Shuo Dai, Si-Yuan Liao, Jun-Rui Pan and Hai-Feng Zhang
{"title":"基于二氧化钒的超宽带吸收及倍频线圆极化转换可调谐元结构的理论研究","authors":"Shuo Dai, Si-Yuan Liao, Jun-Rui Pan and Hai-Feng Zhang","doi":"10.1039/D5NR00490J","DOIUrl":null,"url":null,"abstract":"<p >An ultra-wideband absorption and tripling octave frequency linear-to-circular polarization conversion tunable metastructure (MS) is proposed, utilizing the phase transition property of vanadium dioxide (VO<small><sub>2</sub></small>). In its metallic state, the MS is demonstrated to function as a polarization-insensitive ultra-wideband MS absorber, achieving an absorption value exceeding 90% within a frequency range of 2.37 THz to 4.56 THz. The absorption mechanism is elucidated through an equivalent circuit model, impedance matching theory, and electric field distribution analysis. In the insulating state of VO<small><sub>2</sub></small>, the MS is shown to operate as a converter tripling the octave frequency in linear-to-circular polarization, with an axial ratio below 3 dB across the frequency ranges of 0.95–1.68 THz and 2.25–4.49 THz, corresponding to relative bandwidths of 55.51% and 66.27%. Remarkably, the polarization conversion in the insulating state exhibits tripling octave frequency characteristics, with a fundamental bandwidth spanning 0.95–1.49 THz and a tripling octave frequency bandwidth spanning 2.85–4.48 THz. The MS can switch between distinct functionalities within the terahertz regime, offering significant potential for applications such as spectral analysis, signal encryption, stealth material preparation, and other advanced terahertz technologies.</p>","PeriodicalId":92,"journal":{"name":"Nanoscale","volume":" 20","pages":" 12673-12683"},"PeriodicalIF":5.1000,"publicationDate":"2025-03-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Theoretical investigation of a tunable vanadium dioxide-based metastructure for ultra-wideband absorption and linear-to-circular polarization conversion across triple-octave frequencies†\",\"authors\":\"Shuo Dai, Si-Yuan Liao, Jun-Rui Pan and Hai-Feng Zhang\",\"doi\":\"10.1039/D5NR00490J\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >An ultra-wideband absorption and tripling octave frequency linear-to-circular polarization conversion tunable metastructure (MS) is proposed, utilizing the phase transition property of vanadium dioxide (VO<small><sub>2</sub></small>). In its metallic state, the MS is demonstrated to function as a polarization-insensitive ultra-wideband MS absorber, achieving an absorption value exceeding 90% within a frequency range of 2.37 THz to 4.56 THz. The absorption mechanism is elucidated through an equivalent circuit model, impedance matching theory, and electric field distribution analysis. In the insulating state of VO<small><sub>2</sub></small>, the MS is shown to operate as a converter tripling the octave frequency in linear-to-circular polarization, with an axial ratio below 3 dB across the frequency ranges of 0.95–1.68 THz and 2.25–4.49 THz, corresponding to relative bandwidths of 55.51% and 66.27%. Remarkably, the polarization conversion in the insulating state exhibits tripling octave frequency characteristics, with a fundamental bandwidth spanning 0.95–1.49 THz and a tripling octave frequency bandwidth spanning 2.85–4.48 THz. The MS can switch between distinct functionalities within the terahertz regime, offering significant potential for applications such as spectral analysis, signal encryption, stealth material preparation, and other advanced terahertz technologies.</p>\",\"PeriodicalId\":92,\"journal\":{\"name\":\"Nanoscale\",\"volume\":\" 20\",\"pages\":\" 12673-12683\"},\"PeriodicalIF\":5.1000,\"publicationDate\":\"2025-03-26\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nanoscale\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://pubs.rsc.org/en/content/articlelanding/2025/nr/d5nr00490j\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nanoscale","FirstCategoryId":"88","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2025/nr/d5nr00490j","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Theoretical investigation of a tunable vanadium dioxide-based metastructure for ultra-wideband absorption and linear-to-circular polarization conversion across triple-octave frequencies†
An ultra-wideband absorption and tripling octave frequency linear-to-circular polarization conversion tunable metastructure (MS) is proposed, utilizing the phase transition property of vanadium dioxide (VO2). In its metallic state, the MS is demonstrated to function as a polarization-insensitive ultra-wideband MS absorber, achieving an absorption value exceeding 90% within a frequency range of 2.37 THz to 4.56 THz. The absorption mechanism is elucidated through an equivalent circuit model, impedance matching theory, and electric field distribution analysis. In the insulating state of VO2, the MS is shown to operate as a converter tripling the octave frequency in linear-to-circular polarization, with an axial ratio below 3 dB across the frequency ranges of 0.95–1.68 THz and 2.25–4.49 THz, corresponding to relative bandwidths of 55.51% and 66.27%. Remarkably, the polarization conversion in the insulating state exhibits tripling octave frequency characteristics, with a fundamental bandwidth spanning 0.95–1.49 THz and a tripling octave frequency bandwidth spanning 2.85–4.48 THz. The MS can switch between distinct functionalities within the terahertz regime, offering significant potential for applications such as spectral analysis, signal encryption, stealth material preparation, and other advanced terahertz technologies.
期刊介绍:
Nanoscale is a high-impact international journal, publishing high-quality research across nanoscience and nanotechnology. Nanoscale publishes a full mix of research articles on experimental and theoretical work, including reviews, communications, and full papers.Highly interdisciplinary, this journal appeals to scientists, researchers and professionals interested in nanoscience and nanotechnology, quantum materials and quantum technology, including the areas of physics, chemistry, biology, medicine, materials, energy/environment, information technology, detection science, healthcare and drug discovery, and electronics.