Ke-Yu Yao , Derek Ka-Hei Lai , Hyo-Jung Lim , Bryan Pak-Hei So , Andy Chi-Ho Chan , Patrick Yiu-Man Yip , Duo Wai-Chi Wong , Bingyang Dai , Xin Zhao , Siu Hong Dexter Wong , James Chung-Wai Cheung
{"title":"2H-MoS2润滑增强MWCNT纳米复合材料用于精细生物运动压阻检测与深度学习集成","authors":"Ke-Yu Yao , Derek Ka-Hei Lai , Hyo-Jung Lim , Bryan Pak-Hei So , Andy Chi-Ho Chan , Patrick Yiu-Man Yip , Duo Wai-Chi Wong , Bingyang Dai , Xin Zhao , Siu Hong Dexter Wong , James Chung-Wai Cheung","doi":"10.1016/j.matdes.2025.113861","DOIUrl":null,"url":null,"abstract":"<div><div>Intelligent piezoresistive health monitoring systems integrate advanced nanocomposite architectures with precise algorithmic analysis for real-time physiological assessment. However, existing works often prioritize high sensitivity at the expense of strain tolerance and require complex fabrication procedures. Herein, we present an environmentally friendly, low-cost, and nonionic fabrication approach for a 2H-phase molybdenum disulfide (2H-MoS<sub>2</sub>)-enhanced multi-walled carbon nanotube (MWCNT) strain sensor, developed via a systematically optimized vacuum-assisted filtration process. This study is the first to validate the dual enhancement effect of MoS<sub>2</sub>, leveraging its shear-exfoliation properties to simultaneously improve strain gauge performance and mechanical robustness. The resulting nacre-like layered hybrid nanocomposite achieves a remarkable gauge factor of 675.7 (R<sup>2</sup>∼0.993) at low strain (∼0–4.5 %), representing a 3881.5 % improvement over pure MWCNT systems, alongside enhanced toughness (∼89.17 %) and strain tolerance (∼53.93 %). Meanwhile, the optimized composition ensures low rest-state resistance (∼13.1 Ω), minimal hysteresis (∼5.7 %), and robust durability over 5000 cycles at 10 % strain. As a result, the proposed sensor enables highly consistent, high-fidelity monitoring of various subtle-to-moderate biomotions. Integrated with a fine-tuned InceptionTime deep learning model, it achieves an F1-score of 98 % in classifying Dysphagia Diet Standardization Initiative (IDDSI)-standard swallowing activities, demonstrating its potential for AI-driven health monitoring applications.</div></div>","PeriodicalId":383,"journal":{"name":"Materials & Design","volume":"253 ","pages":"Article 113861"},"PeriodicalIF":7.6000,"publicationDate":"2025-03-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"2H-MoS2 lubrication-enhanced MWCNT nanocomposite for subtle bio-motion piezoresistive detection with deep learning integration\",\"authors\":\"Ke-Yu Yao , Derek Ka-Hei Lai , Hyo-Jung Lim , Bryan Pak-Hei So , Andy Chi-Ho Chan , Patrick Yiu-Man Yip , Duo Wai-Chi Wong , Bingyang Dai , Xin Zhao , Siu Hong Dexter Wong , James Chung-Wai Cheung\",\"doi\":\"10.1016/j.matdes.2025.113861\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Intelligent piezoresistive health monitoring systems integrate advanced nanocomposite architectures with precise algorithmic analysis for real-time physiological assessment. However, existing works often prioritize high sensitivity at the expense of strain tolerance and require complex fabrication procedures. Herein, we present an environmentally friendly, low-cost, and nonionic fabrication approach for a 2H-phase molybdenum disulfide (2H-MoS<sub>2</sub>)-enhanced multi-walled carbon nanotube (MWCNT) strain sensor, developed via a systematically optimized vacuum-assisted filtration process. This study is the first to validate the dual enhancement effect of MoS<sub>2</sub>, leveraging its shear-exfoliation properties to simultaneously improve strain gauge performance and mechanical robustness. The resulting nacre-like layered hybrid nanocomposite achieves a remarkable gauge factor of 675.7 (R<sup>2</sup>∼0.993) at low strain (∼0–4.5 %), representing a 3881.5 % improvement over pure MWCNT systems, alongside enhanced toughness (∼89.17 %) and strain tolerance (∼53.93 %). Meanwhile, the optimized composition ensures low rest-state resistance (∼13.1 Ω), minimal hysteresis (∼5.7 %), and robust durability over 5000 cycles at 10 % strain. As a result, the proposed sensor enables highly consistent, high-fidelity monitoring of various subtle-to-moderate biomotions. Integrated with a fine-tuned InceptionTime deep learning model, it achieves an F1-score of 98 % in classifying Dysphagia Diet Standardization Initiative (IDDSI)-standard swallowing activities, demonstrating its potential for AI-driven health monitoring applications.</div></div>\",\"PeriodicalId\":383,\"journal\":{\"name\":\"Materials & Design\",\"volume\":\"253 \",\"pages\":\"Article 113861\"},\"PeriodicalIF\":7.6000,\"publicationDate\":\"2025-03-26\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Materials & Design\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0264127525002813\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Materials & Design","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0264127525002813","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
2H-MoS2 lubrication-enhanced MWCNT nanocomposite for subtle bio-motion piezoresistive detection with deep learning integration
Intelligent piezoresistive health monitoring systems integrate advanced nanocomposite architectures with precise algorithmic analysis for real-time physiological assessment. However, existing works often prioritize high sensitivity at the expense of strain tolerance and require complex fabrication procedures. Herein, we present an environmentally friendly, low-cost, and nonionic fabrication approach for a 2H-phase molybdenum disulfide (2H-MoS2)-enhanced multi-walled carbon nanotube (MWCNT) strain sensor, developed via a systematically optimized vacuum-assisted filtration process. This study is the first to validate the dual enhancement effect of MoS2, leveraging its shear-exfoliation properties to simultaneously improve strain gauge performance and mechanical robustness. The resulting nacre-like layered hybrid nanocomposite achieves a remarkable gauge factor of 675.7 (R2∼0.993) at low strain (∼0–4.5 %), representing a 3881.5 % improvement over pure MWCNT systems, alongside enhanced toughness (∼89.17 %) and strain tolerance (∼53.93 %). Meanwhile, the optimized composition ensures low rest-state resistance (∼13.1 Ω), minimal hysteresis (∼5.7 %), and robust durability over 5000 cycles at 10 % strain. As a result, the proposed sensor enables highly consistent, high-fidelity monitoring of various subtle-to-moderate biomotions. Integrated with a fine-tuned InceptionTime deep learning model, it achieves an F1-score of 98 % in classifying Dysphagia Diet Standardization Initiative (IDDSI)-standard swallowing activities, demonstrating its potential for AI-driven health monitoring applications.
期刊介绍:
Materials and Design is a multi-disciplinary journal that publishes original research reports, review articles, and express communications. The journal focuses on studying the structure and properties of inorganic and organic materials, advancements in synthesis, processing, characterization, and testing, the design of materials and engineering systems, and their applications in technology. It aims to bring together various aspects of materials science, engineering, physics, and chemistry.
The journal explores themes ranging from materials to design and aims to reveal the connections between natural and artificial materials, as well as experiment and modeling. Manuscripts submitted to Materials and Design should contain elements of discovery and surprise, as they often contribute new insights into the architecture and function of matter.