介孔聚合物上生物质基糠醛电氧化制5-羟基-2(5H)-呋喃酮的机理研究

IF 4.2 2区化学 Q2 CHEMISTRY, MULTIDISCIPLINARY

Chemical Communications Pub Date : 2025-04-09 DOI:10.1039/d5cc01004g

Weixia Zhu , Runlu Yang , Xin Wang , Keying Dai , Chang Su , Jiaxi Duan , Chun Chang , Haoran Wu

引用次数: 0

摘要

首次报道了生物质衍生糠醛在三种球形介孔聚合物（介孔- pda、介孔- ppy和介孔- pmpd）上电氧化制备高附加值5-羟基-2(5H)-呋喃酮（HFO）。结果表明，介观pda具有较高的法拉第效率（92.6%）、选择性（96.4%）和转化率（79.6%）。揭示了高性能背后的机制。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

Mechanistic insights into biomass-based furfural electrooxidation to 5-hydroxy-2(5H)-furanone over mesoporous polymers†

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Mechanistic insights into biomass-based furfural electrooxidation to 5-hydroxy-2(5H)-furanone over mesoporous polymers†

Electrooxidation of biomass-derived furfural to high-value-added 5-hydroxy-2(5H)-furanone (HFO) over three spherical mesoporous polymers (meso-PDA, meso-PPy, and meso-PmPD) is reported for the first time. The results indicate that the meso-PDA delivers the best performance with high faradaic efficiency (92.6%), selectivity (96.4%) and conversion (79.6%). The mechanism behind the high performance was revealed.

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来源期刊

Chemical Communications 化学-化学综合

CiteScore

8.60

自引率

4.10%

发文量

2705

审稿时长

1.4 months

期刊介绍： ChemComm (Chemical Communications) is renowned as the fastest publisher of articles providing information on new avenues of research, drawn from all the world''s major areas of chemical research.