M.A. Goodwin , A. Petts , J.L. McLarty , D.L. Chester , T.C. Stokes , B. Milbrath
{"title":"Gamma spectroscopy measurements of fresh charcoal samples from the Hartlepool advanced gas-cooled reactor","authors":"M.A. Goodwin , A. Petts , J.L. McLarty , D.L. Chester , T.C. Stokes , B. Milbrath","doi":"10.1016/j.apradiso.2025.111764","DOIUrl":null,"url":null,"abstract":"<div><div>Radionuclides are emitted from nuclear power reactors to the atmosphere and are often measured on the International Monitoring System (IMS) – the primary tool of the Comprehensive Nuclear-Test-Ban Treaty (CTBT) for monitoring for signs of nuclear explosions around the world. During refuel of an advanced gas-cooled reactor (AGR) the coolant gas is processed and filtered before being exhausted to the atmosphere. Charcoal and filter paper samples from the processing plant have been measured using high purity germanium γ-ray detectors to identify which radionuclides are present and the activities calculated. Isotopes of radioxenon generated primarily by fission (<sup>133</sup>Xe, <sup>135</sup>Xe, <sup>131m</sup>Xe, <sup>133m</sup>Xe) and by activation (<sup>125</sup>Xe, <sup>127</sup>Xe, <sup>129m</sup>Xe) were identified, as well as <sup>137</sup>Cs, <sup>60</sup>Co and <sup>75</sup>Se. In addition, radionuclide identification confirmation and activity quantification was made using γ-γ coincidence measurement, which provides a more sensitive measurement for low-activity radionuclides.</div></div>","PeriodicalId":8096,"journal":{"name":"Applied Radiation and Isotopes","volume":"220 ","pages":"Article 111764"},"PeriodicalIF":1.6000,"publicationDate":"2025-03-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Applied Radiation and Isotopes","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0969804325001095","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, INORGANIC & NUCLEAR","Score":null,"Total":0}
Gamma spectroscopy measurements of fresh charcoal samples from the Hartlepool advanced gas-cooled reactor
Radionuclides are emitted from nuclear power reactors to the atmosphere and are often measured on the International Monitoring System (IMS) – the primary tool of the Comprehensive Nuclear-Test-Ban Treaty (CTBT) for monitoring for signs of nuclear explosions around the world. During refuel of an advanced gas-cooled reactor (AGR) the coolant gas is processed and filtered before being exhausted to the atmosphere. Charcoal and filter paper samples from the processing plant have been measured using high purity germanium γ-ray detectors to identify which radionuclides are present and the activities calculated. Isotopes of radioxenon generated primarily by fission (133Xe, 135Xe, 131mXe, 133mXe) and by activation (125Xe, 127Xe, 129mXe) were identified, as well as 137Cs, 60Co and 75Se. In addition, radionuclide identification confirmation and activity quantification was made using γ-γ coincidence measurement, which provides a more sensitive measurement for low-activity radionuclides.
期刊介绍:
Applied Radiation and Isotopes provides a high quality medium for the publication of substantial, original and scientific and technological papers on the development and peaceful application of nuclear, radiation and radionuclide techniques in chemistry, physics, biochemistry, biology, medicine, security, engineering and in the earth, planetary and environmental sciences, all including dosimetry. Nuclear techniques are defined in the broadest sense and both experimental and theoretical papers are welcome. They include the development and use of α- and β-particles, X-rays and γ-rays, neutrons and other nuclear particles and radiations from all sources, including radionuclides, synchrotron sources, cyclotrons and reactors and from the natural environment.
The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria.
Papers dealing with radiation processing, i.e., where radiation is used to bring about a biological, chemical or physical change in a material, should be directed to our sister journal Radiation Physics and Chemistry.