{"title":"隧道氧化钝化超薄Bi2O2Se/Si异质结光电探测器提高光电性能","authors":"Tzu-Pu Hung, Wei-Han Chen, Yi-Jyun Chen, Yu-Hao Tu, Zhi-Hao Huang, Yu-Lun Chueh, Chao-Hui Yeh, Chien-Wei Chen, Yang-Yu Jhang, Ying-Hao Chu, Cheng-Ying Chen","doi":"10.1021/acsami.5c03477","DOIUrl":null,"url":null,"abstract":"Two-dimensional (2D) materials have garnered significant attention for next-generation optoelectronic devices due to their exceptional physical properties. This study introduces a high-performance ultrathin Bi<sub>2</sub>O<sub>2</sub>Se/Si heterojunction photodetector with tunneling oxide passivation, fabricated using a transfer-free pulsed laser deposition method. The Bi<sub>2</sub>O<sub>2</sub>Se layer exhibits strong air stability and compatibility for practical applications. By incorporating a thin SiO<sub>2</sub> tunneling layer, the heterostructure achieves a low dark current (∼22.3 nA/cm<sup>2</sup>), a high on/off ratio (∼8 × 10<sup>6</sup>), and a responsivity of 23.0 A/W. Compared to traditional CdS/Si devices, this photodetector demonstrates superior performance, including faster response time and higher stability. These findings underscore the potential of Bi<sub>2</sub>O<sub>2</sub>Se/Si heterostructures for advanced photonic and optoelectronic applications.","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":"39 1","pages":""},"PeriodicalIF":8.3000,"publicationDate":"2025-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Ultrathin Bi2O2Se/Si Heterojunction Photodetector with Tunneling Oxide Passivation for Enhanced Optoelectronic Performance\",\"authors\":\"Tzu-Pu Hung, Wei-Han Chen, Yi-Jyun Chen, Yu-Hao Tu, Zhi-Hao Huang, Yu-Lun Chueh, Chao-Hui Yeh, Chien-Wei Chen, Yang-Yu Jhang, Ying-Hao Chu, Cheng-Ying Chen\",\"doi\":\"10.1021/acsami.5c03477\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Two-dimensional (2D) materials have garnered significant attention for next-generation optoelectronic devices due to their exceptional physical properties. This study introduces a high-performance ultrathin Bi<sub>2</sub>O<sub>2</sub>Se/Si heterojunction photodetector with tunneling oxide passivation, fabricated using a transfer-free pulsed laser deposition method. The Bi<sub>2</sub>O<sub>2</sub>Se layer exhibits strong air stability and compatibility for practical applications. By incorporating a thin SiO<sub>2</sub> tunneling layer, the heterostructure achieves a low dark current (∼22.3 nA/cm<sup>2</sup>), a high on/off ratio (∼8 × 10<sup>6</sup>), and a responsivity of 23.0 A/W. Compared to traditional CdS/Si devices, this photodetector demonstrates superior performance, including faster response time and higher stability. These findings underscore the potential of Bi<sub>2</sub>O<sub>2</sub>Se/Si heterostructures for advanced photonic and optoelectronic applications.\",\"PeriodicalId\":5,\"journal\":{\"name\":\"ACS Applied Materials & Interfaces\",\"volume\":\"39 1\",\"pages\":\"\"},\"PeriodicalIF\":8.3000,\"publicationDate\":\"2025-04-23\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Materials & Interfaces\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1021/acsami.5c03477\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Materials & Interfaces","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acsami.5c03477","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Ultrathin Bi2O2Se/Si Heterojunction Photodetector with Tunneling Oxide Passivation for Enhanced Optoelectronic Performance
Two-dimensional (2D) materials have garnered significant attention for next-generation optoelectronic devices due to their exceptional physical properties. This study introduces a high-performance ultrathin Bi2O2Se/Si heterojunction photodetector with tunneling oxide passivation, fabricated using a transfer-free pulsed laser deposition method. The Bi2O2Se layer exhibits strong air stability and compatibility for practical applications. By incorporating a thin SiO2 tunneling layer, the heterostructure achieves a low dark current (∼22.3 nA/cm2), a high on/off ratio (∼8 × 106), and a responsivity of 23.0 A/W. Compared to traditional CdS/Si devices, this photodetector demonstrates superior performance, including faster response time and higher stability. These findings underscore the potential of Bi2O2Se/Si heterostructures for advanced photonic and optoelectronic applications.
期刊介绍:
ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.