Roshan Krishna Kumar, Geng Li, Riccardo Bertini, Swati Chaudhary, Krystian Nowakowski, Jeong Min Park, Sebastian Castilla, Zhen Zhan, Pierre A. Pantaleón, Hitesh Agarwal, Sergi Batlle-Porro, Eike Icking, Matteo Ceccanti, Antoine Reserbat-Plantey, Giulia Piccinini, Julien Barrier, Ekaterina Khestanova, Takashi Taniguchi, Kenji Watanabe, Christoph Stampfer, Gil Refael, Francisco Guinea, Pablo Jarillo-Herrero, Justin C. W. Song, Petr Stepanov, Cyprian Lewandowski, Frank H. L. Koppens
{"title":"太赫兹光电流探针的量子几何和相互作用的魔角扭曲双层石墨烯","authors":"Roshan Krishna Kumar, Geng Li, Riccardo Bertini, Swati Chaudhary, Krystian Nowakowski, Jeong Min Park, Sebastian Castilla, Zhen Zhan, Pierre A. Pantaleón, Hitesh Agarwal, Sergi Batlle-Porro, Eike Icking, Matteo Ceccanti, Antoine Reserbat-Plantey, Giulia Piccinini, Julien Barrier, Ekaterina Khestanova, Takashi Taniguchi, Kenji Watanabe, Christoph Stampfer, Gil Refael, Francisco Guinea, Pablo Jarillo-Herrero, Justin C. W. Song, Petr Stepanov, Cyprian Lewandowski, Frank H. L. Koppens","doi":"10.1038/s41563-025-02180-3","DOIUrl":null,"url":null,"abstract":"<p>Moiré materials represent strongly interacting electron systems bridging topological and correlated physics. Despite notable advances, decoding wavefunction properties underlying the quantum geometry remains challenging. Here we utilize polarization-resolved photocurrent measurements to probe magic-angle twisted bilayer graphene, leveraging its sensitivity to the Berry connection that encompasses quantum ‘textures’ of electron wavefunctions. Using terahertz light resonant with optical transitions of its flat bands, we observe bulk photocurrents driven by broken symmetries and reveal the interplay between electron interactions and quantum geometry. We observe inversion-breaking gapped states undetectable through quantum transport, sharp changes in the polarization axes caused by interaction-induced band renormalization and recurring photocurrent patterns at integer filling factors of the moiré unit cell that track the evolution of quantum geometry through the cascade of phase transitions. The large and tunable terahertz response intrinsic to flat-band systems offers direct insights into the quantum geometry of interacting electrons and paves the way for innovative terahertz quantum technologies.</p>","PeriodicalId":19058,"journal":{"name":"Nature Materials","volume":"58 1","pages":""},"PeriodicalIF":37.2000,"publicationDate":"2025-03-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Terahertz photocurrent probe of quantum geometry and interactions in magic-angle twisted bilayer graphene\",\"authors\":\"Roshan Krishna Kumar, Geng Li, Riccardo Bertini, Swati Chaudhary, Krystian Nowakowski, Jeong Min Park, Sebastian Castilla, Zhen Zhan, Pierre A. 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Using terahertz light resonant with optical transitions of its flat bands, we observe bulk photocurrents driven by broken symmetries and reveal the interplay between electron interactions and quantum geometry. We observe inversion-breaking gapped states undetectable through quantum transport, sharp changes in the polarization axes caused by interaction-induced band renormalization and recurring photocurrent patterns at integer filling factors of the moiré unit cell that track the evolution of quantum geometry through the cascade of phase transitions. 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Terahertz photocurrent probe of quantum geometry and interactions in magic-angle twisted bilayer graphene
Moiré materials represent strongly interacting electron systems bridging topological and correlated physics. Despite notable advances, decoding wavefunction properties underlying the quantum geometry remains challenging. Here we utilize polarization-resolved photocurrent measurements to probe magic-angle twisted bilayer graphene, leveraging its sensitivity to the Berry connection that encompasses quantum ‘textures’ of electron wavefunctions. Using terahertz light resonant with optical transitions of its flat bands, we observe bulk photocurrents driven by broken symmetries and reveal the interplay between electron interactions and quantum geometry. We observe inversion-breaking gapped states undetectable through quantum transport, sharp changes in the polarization axes caused by interaction-induced band renormalization and recurring photocurrent patterns at integer filling factors of the moiré unit cell that track the evolution of quantum geometry through the cascade of phase transitions. The large and tunable terahertz response intrinsic to flat-band systems offers direct insights into the quantum geometry of interacting electrons and paves the way for innovative terahertz quantum technologies.
期刊介绍:
Nature Materials is a monthly multi-disciplinary journal aimed at bringing together cutting-edge research across the entire spectrum of materials science and engineering. It covers all applied and fundamental aspects of the synthesis/processing, structure/composition, properties, and performance of materials. The journal recognizes that materials research has an increasing impact on classical disciplines such as physics, chemistry, and biology.
Additionally, Nature Materials provides a forum for the development of a common identity among materials scientists and encourages interdisciplinary collaboration. It takes an integrated and balanced approach to all areas of materials research, fostering the exchange of ideas between scientists involved in different disciplines.
Nature Materials is an invaluable resource for scientists in academia and industry who are active in discovering and developing materials and materials-related concepts. It offers engaging and informative papers of exceptional significance and quality, with the aim of influencing the development of society in the future.