Bing Wang, Zairan Yu, Shuang Chen, Nicola Da Roit, Dieter Schild, Michael Zimmermann, Yuemin Wang, Silke Behrens
{"title":"内页后盖：在纳米颗粒衍生的双功能Pd/CeO2/Al2O3催化剂上从合成气一步合成二甲醚(Angew。化学16/2025)","authors":"Bing Wang, Zairan Yu, Shuang Chen, Nicola Da Roit, Dieter Schild, Michael Zimmermann, Yuemin Wang, Silke Behrens","doi":"10.1002/ange.202505854","DOIUrl":null,"url":null,"abstract":"<p>The single-step syngas-to-dimethyl ether process offers both economic and technical advantages over the current two-step industrial synthesis. A highly active bifunctional Pd/CeO<sub>2</sub>/γ-Al<sub>2</sub>O<sub>3</sub> catalyst is reported by Yuemin Wang, Silke Behrens et al. in their Research Article (e202423273). Pd clusters/particles confined on the nanoparticulate ceria matrix feature abundant interfacial Pd<sup>2+</sup> sites and adjacent O vacancies, accounting for the superior performance in both activity and stability.\n\n <figure>\n <div><picture>\n <source></source></picture><p></p>\n </div>\n </figure></p>","PeriodicalId":7803,"journal":{"name":"Angewandte Chemie","volume":"137 16","pages":""},"PeriodicalIF":0.0000,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202505854","citationCount":"0","resultStr":"{\"title\":\"Inside Back Cover: Single-Step Synthesis of Dimethyl Ether from Syngas over Nanoparticle-Derived Bifunctional Pd/CeO2/Al2O3 Catalysts (Angew. Chem. 16/2025)\",\"authors\":\"Bing Wang, Zairan Yu, Shuang Chen, Nicola Da Roit, Dieter Schild, Michael Zimmermann, Yuemin Wang, Silke Behrens\",\"doi\":\"10.1002/ange.202505854\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>The single-step syngas-to-dimethyl ether process offers both economic and technical advantages over the current two-step industrial synthesis. A highly active bifunctional Pd/CeO<sub>2</sub>/γ-Al<sub>2</sub>O<sub>3</sub> catalyst is reported by Yuemin Wang, Silke Behrens et al. in their Research Article (e202423273). Pd clusters/particles confined on the nanoparticulate ceria matrix feature abundant interfacial Pd<sup>2+</sup> sites and adjacent O vacancies, accounting for the superior performance in both activity and stability.\\n\\n <figure>\\n <div><picture>\\n <source></source></picture><p></p>\\n </div>\\n </figure></p>\",\"PeriodicalId\":7803,\"journal\":{\"name\":\"Angewandte Chemie\",\"volume\":\"137 16\",\"pages\":\"\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2025-03-27\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://onlinelibrary.wiley.com/doi/epdf/10.1002/ange.202505854\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Angewandte Chemie\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://onlinelibrary.wiley.com/doi/10.1002/ange.202505854\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Angewandte Chemie","FirstCategoryId":"1085","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/ange.202505854","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
Inside Back Cover: Single-Step Synthesis of Dimethyl Ether from Syngas over Nanoparticle-Derived Bifunctional Pd/CeO2/Al2O3 Catalysts (Angew. Chem. 16/2025)
The single-step syngas-to-dimethyl ether process offers both economic and technical advantages over the current two-step industrial synthesis. A highly active bifunctional Pd/CeO2/γ-Al2O3 catalyst is reported by Yuemin Wang, Silke Behrens et al. in their Research Article (e202423273). Pd clusters/particles confined on the nanoparticulate ceria matrix feature abundant interfacial Pd2+ sites and adjacent O vacancies, accounting for the superior performance in both activity and stability.
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