{"title":"基于垂直热传导结构和基于传感器响应过程的神经网络预测算法的超快氢气探测系统","authors":"Ruilin Yang, Zhen Yuan*, Changrong Jiang, Xinjie Zhang, Zilong Qiao, Jianping Zhang, Junge Liang, Si Wang, Zaihua Duan, Yuanming Wu, Weizhi Li*, Yadong Jiang and Huiling Tai*, ","doi":"10.1021/acssensors.4c0348710.1021/acssensors.4c03487","DOIUrl":null,"url":null,"abstract":"<p >Hydrogen detection plays a crucial role in various scenes of hydrogen energy such as hydrogen vehicles, hydrogen transportation and hydrogen storage. It is essential to develop a hydrogen detection system with ultrafast response times (<1 s) for the timely detection of hydrogen leaks. Here we report an ultrafast (0.4 s) hydrogen detection system based on a wafer-scale fabrication process. It consists of a low power (20.2 mW) hydrogen sensor based on vertical thermal conduction structure and a signal processing circuit introduced with a neural network prediction algorithm based on sensor response process. The fabricated sensor exhibits rapid response, wide detection range, and wide operating temperature, while showing good long-term stability and excellent selectivity. Meanwhile, the model significantly enhanced the detection speed by enabling hydrogen concentration prediction using only the initial 40 data points (sampling frequency of 100 Hz) from the sensor response before the sensor completes the entire response process. This work introduces a novel approach to achieve an ultrafast hydrogen detection system, which demonstrates significant application promise in the fields of low-power sensors and rapid gas detection.</p>","PeriodicalId":24,"journal":{"name":"ACS Sensors","volume":"10 3","pages":"2181–2190 2181–2190"},"PeriodicalIF":9.1000,"publicationDate":"2025-03-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Ultrafast Hydrogen Detection System Using Vertical Thermal Conduction Structure and Neural Network Prediction Algorithm Based on Sensor Response Process\",\"authors\":\"Ruilin Yang, Zhen Yuan*, Changrong Jiang, Xinjie Zhang, Zilong Qiao, Jianping Zhang, Junge Liang, Si Wang, Zaihua Duan, Yuanming Wu, Weizhi Li*, Yadong Jiang and Huiling Tai*, \",\"doi\":\"10.1021/acssensors.4c0348710.1021/acssensors.4c03487\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Hydrogen detection plays a crucial role in various scenes of hydrogen energy such as hydrogen vehicles, hydrogen transportation and hydrogen storage. It is essential to develop a hydrogen detection system with ultrafast response times (<1 s) for the timely detection of hydrogen leaks. Here we report an ultrafast (0.4 s) hydrogen detection system based on a wafer-scale fabrication process. It consists of a low power (20.2 mW) hydrogen sensor based on vertical thermal conduction structure and a signal processing circuit introduced with a neural network prediction algorithm based on sensor response process. The fabricated sensor exhibits rapid response, wide detection range, and wide operating temperature, while showing good long-term stability and excellent selectivity. Meanwhile, the model significantly enhanced the detection speed by enabling hydrogen concentration prediction using only the initial 40 data points (sampling frequency of 100 Hz) from the sensor response before the sensor completes the entire response process. This work introduces a novel approach to achieve an ultrafast hydrogen detection system, which demonstrates significant application promise in the fields of low-power sensors and rapid gas detection.</p>\",\"PeriodicalId\":24,\"journal\":{\"name\":\"ACS Sensors\",\"volume\":\"10 3\",\"pages\":\"2181–2190 2181–2190\"},\"PeriodicalIF\":9.1000,\"publicationDate\":\"2025-03-11\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Sensors\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acssensors.4c03487\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, ANALYTICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Sensors","FirstCategoryId":"92","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acssensors.4c03487","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, ANALYTICAL","Score":null,"Total":0}
Ultrafast Hydrogen Detection System Using Vertical Thermal Conduction Structure and Neural Network Prediction Algorithm Based on Sensor Response Process
Hydrogen detection plays a crucial role in various scenes of hydrogen energy such as hydrogen vehicles, hydrogen transportation and hydrogen storage. It is essential to develop a hydrogen detection system with ultrafast response times (<1 s) for the timely detection of hydrogen leaks. Here we report an ultrafast (0.4 s) hydrogen detection system based on a wafer-scale fabrication process. It consists of a low power (20.2 mW) hydrogen sensor based on vertical thermal conduction structure and a signal processing circuit introduced with a neural network prediction algorithm based on sensor response process. The fabricated sensor exhibits rapid response, wide detection range, and wide operating temperature, while showing good long-term stability and excellent selectivity. Meanwhile, the model significantly enhanced the detection speed by enabling hydrogen concentration prediction using only the initial 40 data points (sampling frequency of 100 Hz) from the sensor response before the sensor completes the entire response process. This work introduces a novel approach to achieve an ultrafast hydrogen detection system, which demonstrates significant application promise in the fields of low-power sensors and rapid gas detection.
期刊介绍:
ACS Sensors is a peer-reviewed research journal that focuses on the dissemination of new and original knowledge in the field of sensor science, particularly those that selectively sense chemical or biological species or processes. The journal covers a broad range of topics, including but not limited to biosensors, chemical sensors, gas sensors, intracellular sensors, single molecule sensors, cell chips, and microfluidic devices. It aims to publish articles that address conceptual advances in sensing technology applicable to various types of analytes or application papers that report on the use of existing sensing concepts in new ways or for new analytes.