双网络启发的机械超材料

IF 37.2 1区 材料科学 Q1 CHEMISTRY, PHYSICAL
James Utama Surjadi, Bastien F. G. Aymon, Molly Carton, Carlos M. Portela
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引用次数: 0

摘要

机械超材料可以在低密度下获得高刚度和高强度,但通常是以低延展性和低拉伸性为代价的——这是材料中一个持久的权衡。相比之下,双网状水凝胶具有互穿的柔性和刚性聚合物网络,并具有前所未有的高刚度和拉伸性组合,从而具有优异的韧性。在这里,我们通过将单片桁架(刚性)和编织(柔性)组件集成到一个超材料结构中,提出了双网络启发的超材料,与纯材料相比,其刚度和拉伸性增加了十倍。非线性计算力学模型表明,在这些双网络启发的超材料中,能量耗散的增强是由于网络之间的纠缠导致摩擦耗散的增加。通过引入通常会降低机械性能的内部缺陷,我们证明了这些超材料通过失效离域的能量耗散增加了三倍。这项工作为开发受聚合物网络拓扑结构启发的高依从性超材料开辟了道路。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Double-network-inspired mechanical metamaterials

Double-network-inspired mechanical metamaterials

Mechanical metamaterials can achieve high stiffness and strength at low densities, but often at the expense of low ductility and stretchability—a persistent trade-off in materials. In contrast, double-network hydrogels feature interpenetrating compliant and stiff polymer networks, and exhibit unprecedented combinations of high stiffness and stretchability, resulting in exceptional toughness. Here we present double-network-inspired metamaterials by integrating monolithic truss (stiff) and woven (compliant) components into a metamaterial architecture, which achieves a tenfold increase in stiffness and stretchability compared to its pure counterparts. Nonlinear computational mechanics models elucidate that enhanced energy dissipation in these double-network-inspired metamaterials stems from increased frictional dissipation due to entanglements between networks. Through introduction of internal defects, which typically degrade mechanical properties, we demonstrate a threefold increase in energy dissipation for these metamaterials via failure delocalization. This work opens avenues for developing metamaterials in a high-compliance regime inspired by polymer network topologies.

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来源期刊
Nature Materials
Nature Materials 工程技术-材料科学:综合
CiteScore
62.20
自引率
0.70%
发文量
221
审稿时长
3.2 months
期刊介绍: Nature Materials is a monthly multi-disciplinary journal aimed at bringing together cutting-edge research across the entire spectrum of materials science and engineering. It covers all applied and fundamental aspects of the synthesis/processing, structure/composition, properties, and performance of materials. The journal recognizes that materials research has an increasing impact on classical disciplines such as physics, chemistry, and biology. Additionally, Nature Materials provides a forum for the development of a common identity among materials scientists and encourages interdisciplinary collaboration. It takes an integrated and balanced approach to all areas of materials research, fostering the exchange of ideas between scientists involved in different disciplines. Nature Materials is an invaluable resource for scientists in academia and industry who are active in discovering and developing materials and materials-related concepts. It offers engaging and informative papers of exceptional significance and quality, with the aim of influencing the development of society in the future.
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