太赫兹光电流探针的量子几何和相互作用的魔角扭曲双层石墨烯

IF 37.2 1区 材料科学 Q1 CHEMISTRY, PHYSICAL
Roshan Krishna Kumar, Geng Li, Riccardo Bertini, Swati Chaudhary, Krystian Nowakowski, Jeong Min Park, Sebastian Castilla, Zhen Zhan, Pierre A. Pantaleón, Hitesh Agarwal, Sergi Batlle-Porro, Eike Icking, Matteo Ceccanti, Antoine Reserbat-Plantey, Giulia Piccinini, Julien Barrier, Ekaterina Khestanova, Takashi Taniguchi, Kenji Watanabe, Christoph Stampfer, Gil Refael, Francisco Guinea, Pablo Jarillo-Herrero, Justin C. W. Song, Petr Stepanov, Cyprian Lewandowski, Frank H. L. Koppens
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引用次数: 0

摘要

波纹材料代表了强相互作用的电子系统,桥接拓扑和相关物理。尽管取得了显著的进展,但解码量子几何背后的波函数特性仍然具有挑战性。在这里,我们利用偏振分辨光电流测量来探测魔角扭曲双层石墨烯,利用其对包含电子波函数量子“纹理”的Berry连接的灵敏度。利用具有平带光学跃迁的太赫兹光共振,我们观察到由破缺对称性驱动的体光电流,并揭示了电子相互作用与量子几何之间的相互作用。我们观察到通过量子输运无法检测到的反转破缺间隙态,由相互作用诱导的带重整化引起的极化轴的急剧变化,以及在通过相变级联跟踪量子几何演化的moir单元胞的整数填充因子处反复出现的光电流模式。平带系统固有的大而可调谐的太赫兹响应提供了对相互作用电子的量子几何的直接见解,并为创新的太赫兹量子技术铺平了道路。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Terahertz photocurrent probe of quantum geometry and interactions in magic-angle twisted bilayer graphene

Terahertz photocurrent probe of quantum geometry and interactions in magic-angle twisted bilayer graphene

Moiré materials represent strongly interacting electron systems bridging topological and correlated physics. Despite notable advances, decoding wavefunction properties underlying the quantum geometry remains challenging. Here we utilize polarization-resolved photocurrent measurements to probe magic-angle twisted bilayer graphene, leveraging its sensitivity to the Berry connection that encompasses quantum ‘textures’ of electron wavefunctions. Using terahertz light resonant with optical transitions of its flat bands, we observe bulk photocurrents driven by broken symmetries and reveal the interplay between electron interactions and quantum geometry. We observe inversion-breaking gapped states undetectable through quantum transport, sharp changes in the polarization axes caused by interaction-induced band renormalization and recurring photocurrent patterns at integer filling factors of the moiré unit cell that track the evolution of quantum geometry through the cascade of phase transitions. The large and tunable terahertz response intrinsic to flat-band systems offers direct insights into the quantum geometry of interacting electrons and paves the way for innovative terahertz quantum technologies.

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来源期刊
Nature Materials
Nature Materials 工程技术-材料科学:综合
CiteScore
62.20
自引率
0.70%
发文量
221
审稿时长
3.2 months
期刊介绍: Nature Materials is a monthly multi-disciplinary journal aimed at bringing together cutting-edge research across the entire spectrum of materials science and engineering. It covers all applied and fundamental aspects of the synthesis/processing, structure/composition, properties, and performance of materials. The journal recognizes that materials research has an increasing impact on classical disciplines such as physics, chemistry, and biology. Additionally, Nature Materials provides a forum for the development of a common identity among materials scientists and encourages interdisciplinary collaboration. It takes an integrated and balanced approach to all areas of materials research, fostering the exchange of ideas between scientists involved in different disciplines. Nature Materials is an invaluable resource for scientists in academia and industry who are active in discovering and developing materials and materials-related concepts. It offers engaging and informative papers of exceptional significance and quality, with the aim of influencing the development of society in the future.
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