ZSM-5沸石催化乙醇制烃反应催化剂改性研究进展

IF 5.9 3区工程技术 Q1 CHEMISTRY, MULTIDISCIPLINARY

Journal of Industrial and Engineering Chemistry Pub Date : 2024-11-17 DOI:10.1016/j.jiec.2024.11.031

Yiyang Lin , Haitao Yin , Shuang Chen , Jiaqi Wang , Wen Li , Yining Gao , Mingyuan Sheng , Nanzhe Jiang

{"title":"ZSM-5沸石催化乙醇制烃反应催化剂改性研究进展","authors":"Yiyang Lin , Haitao Yin , Shuang Chen , Jiaqi Wang , Wen Li , Yining Gao , Mingyuan Sheng , Nanzhe Jiang","doi":"10.1016/j.jiec.2024.11.031","DOIUrl":null,"url":null,"abstract":"<div><div>Ethanol-to-hydrocarbons (ETH) conversion represents a pivotal reaction in non-homogeneous catalysis, offering a sustainable solution for the production of significant platform chemicals, including olefins, gasoline, and aromatics. However, it is imperative to continue enhancing the catalytic efficiency and extending the operational longevity of the catalysts. This review presents a comprehensive overview of the latest research developments in the field of catalytic conversion of ethanol to hydrocarbons. It emphasizes the pivotal role of zeolite catalysts in the conversion of ethanol to hydrocarbons and offers insights into the recent scientific discoveries pertaining to the reaction mechanism of ETH conversion. In addition, we investigate the catalyst optimization and design, with the objective of enhancing the selectivity of the target product and prolonging the catalyst life. This topic has not been fully addressed in recent reviews. The aim of this review is to offer theoretical insights into the ETH reaction mechanism and to guide the development of more efficient ETH catalysts.</div></div>","PeriodicalId":363,"journal":{"name":"Journal of Industrial and Engineering Chemistry","volume":"146 ","pages":"Pages 87-108"},"PeriodicalIF":5.9000,"publicationDate":"2024-11-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Research and progress in catalyst modification for ZSM-5 zeolite catalyzed ethanol-to hydrocarbon reaction\",\"authors\":\"Yiyang Lin , Haitao Yin , Shuang Chen , Jiaqi Wang , Wen Li , Yining Gao , Mingyuan Sheng , Nanzhe Jiang\",\"doi\":\"10.1016/j.jiec.2024.11.031\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Ethanol-to-hydrocarbons (ETH) conversion represents a pivotal reaction in non-homogeneous catalysis, offering a sustainable solution for the production of significant platform chemicals, including olefins, gasoline, and aromatics. However, it is imperative to continue enhancing the catalytic efficiency and extending the operational longevity of the catalysts. This review presents a comprehensive overview of the latest research developments in the field of catalytic conversion of ethanol to hydrocarbons. It emphasizes the pivotal role of zeolite catalysts in the conversion of ethanol to hydrocarbons and offers insights into the recent scientific discoveries pertaining to the reaction mechanism of ETH conversion. In addition, we investigate the catalyst optimization and design, with the objective of enhancing the selectivity of the target product and prolonging the catalyst life. This topic has not been fully addressed in recent reviews. The aim of this review is to offer theoretical insights into the ETH reaction mechanism and to guide the development of more efficient ETH catalysts.</div></div>\",\"PeriodicalId\":363,\"journal\":{\"name\":\"Journal of Industrial and Engineering Chemistry\",\"volume\":\"146 \",\"pages\":\"Pages 87-108\"},\"PeriodicalIF\":5.9000,\"publicationDate\":\"2024-11-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Industrial and Engineering Chemistry\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1226086X24007706\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Industrial and Engineering Chemistry","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1226086X24007706","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}

引用次数: 0

摘要

乙醇制碳氢化合物（ETH）转化是非均相催化反应中的一个关键反应，为烯烃、汽油和芳烃等重要平台化学品的生产提供了一种可持续的解决方案。然而，当务之急是继续提高催化效率，延长催化剂的使用寿命。本综述全面概述了乙醇催化转化为碳氢化合物领域的最新研究进展。它强调了沸石催化剂在乙醇转化为碳氢化合物过程中的关键作用，并深入探讨了有关 ETH 转化反应机理的最新科学发现。此外，我们还研究了催化剂的优化和设计，目的是提高目标产物的选择性并延长催化剂的使用寿命。在最近的综述中，这一主题尚未得到充分讨论。本综述旨在提供有关 ETH 反应机理的理论见解，并为开发更高效的 ETH 催化剂提供指导。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

Research and progress in catalyst modification for ZSM-5 zeolite catalyzed ethanol-to hydrocarbon reaction

查看原文本刊更多论文

Research and progress in catalyst modification for ZSM-5 zeolite catalyzed ethanol-to hydrocarbon reaction

Ethanol-to-hydrocarbons (ETH) conversion represents a pivotal reaction in non-homogeneous catalysis, offering a sustainable solution for the production of significant platform chemicals, including olefins, gasoline, and aromatics. However, it is imperative to continue enhancing the catalytic efficiency and extending the operational longevity of the catalysts. This review presents a comprehensive overview of the latest research developments in the field of catalytic conversion of ethanol to hydrocarbons. It emphasizes the pivotal role of zeolite catalysts in the conversion of ethanol to hydrocarbons and offers insights into the recent scientific discoveries pertaining to the reaction mechanism of ETH conversion. In addition, we investigate the catalyst optimization and design, with the objective of enhancing the selectivity of the target product and prolonging the catalyst life. This topic has not been fully addressed in recent reviews. The aim of this review is to offer theoretical insights into the ETH reaction mechanism and to guide the development of more efficient ETH catalysts.

求助全文

通过发布文献求助，成功后即可免费获取论文全文。去求助

来源期刊

Journal of Industrial and Engineering Chemistry 工程技术-工程：化工

CiteScore

10.40

自引率

6.60%

发文量

639

审稿时长

29 days

期刊介绍： Journal of Industrial and Engineering Chemistry is published monthly in English by the Korean Society of Industrial and Engineering Chemistry. JIEC brings together multidisciplinary interests in one journal and is to disseminate information on all aspects of research and development in industrial and engineering chemistry. Contributions in the form of research articles, short communications, notes and reviews are considered for publication. The editors welcome original contributions that have not been and are not to be published elsewhere. Instruction to authors and a manuscript submissions form are printed at the end of each issue. Bulk reprints of individual articles can be ordered. This publication is partially supported by Korea Research Foundation and the Korean Federation of Science and Technology Societies.