半heusler拓扑半金属GdPtBi异常磁输运性质的调谐。

IF 12.2 2区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Orest Pavlosiuk, Piotr Wiśniewski, Romain Grasset, Marcin Konczykowski, Andrzej Ptok, Dariusz Kaczorowski
{"title":"半heusler拓扑半金属GdPtBi异常磁输运性质的调谐。","authors":"Orest Pavlosiuk, Piotr Wiśniewski, Romain Grasset, Marcin Konczykowski, Andrzej Ptok, Dariusz Kaczorowski","doi":"10.1039/d4mh01875c","DOIUrl":null,"url":null,"abstract":"<p><p>Half-Heusler compounds from the <i>RE</i>PtBi family exemplify Weyl semimetals in which an external magnetic field induces Weyl nodes. These materials exceptionally host topologically non-trivial states near the Fermi level and their manifestation can be clearly seen in the magnetotransport properties. In this study, we tune the Fermi level of the archetypal half-Heusler Weyl semimetal GdPtBi through high-energy electron irradiation, moving it away from the Weyl nodes to investigate the resilience of the contribution of topologically non-trivial states to magnetotransport properties. Remarkably, we observe that the negative longitudinal magnetoresistance, which is a definitive indicator of the chiral magnetic anomaly occurring in topological semimetals, persists even when the Fermi level is shifted by 100 meV from its original position in the pristine sample. Additionally, the anomalous Hall effect shows complex variations as the Fermi level is altered, attributed to the energy-dependent nature of the Berry curvature, which arises from avoided band crossing. Our findings show the robust influence of Weyl nodes on the magneto-transport properties of GdPtBi, irrespective of the Fermi level position, a behaviour likely applicable to many half-Heusler Weyl semimetals.</p>","PeriodicalId":87,"journal":{"name":"Materials Horizons","volume":" ","pages":""},"PeriodicalIF":12.2000,"publicationDate":"2025-04-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Tuning of anomalous magnetotransport properties in half-Heusler topological semimetal GdPtBi.\",\"authors\":\"Orest Pavlosiuk, Piotr Wiśniewski, Romain Grasset, Marcin Konczykowski, Andrzej Ptok, Dariusz Kaczorowski\",\"doi\":\"10.1039/d4mh01875c\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Half-Heusler compounds from the <i>RE</i>PtBi family exemplify Weyl semimetals in which an external magnetic field induces Weyl nodes. These materials exceptionally host topologically non-trivial states near the Fermi level and their manifestation can be clearly seen in the magnetotransport properties. In this study, we tune the Fermi level of the archetypal half-Heusler Weyl semimetal GdPtBi through high-energy electron irradiation, moving it away from the Weyl nodes to investigate the resilience of the contribution of topologically non-trivial states to magnetotransport properties. Remarkably, we observe that the negative longitudinal magnetoresistance, which is a definitive indicator of the chiral magnetic anomaly occurring in topological semimetals, persists even when the Fermi level is shifted by 100 meV from its original position in the pristine sample. Additionally, the anomalous Hall effect shows complex variations as the Fermi level is altered, attributed to the energy-dependent nature of the Berry curvature, which arises from avoided band crossing. Our findings show the robust influence of Weyl nodes on the magneto-transport properties of GdPtBi, irrespective of the Fermi level position, a behaviour likely applicable to many half-Heusler Weyl semimetals.</p>\",\"PeriodicalId\":87,\"journal\":{\"name\":\"Materials Horizons\",\"volume\":\" \",\"pages\":\"\"},\"PeriodicalIF\":12.2000,\"publicationDate\":\"2025-04-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Materials Horizons\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1039/d4mh01875c\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Materials Horizons","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1039/d4mh01875c","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

来自REPtBi家族的半heusler化合物是外磁场诱导Weyl节点的Weyl半金属的例子。这些材料在费米能级附近异常地拥有拓扑非平凡态,它们的表现可以在磁输运性质中清楚地看到。在这项研究中,我们通过高能电子辐照调整原型半heusler Weyl半金属GdPtBi的费米能级,将其从Weyl节点移开,以研究拓扑非平凡态对磁输运性质贡献的弹性。值得注意的是,我们观察到负纵向磁电阻(这是拓扑半金属中发生手性磁异常的明确指标)即使在原始样品中的费米能级从其原始位置移动100 meV时仍然存在。此外,反常霍尔效应显示出复杂的变化,随着费米能级的改变,归因于贝里曲率的能量依赖性质,这是由避免带交叉引起的。我们的研究结果表明,无论费米能级位置如何,Weyl节点对GdPtBi的磁输运特性都有强大的影响,这种行为可能适用于许多半heusler Weyl半金属。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Tuning of anomalous magnetotransport properties in half-Heusler topological semimetal GdPtBi.

Half-Heusler compounds from the REPtBi family exemplify Weyl semimetals in which an external magnetic field induces Weyl nodes. These materials exceptionally host topologically non-trivial states near the Fermi level and their manifestation can be clearly seen in the magnetotransport properties. In this study, we tune the Fermi level of the archetypal half-Heusler Weyl semimetal GdPtBi through high-energy electron irradiation, moving it away from the Weyl nodes to investigate the resilience of the contribution of topologically non-trivial states to magnetotransport properties. Remarkably, we observe that the negative longitudinal magnetoresistance, which is a definitive indicator of the chiral magnetic anomaly occurring in topological semimetals, persists even when the Fermi level is shifted by 100 meV from its original position in the pristine sample. Additionally, the anomalous Hall effect shows complex variations as the Fermi level is altered, attributed to the energy-dependent nature of the Berry curvature, which arises from avoided band crossing. Our findings show the robust influence of Weyl nodes on the magneto-transport properties of GdPtBi, irrespective of the Fermi level position, a behaviour likely applicable to many half-Heusler Weyl semimetals.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Materials Horizons
Materials Horizons CHEMISTRY, MULTIDISCIPLINARY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
18.90
自引率
2.30%
发文量
306
审稿时长
1.3 months
期刊介绍: Materials Horizons is a leading journal in materials science that focuses on publishing exceptionally high-quality and innovative research. The journal prioritizes original research that introduces new concepts or ways of thinking, rather than solely reporting technological advancements. However, groundbreaking articles featuring record-breaking material performance may also be published. To be considered for publication, the work must be of significant interest to our community-spanning readership. Starting from 2021, all articles published in Materials Horizons will be indexed in MEDLINE©. The journal publishes various types of articles, including Communications, Reviews, Opinion pieces, Focus articles, and Comments. It serves as a core journal for researchers from academia, government, and industry across all areas of materials research. Materials Horizons is a Transformative Journal and compliant with Plan S. It has an impact factor of 13.3 and is indexed in MEDLINE.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信