{"title":"基于双极光电晶体管的圆形光电效应控制偏振计用于空间分辨映射","authors":"Ruixue Bai, Xiaoshan Du, Rui Zhou, Yaojie Zhu, Xilin Zhang, Yulun Liu, Zuowei Yan, Hui Ma, Weibo Gao, Chongyun Jiang","doi":"10.1021/acsnano.4c18833","DOIUrl":null,"url":null,"abstract":"The circular photogalvanic effect (CPGE), converted from the photon angular moment as a spin-polarized charge current via inversion asymmetry, is an effective approach to detecting circularly polarized light. However, the CPGE current is typically weak, and even the electrical gate gives quite limited improvement, necessitating the use of auxiliary amplifiers to strengthen the signals for practical applications. Here, we constitute a vertical bipolar phototransistor based on MoS<sub>2</sub>/ZrGeTe<sub>4</sub>/MoS<sub>2</sub> heterojunction with a noncentrosymmetric active region, which can detect and amplify the CPGE photocurrents for all directions, with a CPGE gain of 25. Thereupon, we achieve tens of μA/W CPGE responsivity from visible to near-infrared (NIR) and wide acceptance angles from 45° to −45° at room temperature, revealing multiscenario applications. The full Stokes spatially resolved mapping of the NIR vortex beam demonstrates its practical applicability as a polarimeter with high sensitivity. Our work provides an approach to developing nanostructured polarimeters controlled by inversion symmetry and devoid of external amplification modules, which leads to potential applications for future nanophotonics and optoelectronic nanodevices.","PeriodicalId":21,"journal":{"name":"ACS Nano","volume":"1 1","pages":""},"PeriodicalIF":16.0000,"publicationDate":"2025-04-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"A Circular Photogalvanic Effect-Controlled Polarimeter based on a Bipolar Phototransistor Utilized in Spatially Resolved Mapping\",\"authors\":\"Ruixue Bai, Xiaoshan Du, Rui Zhou, Yaojie Zhu, Xilin Zhang, Yulun Liu, Zuowei Yan, Hui Ma, Weibo Gao, Chongyun Jiang\",\"doi\":\"10.1021/acsnano.4c18833\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The circular photogalvanic effect (CPGE), converted from the photon angular moment as a spin-polarized charge current via inversion asymmetry, is an effective approach to detecting circularly polarized light. However, the CPGE current is typically weak, and even the electrical gate gives quite limited improvement, necessitating the use of auxiliary amplifiers to strengthen the signals for practical applications. Here, we constitute a vertical bipolar phototransistor based on MoS<sub>2</sub>/ZrGeTe<sub>4</sub>/MoS<sub>2</sub> heterojunction with a noncentrosymmetric active region, which can detect and amplify the CPGE photocurrents for all directions, with a CPGE gain of 25. Thereupon, we achieve tens of μA/W CPGE responsivity from visible to near-infrared (NIR) and wide acceptance angles from 45° to −45° at room temperature, revealing multiscenario applications. The full Stokes spatially resolved mapping of the NIR vortex beam demonstrates its practical applicability as a polarimeter with high sensitivity. Our work provides an approach to developing nanostructured polarimeters controlled by inversion symmetry and devoid of external amplification modules, which leads to potential applications for future nanophotonics and optoelectronic nanodevices.\",\"PeriodicalId\":21,\"journal\":{\"name\":\"ACS Nano\",\"volume\":\"1 1\",\"pages\":\"\"},\"PeriodicalIF\":16.0000,\"publicationDate\":\"2025-04-16\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Nano\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1021/acsnano.4c18833\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Nano","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acsnano.4c18833","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
A Circular Photogalvanic Effect-Controlled Polarimeter based on a Bipolar Phototransistor Utilized in Spatially Resolved Mapping
The circular photogalvanic effect (CPGE), converted from the photon angular moment as a spin-polarized charge current via inversion asymmetry, is an effective approach to detecting circularly polarized light. However, the CPGE current is typically weak, and even the electrical gate gives quite limited improvement, necessitating the use of auxiliary amplifiers to strengthen the signals for practical applications. Here, we constitute a vertical bipolar phototransistor based on MoS2/ZrGeTe4/MoS2 heterojunction with a noncentrosymmetric active region, which can detect and amplify the CPGE photocurrents for all directions, with a CPGE gain of 25. Thereupon, we achieve tens of μA/W CPGE responsivity from visible to near-infrared (NIR) and wide acceptance angles from 45° to −45° at room temperature, revealing multiscenario applications. The full Stokes spatially resolved mapping of the NIR vortex beam demonstrates its practical applicability as a polarimeter with high sensitivity. Our work provides an approach to developing nanostructured polarimeters controlled by inversion symmetry and devoid of external amplification modules, which leads to potential applications for future nanophotonics and optoelectronic nanodevices.
期刊介绍:
ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.