基于等离子体催化的CO2转化研究进展与展望

Lefei Cao, Fei Qi, Nan Zhang, Yayun Pu, Xiaosheng Tang, Qiang Huang
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摘要

为了解决温室效应和能源困境的问题,将二氧化碳转化为有价值的化学品和可用的燃料是一个全球性的热点话题。本文首先综述了不同的CO2转化方法,包括热催化、生物催化、电催化、光催化和等离子体催化。然后,全面概述了目前探索的等离子体驱动CO2转换,如微波放电等离子体、滑动电弧放电等离子体、射频电感耦合等离子体和介质阻挡放电等离子体,重点介绍了它们的实验设置、成就和局限性。此外,还详细讨论了等离子体与光催化剂之间的协同作用对CO2转化的激活作用。最后,简要总结了等离子体催化CO2转化面临的挑战和未来的发展趋势。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Progress and future of CO2 conversion based on plasma catalysis

Progress and future of CO2 conversion based on plasma catalysis
To address the issues of the greenhouse effect and energy dilemma, it is a global hot topic on converting CO2 to valuable chemicals and useable fuels. In this review, firstly, we shortly summarize different CO2 conversion methods including thermal catalysis, biocatalysis, electrocatalysis, photocatalysis, and plasma catalysis. Then, a comprehensive overview of the currently explored plasma driven CO2 conversion is presented, such as microwave discharge plasma, gliding arc discharge plasma, radiofrequency inductively coupled plasma, and dielectric barrier discharge plasma, with an emphasis on their experimental setups, achievements and limitations. Furthermore, the activation of CO2 conversion via the synergistic effect between the plasma and photocatalyst is discussed in detail. Finally, the associated challenges and future development trends for plasma catalytic CO2 conversion are briefly concluded.
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