing specifically on anthropogenic impacts;
•Mathematical modelling, systems analysis, machine learning, and beneficial use of big data related to the anthropogenic water cycle;
•Socio-economic, policy, and regulations studies.