推进环保磷化铟量子点:实现宽色域显示纯色发光的综合策略

IF 19.3 1区 材料科学 Q1 CHEMISTRY, PHYSICAL
Jie Zhao, Rui Jiang, Maoyuan Huang, Yifei Qiao, Sinong Wang, Wanlu Zhang, Pengfei Tian, Jun Wang, Ruiqian Guo, Shiliang Mei
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引用次数: 0

摘要

磷化铟(InP)量子点(QDs)是下一代显示器和光电子学中有前途的环保发射器,具有高效率,窄谱线宽度和可调谐的发光。然而,由于合成和制造困难,它们的商业化面临挑战,特别是在提高光致发光量子产率(PLQY),半最大全宽度(FWHM)和外部量子效率(EQE)方面进展缓慢。尽管存在稳定性和使用寿命等共同挑战,但InP量子点的更宽FWHM已日益成为其商业化的关键瓶颈,特别是考虑到最近的突破,包括纯核/核壳InP量子点的近统一PLQY和电致发光应用中超过20%的EQE。本文综述了InP量子点中FWHM的扩展机制,并概述了通过尺寸、晶格、带隙、表面和器件结构工程来缩小FWHM的策略。它还强调了高性能InP量子点及其电致发光应用的趋势和未来方向,旨在推进其在无重金属显示和光电子领域的商业化。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Advancing Ecofriendly Indium Phosphide Quantum Dots: Comprehensive Strategies toward Color-Pure Luminescence for Wide Color Gamut Displays

Advancing Ecofriendly Indium Phosphide Quantum Dots: Comprehensive Strategies toward Color-Pure Luminescence for Wide Color Gamut Displays
Indium phosphide (InP) quantum dots (QDs) are promising eco-friendly emitters for next-generation displays and optoelectronics, offering high efficiency, narrow spectral linewidths, and tunable luminescence. However, their commercialization faces challenges due to synthesis and fabrication difficulties, particularly slow progress in improving photoluminescence quantum yield (PLQY), full-width at half-maximum (FWHM), and external quantum efficiency (EQE). Despite persistent shared challenges such as stability and operational lifetime, the broader FWHM of InP QDs has increasingly emerged as a critical bottleneck for their commercialization, especially given recent breakthroughs, including near-unity PLQY in core-only/core–shell InP QDs and over 20% EQE in their electroluminescent applications. This review examines FWHM broadening mechanisms in InP QDs and outlines strategies to narrow FWHM through size, lattice, bandgap, surface, and device architecture engineering. It also highlights trends and future directions for high-performance InP QDs and their electroluminescent applications, aiming to advance their commercialization in heavy metal-free displays and optoelectronics.
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来源期刊
ACS Energy Letters
ACS Energy Letters Energy-Renewable Energy, Sustainability and the Environment
CiteScore
31.20
自引率
5.00%
发文量
469
审稿时长
1 months
期刊介绍: ACS Energy Letters is a monthly journal that publishes papers reporting new scientific advances in energy research. The journal focuses on topics that are of interest to scientists working in the fundamental and applied sciences. Rapid publication is a central criterion for acceptance, and the journal is known for its quick publication times, with an average of 4-6 weeks from submission to web publication in As Soon As Publishable format. ACS Energy Letters is ranked as the number one journal in the Web of Science Electrochemistry category. It also ranks within the top 10 journals for Physical Chemistry, Energy & Fuels, and Nanoscience & Nanotechnology. The journal offers several types of articles, including Letters, Energy Express, Perspectives, Reviews, Editorials, Viewpoints and Energy Focus. Additionally, authors have the option to submit videos that summarize or support the information presented in a Perspective or Review article, which can be highlighted on the journal's website. ACS Energy Letters is abstracted and indexed in Chemical Abstracts Service/SciFinder, EBSCO-summon, PubMed, Web of Science, Scopus and Portico.
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