{"title":"电催化乙二醇氧化过渡金属催化剂的研究进展","authors":"Hongjing Wu, Xiaoyue Zheng, Jiajia Liu, Yanru Yuan, Yuquan Yang, Chenjing Wang, Li Zhou, Lulu Wang, Binbin Jia, Xiaoyu Fan, Jinlong Zheng","doi":"10.1039/d4nr05000b","DOIUrl":null,"url":null,"abstract":"As a small alcohol molecule with low oxidation potential, ethylene glycol is also a key monomer in the production of polyethylene terephthalate (PET). The realization of efficient ethylene glycol oxidation can further realize the recycling of waste PET. At present, there have been a lot of researches on catalysts for Ethylene glycol oxidation(EGOR), among which transition metal catalysts (including Fe, Co, Ni and other conventional non-precious metals and Pt, Pb and other precious metals) have a good application prospect in the oxidation reaction of ethylene glycol due to their unique electronic structure. In this work, the synthesis strategies of transition metal catalysts used for electrocatalytic oxidation of EG were summarized and the performance of different types of catalysts in ethylene glycol oxidation was reviewed. Advanced characterization methods were used to understand the oxidation mechanism of EG and to control the EGOR intermediates into target products. Therefore, we need to further explore efficient ethylene glycol oxidation catalysts to achieve efficient reactions.","PeriodicalId":92,"journal":{"name":"Nanoscale","volume":"95 1","pages":""},"PeriodicalIF":5.8000,"publicationDate":"2025-04-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Research progress of transition metal catalysts for electrocatalytic Ethylene glycol oxidation\",\"authors\":\"Hongjing Wu, Xiaoyue Zheng, Jiajia Liu, Yanru Yuan, Yuquan Yang, Chenjing Wang, Li Zhou, Lulu Wang, Binbin Jia, Xiaoyu Fan, Jinlong Zheng\",\"doi\":\"10.1039/d4nr05000b\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"As a small alcohol molecule with low oxidation potential, ethylene glycol is also a key monomer in the production of polyethylene terephthalate (PET). The realization of efficient ethylene glycol oxidation can further realize the recycling of waste PET. At present, there have been a lot of researches on catalysts for Ethylene glycol oxidation(EGOR), among which transition metal catalysts (including Fe, Co, Ni and other conventional non-precious metals and Pt, Pb and other precious metals) have a good application prospect in the oxidation reaction of ethylene glycol due to their unique electronic structure. In this work, the synthesis strategies of transition metal catalysts used for electrocatalytic oxidation of EG were summarized and the performance of different types of catalysts in ethylene glycol oxidation was reviewed. Advanced characterization methods were used to understand the oxidation mechanism of EG and to control the EGOR intermediates into target products. Therefore, we need to further explore efficient ethylene glycol oxidation catalysts to achieve efficient reactions.\",\"PeriodicalId\":92,\"journal\":{\"name\":\"Nanoscale\",\"volume\":\"95 1\",\"pages\":\"\"},\"PeriodicalIF\":5.8000,\"publicationDate\":\"2025-04-12\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nanoscale\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1039/d4nr05000b\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nanoscale","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1039/d4nr05000b","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Research progress of transition metal catalysts for electrocatalytic Ethylene glycol oxidation
As a small alcohol molecule with low oxidation potential, ethylene glycol is also a key monomer in the production of polyethylene terephthalate (PET). The realization of efficient ethylene glycol oxidation can further realize the recycling of waste PET. At present, there have been a lot of researches on catalysts for Ethylene glycol oxidation(EGOR), among which transition metal catalysts (including Fe, Co, Ni and other conventional non-precious metals and Pt, Pb and other precious metals) have a good application prospect in the oxidation reaction of ethylene glycol due to their unique electronic structure. In this work, the synthesis strategies of transition metal catalysts used for electrocatalytic oxidation of EG were summarized and the performance of different types of catalysts in ethylene glycol oxidation was reviewed. Advanced characterization methods were used to understand the oxidation mechanism of EG and to control the EGOR intermediates into target products. Therefore, we need to further explore efficient ethylene glycol oxidation catalysts to achieve efficient reactions.
期刊介绍:
Nanoscale is a high-impact international journal, publishing high-quality research across nanoscience and nanotechnology. Nanoscale publishes a full mix of research articles on experimental and theoretical work, including reviews, communications, and full papers.Highly interdisciplinary, this journal appeals to scientists, researchers and professionals interested in nanoscience and nanotechnology, quantum materials and quantum technology, including the areas of physics, chemistry, biology, medicine, materials, energy/environment, information technology, detection science, healthcare and drug discovery, and electronics.