基于双极光电晶体管的圆形光电效应控制偏振计用于空间分辨映射

IF 16 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
ACS Nano Pub Date : 2025-04-16 DOI:10.1021/acsnano.4c18833
Ruixue Bai, Xiaoshan Du, Rui Zhou, Yaojie Zhu, Xilin Zhang, Yulun Liu, Zuowei Yan, Hui Ma, Weibo Gao, Chongyun Jiang
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引用次数: 0

摘要

圆光电效应(CPGE)是一种检测圆偏振光的有效方法,它将光子角矩通过反转不对称转化为自旋极化电荷电流。然而,CPGE电流通常很弱,甚至电气门也提供了相当有限的改进,因此需要使用辅助放大器来增强实际应用中的信号。在此,我们构建了一个基于MoS2/ZrGeTe4/MoS2异质结的垂直双极光电晶体管,具有非中心对称的有源区,可以检测和放大所有方向的CPGE光电流,CPGE增益为25。因此,我们在室温下实现了从可见光到近红外(NIR)的数十μA/W的CPGE响应率和45°到- 45°的宽接受角,揭示了多场景应用。近红外涡旋光束的全Stokes空间分辨映射证明了它作为高灵敏度偏振计的实际适用性。我们的工作提供了一种方法来开发由反转对称控制的纳米结构偏振计,并且没有外部放大模块,这将导致未来纳米光子学和光电子纳米器件的潜在应用。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

A Circular Photogalvanic Effect-Controlled Polarimeter based on a Bipolar Phototransistor Utilized in Spatially Resolved Mapping

A Circular Photogalvanic Effect-Controlled Polarimeter based on a Bipolar Phototransistor Utilized in Spatially Resolved Mapping
The circular photogalvanic effect (CPGE), converted from the photon angular moment as a spin-polarized charge current via inversion asymmetry, is an effective approach to detecting circularly polarized light. However, the CPGE current is typically weak, and even the electrical gate gives quite limited improvement, necessitating the use of auxiliary amplifiers to strengthen the signals for practical applications. Here, we constitute a vertical bipolar phototransistor based on MoS2/ZrGeTe4/MoS2 heterojunction with a noncentrosymmetric active region, which can detect and amplify the CPGE photocurrents for all directions, with a CPGE gain of 25. Thereupon, we achieve tens of μA/W CPGE responsivity from visible to near-infrared (NIR) and wide acceptance angles from 45° to −45° at room temperature, revealing multiscenario applications. The full Stokes spatially resolved mapping of the NIR vortex beam demonstrates its practical applicability as a polarimeter with high sensitivity. Our work provides an approach to developing nanostructured polarimeters controlled by inversion symmetry and devoid of external amplification modules, which leads to potential applications for future nanophotonics and optoelectronic nanodevices.
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来源期刊
ACS Nano
ACS Nano 工程技术-材料科学:综合
CiteScore
26.00
自引率
4.10%
发文量
1627
审稿时长
1.7 months
期刊介绍: ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.
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