多壁碳纳米管负载掺杂钒酸锌光催化剂对吖啶橙染料的增强降解

IF 2.8 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Hamdah S. Alanazi, Alanood Sulaiman Ababtain, Rajeh Alotaibi, Ali Aloriny, Imran Hasan, Fahad Alharthi
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引用次数: 0

摘要

吖啶橙(AO)染料是应用最广泛的有机染料之一。然而,吖啶橙染料对水生环境和人类都有严重的负面影响。因此,监测吖啶橙染料的存在是至关重要的。本文报道了一种新型复合材料的设计和合成,用于去除水中的吖啶橙染料。本文报道了水热辅助合成掺杂钒酸锌(Zn3V2O8)修饰的多壁碳纳米管(MWCNT)复合材料。通过XRD对In-ZnV@MWCNT复合材料的相纯度、结晶性质和结构进行了表征。通过扫描电镜和透射电镜研究了In-ZnV@MWCNT的表面形貌等结构特性。利用FTIR、XPS、uv -可见光谱和EDX等方法研究了In-ZnV@MWCNT复合材料的其他理化性质。随后,在紫外光下测定了In-ZnV@MWCNT的光催化活性。在pH = 3的条件下,20 mg In-ZnV@MWCNT对AO染料的光降解效果最好。使用In-ZnV@MWCNT对AO染料的光催化降解性能最高,达到99.60%以上。In-ZnV@MWCNT在5次循环中也表现出良好的稳定性。在此,我们提出了一种新型、环保、经济、稳定、高效的光催化剂来去除AO染料。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Multiwalled carbon nanotube supported indium doped zinc vanadate photocatalyst for enhanced degradation of acridine orange dye

Acridine orange (AO) dye is one of the most widely used organic dye in various applications. However, acridine orange dye has some serious negative impacts for aquatic environments and human beings. Therefore, it is very crucial to monitor the presence of acridine orange dye. This work reported the design and synthesis of a novel composite material for the removal of acridine orange dye from aqueous solution. Herein, we reported the hydrothermal assisted synthesis of indium doped zinc vanadate (Zn3V2O8) decorated multi-walled carbon nanotubes (MWCNT) composite. The phase purity, crystalline nature and formation of the In-ZnV@MWCNT composite have been authenticated by XRD. The structural properties such as surface morphology of the In-ZnV@MWCNT was examined by SEM and TEM studies. Other physiochemical properties of the In-ZnV@MWCNT composite were investigated by FTIR, XPS, UV–visible spectroscopy and EDX methods. Subsequently, photocatalytic activities of the In-ZnV@MWCNT have been determined under UV light. The 20 mg In-ZnV@MWCNT exhibited the highest performance for the photodegradation of AO dye under pH of 3. The highest photocatalytic AO dye degradation performance of more than 99.60% was achieved using In-ZnV@MWCNT. The In-ZnV@MWCNT also demonstrated good stability up to five cycles. Herein, we proposed a novel, eco-friendly, cost-effective, stable and highly efficient photocatalyst for the removal of AO dye.

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来源期刊
CiteScore
5.70
自引率
18.20%
发文量
229
审稿时长
2.6 months
期刊介绍: Research on Chemical Intermediates publishes current research articles and concise dynamic reviews on the properties, structures and reactivities of intermediate species in all the various domains of chemistry. The journal also contains articles in related disciplines such as spectroscopy, molecular biology and biochemistry, atmospheric and environmental sciences, catalysis, photochemistry and photophysics. In addition, special issues dedicated to specific topics in the field are regularly published.
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