克服干旱地区的能源-水关系-绿色氢载体和基础化学品的水积极生产:DryHy项目-技术方面†

IF 5 3区 材料科学 Q2 CHEMISTRY, PHYSICAL
Victor Selmert, Leandros Paschalidis, Nicolas Kruse, Steffen Dirkes, Ansgar Kretzschmar, Gbenga Jerome, Carl Jung, Lu Xu, Nils Beltermann, Hermann Tempel, Roland Peters, Remzi Can Samsun and Rüdiger-A. Eichel
{"title":"克服干旱地区的能源-水关系-绿色氢载体和基础化学品的水积极生产:DryHy项目-技术方面†","authors":"Victor Selmert, Leandros Paschalidis, Nicolas Kruse, Steffen Dirkes, Ansgar Kretzschmar, Gbenga Jerome, Carl Jung, Lu Xu, Nils Beltermann, Hermann Tempel, Roland Peters, Remzi Can Samsun and Rüdiger-A. Eichel","doi":"10.1039/D4SE01783H","DOIUrl":null,"url":null,"abstract":"<p >The application of Direct Air Capture (DAC) for extracting CO<small><sub>2</sub></small> from the atmosphere has a great potential to reduce net CO<small><sub>2</sub></small> emissions and help achieve climate goals. Besides storing the separated CO<small><sub>2</sub></small>, it can be used as a carbon feedstock for producing CO<small><sub>2</sub></small>-neutral e-fuels, marking a critical research focus area. Despite advancements in various DAC technologies and processes, their large-scale implementation remains limited, among other reasons, because of the large amounts of energy required to power such processes. This article explores the utilization of DAC for water-conscious production of methanol in sunny regions, using cost-efficient photovoltaic power. The selected approach is presented, which involves a process on demonstrator scale with amine-based DAC for CO<small><sub>2</sub></small> and water separation from air, high-temperature electrolysis using solid oxide electrolysis cells (SOEC) for syngas production, and subsequent methanol synthesis. We also discuss alternative methods, potential locations, and implementation strategies, highlighting the advantages but also the challenges of producing green methanol in sunny regions outside Germany.</p>","PeriodicalId":104,"journal":{"name":"Sustainable Energy & Fuels","volume":" 7","pages":" 1672-1682"},"PeriodicalIF":5.0000,"publicationDate":"2025-02-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.rsc.org/en/content/articlepdf/2025/se/d4se01783h?page=search","citationCount":"0","resultStr":"{\"title\":\"Overcoming the energy–water nexus in dry regions – water-positive production of green hydrogen carriers and base chemicals: the DryHy project – technical aspects†\",\"authors\":\"Victor Selmert, Leandros Paschalidis, Nicolas Kruse, Steffen Dirkes, Ansgar Kretzschmar, Gbenga Jerome, Carl Jung, Lu Xu, Nils Beltermann, Hermann Tempel, Roland Peters, Remzi Can Samsun and Rüdiger-A. Eichel\",\"doi\":\"10.1039/D4SE01783H\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >The application of Direct Air Capture (DAC) for extracting CO<small><sub>2</sub></small> from the atmosphere has a great potential to reduce net CO<small><sub>2</sub></small> emissions and help achieve climate goals. Besides storing the separated CO<small><sub>2</sub></small>, it can be used as a carbon feedstock for producing CO<small><sub>2</sub></small>-neutral e-fuels, marking a critical research focus area. Despite advancements in various DAC technologies and processes, their large-scale implementation remains limited, among other reasons, because of the large amounts of energy required to power such processes. This article explores the utilization of DAC for water-conscious production of methanol in sunny regions, using cost-efficient photovoltaic power. The selected approach is presented, which involves a process on demonstrator scale with amine-based DAC for CO<small><sub>2</sub></small> and water separation from air, high-temperature electrolysis using solid oxide electrolysis cells (SOEC) for syngas production, and subsequent methanol synthesis. We also discuss alternative methods, potential locations, and implementation strategies, highlighting the advantages but also the challenges of producing green methanol in sunny regions outside Germany.</p>\",\"PeriodicalId\":104,\"journal\":{\"name\":\"Sustainable Energy & Fuels\",\"volume\":\" 7\",\"pages\":\" 1672-1682\"},\"PeriodicalIF\":5.0000,\"publicationDate\":\"2025-02-25\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://pubs.rsc.org/en/content/articlepdf/2025/se/d4se01783h?page=search\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Sustainable Energy & Fuels\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://pubs.rsc.org/en/content/articlelanding/2025/se/d4se01783h\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Sustainable Energy & Fuels","FirstCategoryId":"88","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2025/se/d4se01783h","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0

摘要

直接空气捕集(DAC)技术用于从大气中提取二氧化碳,在减少二氧化碳净排放和帮助实现气候目标方面具有巨大的潜力。除了储存分离的二氧化碳外,它还可以用作生产二氧化碳中性电子燃料的碳原料,这标志着一个关键的研究重点领域。尽管各种DAC技术和工艺取得了进步,但它们的大规模实施仍然有限,其中一个原因是需要大量的能源来为这些工艺提供动力。本文探讨了在阳光充足的地区,利用成本效益高的光伏发电,将DAC用于节水生产甲醇。所选择的方法包括一个示范规模的过程,以胺基DAC从空气中分离二氧化碳和水,使用固体氧化物电解电池(SOEC)进行高温电解以生产合成气,以及随后的甲醇合成。我们还讨论了替代方法、潜在地点和实施策略,强调了在德国以外阳光充足的地区生产绿色甲醇的优势和挑战。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Overcoming the energy–water nexus in dry regions – water-positive production of green hydrogen carriers and base chemicals: the DryHy project – technical aspects†

Overcoming the energy–water nexus in dry regions – water-positive production of green hydrogen carriers and base chemicals: the DryHy project – technical aspects†

The application of Direct Air Capture (DAC) for extracting CO2 from the atmosphere has a great potential to reduce net CO2 emissions and help achieve climate goals. Besides storing the separated CO2, it can be used as a carbon feedstock for producing CO2-neutral e-fuels, marking a critical research focus area. Despite advancements in various DAC technologies and processes, their large-scale implementation remains limited, among other reasons, because of the large amounts of energy required to power such processes. This article explores the utilization of DAC for water-conscious production of methanol in sunny regions, using cost-efficient photovoltaic power. The selected approach is presented, which involves a process on demonstrator scale with amine-based DAC for CO2 and water separation from air, high-temperature electrolysis using solid oxide electrolysis cells (SOEC) for syngas production, and subsequent methanol synthesis. We also discuss alternative methods, potential locations, and implementation strategies, highlighting the advantages but also the challenges of producing green methanol in sunny regions outside Germany.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Sustainable Energy & Fuels
Sustainable Energy & Fuels Energy-Energy Engineering and Power Technology
CiteScore
10.00
自引率
3.60%
发文量
394
期刊介绍: Sustainable Energy & Fuels will publish research that contributes to the development of sustainable energy technologies with a particular emphasis on new and next-generation technologies.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信