{"title":"外封底：单层二硫化钼平面内硫空位富集促进C─O键解理和逆水气转换活性[j]。化学17/2025)","authors":"Zhiyuan Zheng, Xin Shang, Weijue Wang, Xiaofeng Yang, Xiong Su, Yanqiang Huang","doi":"10.1002/ange.202506409","DOIUrl":null,"url":null,"abstract":"<p>A precise strategy for tuning defective structures in two-dimensional catalysts was developed by Yanqiang Huang, Xiong Su, Xin Shang et al. in their Research Article (e202422953). By employing a soft–hard dual-template approach, single-layer MoS<sub>2</sub> with enriched in-plane sulfur vacancies was synthesized. These vacancies significantly promote C─O bond cleavage, resulting in remarkable catalytic performance in the reverse water–gas shift reaction.\n\n <figure>\n <div><picture>\n <source></source></picture><p></p>\n </div>\n </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 17","pages":""},"PeriodicalIF":0.0000,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202506409","citationCount":"0","resultStr":"{\"title\":\"Outside Back Cover: Boosting C─O Bond Cleavage and Reverse Water-Gas Shift Activity via Enriched in-plane Sulfur Vacancies in Single-Layer Molybdenum Disulfide (Angew. Chem. 17/2025)\",\"authors\":\"Zhiyuan Zheng, Xin Shang, Weijue Wang, Xiaofeng Yang, Xiong Su, Yanqiang Huang\",\"doi\":\"10.1002/ange.202506409\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>A precise strategy for tuning defective structures in two-dimensional catalysts was developed by Yanqiang Huang, Xiong Su, Xin Shang et al. in their Research Article (e202422953). By employing a soft–hard dual-template approach, single-layer MoS<sub>2</sub> with enriched in-plane sulfur vacancies was synthesized. These vacancies significantly promote C─O bond cleavage, resulting in remarkable catalytic performance in the reverse water–gas shift reaction.\\n\\n <figure>\\n <div><picture>\\n <source></source></picture><p></p>\\n </div>\\n </figure></p>\",\"PeriodicalId\":7803,\"journal\":{\"name\":\"Angewandte Chemie\",\"volume\":\"137 17\",\"pages\":\"\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2025-03-27\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202506409\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Angewandte Chemie\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://onlinelibrary.wiley.com/doi/10.1002/ange.202506409\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Angewandte Chemie","FirstCategoryId":"1085","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/ange.202506409","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
Outside Back Cover: Boosting C─O Bond Cleavage and Reverse Water-Gas Shift Activity via Enriched in-plane Sulfur Vacancies in Single-Layer Molybdenum Disulfide (Angew. Chem. 17/2025)
A precise strategy for tuning defective structures in two-dimensional catalysts was developed by Yanqiang Huang, Xiong Su, Xin Shang et al. in their Research Article (e202422953). By employing a soft–hard dual-template approach, single-layer MoS2 with enriched in-plane sulfur vacancies was synthesized. These vacancies significantly promote C─O bond cleavage, resulting in remarkable catalytic performance in the reverse water–gas shift reaction.
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