{"title":"密度对赤泥基盾构射线衰减特性的内在影响","authors":"Rahul Arya , Rini Paulose , Abhijit Bijanu , Varsha Agrawal , Rahitashya Shil , Deepti Mishra , Kaushik Banerjee , Sujoy Chatterjee , Sarmishtha Bhattacharyya , Abhay Bhisikar , Paparao Mondi , Upendra Singh , Jyoti Pendam , Shabi Thankaraj Salammal","doi":"10.1016/j.radphyschem.2025.112757","DOIUrl":null,"url":null,"abstract":"<div><div>High-energy radiation shielding materials are vital for protecting against radiation hazards. Both the atomic number and density of the shield plays a prominent role in attenuating high-energy photons. This study reports the inherent role of density on the gamma ray attenuation characteristics of the shields. The radiation shields with various densities between 2.12 to 5.23 g/cm<sup>3</sup> were fabricated by varying their porosity through hot compaction rather than altering their compositions or materials as reported in literatures. Red mud (100 %) (Alumina industry waste) (RM) and red mud:Bi<sub>2</sub>O<sub>3</sub> (50:50 wt%) mixtures (RMBi) were used to fabricate the shields. For example, the RMBi samples with density varying between 2.63 to 5.23 g/cm<sup>3</sup> were prepared by applying 0–39.02 MPa pressure at 1000 °C. Eventually, the porosity of RMBi sample has decreased from 50 % to 2 % while increasing the pressure. The compressive strength of RMBi samples are 6.8, 101.8, 243.2 and 283.3 MPa. The gamma ray attenuation characteristics of the shields were studied using <sup>22</sup>Na source (0.511 and 1.274 MeV) in a narrow beam geometry. The linear attenuation coefficient (μ) of RMBi sample was found to increase from 0.0176 to 0.0272 mm<sup>-1</sup> while increasing the density from 2.63 to 5.23 g/cm<sup>3</sup>. The attenuation characteristics such as μ, half value layer and mean free path are well in agreement with the theoretical values obtained through Phy-X/PSD software except the effective atomic number (Z<sub>eff</sub>). The Compton backscattering experiment was performed using <sup>137</sup>Cs point source (0.662 MeV) to determine Z<sub>eff</sub>. The Z<sub>eff</sub> of RMBi sample was noticed to increase from 20.99 to 40.92 while increasing the density of the shield whereas the Z<sub>eff</sub> stays constant (19.90) when calculated using Phy-X/PSD software.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"234 ","pages":"Article 112757"},"PeriodicalIF":2.8000,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Inherent role of density on the gamma ray attenuation characteristics of red mud based shield\",\"authors\":\"Rahul Arya , Rini Paulose , Abhijit Bijanu , Varsha Agrawal , Rahitashya Shil , Deepti Mishra , Kaushik Banerjee , Sujoy Chatterjee , Sarmishtha Bhattacharyya , Abhay Bhisikar , Paparao Mondi , Upendra Singh , Jyoti Pendam , Shabi Thankaraj Salammal\",\"doi\":\"10.1016/j.radphyschem.2025.112757\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>High-energy radiation shielding materials are vital for protecting against radiation hazards. Both the atomic number and density of the shield plays a prominent role in attenuating high-energy photons. This study reports the inherent role of density on the gamma ray attenuation characteristics of the shields. The radiation shields with various densities between 2.12 to 5.23 g/cm<sup>3</sup> were fabricated by varying their porosity through hot compaction rather than altering their compositions or materials as reported in literatures. Red mud (100 %) (Alumina industry waste) (RM) and red mud:Bi<sub>2</sub>O<sub>3</sub> (50:50 wt%) mixtures (RMBi) were used to fabricate the shields. For example, the RMBi samples with density varying between 2.63 to 5.23 g/cm<sup>3</sup> were prepared by applying 0–39.02 MPa pressure at 1000 °C. Eventually, the porosity of RMBi sample has decreased from 50 % to 2 % while increasing the pressure. The compressive strength of RMBi samples are 6.8, 101.8, 243.2 and 283.3 MPa. The gamma ray attenuation characteristics of the shields were studied using <sup>22</sup>Na source (0.511 and 1.274 MeV) in a narrow beam geometry. The linear attenuation coefficient (μ) of RMBi sample was found to increase from 0.0176 to 0.0272 mm<sup>-1</sup> while increasing the density from 2.63 to 5.23 g/cm<sup>3</sup>. The attenuation characteristics such as μ, half value layer and mean free path are well in agreement with the theoretical values obtained through Phy-X/PSD software except the effective atomic number (Z<sub>eff</sub>). The Compton backscattering experiment was performed using <sup>137</sup>Cs point source (0.662 MeV) to determine Z<sub>eff</sub>. The Z<sub>eff</sub> of RMBi sample was noticed to increase from 20.99 to 40.92 while increasing the density of the shield whereas the Z<sub>eff</sub> stays constant (19.90) when calculated using Phy-X/PSD software.</div></div>\",\"PeriodicalId\":20861,\"journal\":{\"name\":\"Radiation Physics and Chemistry\",\"volume\":\"234 \",\"pages\":\"Article 112757\"},\"PeriodicalIF\":2.8000,\"publicationDate\":\"2025-03-27\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Radiation Physics and Chemistry\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0969806X2500249X\",\"RegionNum\":3,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Radiation Physics and Chemistry","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0969806X2500249X","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Inherent role of density on the gamma ray attenuation characteristics of red mud based shield
High-energy radiation shielding materials are vital for protecting against radiation hazards. Both the atomic number and density of the shield plays a prominent role in attenuating high-energy photons. This study reports the inherent role of density on the gamma ray attenuation characteristics of the shields. The radiation shields with various densities between 2.12 to 5.23 g/cm3 were fabricated by varying their porosity through hot compaction rather than altering their compositions or materials as reported in literatures. Red mud (100 %) (Alumina industry waste) (RM) and red mud:Bi2O3 (50:50 wt%) mixtures (RMBi) were used to fabricate the shields. For example, the RMBi samples with density varying between 2.63 to 5.23 g/cm3 were prepared by applying 0–39.02 MPa pressure at 1000 °C. Eventually, the porosity of RMBi sample has decreased from 50 % to 2 % while increasing the pressure. The compressive strength of RMBi samples are 6.8, 101.8, 243.2 and 283.3 MPa. The gamma ray attenuation characteristics of the shields were studied using 22Na source (0.511 and 1.274 MeV) in a narrow beam geometry. The linear attenuation coefficient (μ) of RMBi sample was found to increase from 0.0176 to 0.0272 mm-1 while increasing the density from 2.63 to 5.23 g/cm3. The attenuation characteristics such as μ, half value layer and mean free path are well in agreement with the theoretical values obtained through Phy-X/PSD software except the effective atomic number (Zeff). The Compton backscattering experiment was performed using 137Cs point source (0.662 MeV) to determine Zeff. The Zeff of RMBi sample was noticed to increase from 20.99 to 40.92 while increasing the density of the shield whereas the Zeff stays constant (19.90) when calculated using Phy-X/PSD software.
期刊介绍:
Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing.
The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.