宽带极紫外涡旋光束的产生动力学

IF 6.7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Antonios Pelekanidis, Fengling Zhang, Kjeld S. E. Eikema and Stefan Witte*, 
{"title":"宽带极紫外涡旋光束的产生动力学","authors":"Antonios Pelekanidis,&nbsp;Fengling Zhang,&nbsp;Kjeld S. E. Eikema and Stefan Witte*,&nbsp;","doi":"10.1021/acsphotonics.4c0251610.1021/acsphotonics.4c02516","DOIUrl":null,"url":null,"abstract":"<p >Light beams carrying orbital angular momentum (OAM) can be generated in the extreme ultraviolet and soft X-ray spectra by means of high harmonic generation (HHG). In HHG, phase properties of the drive laser, such as curvature, aberrations, and topological charge, are upconverted to the harmonic beams and coherently added to the inherent dipole phase. The strong nonlinearity of the HHG process, combined with the rapid phase variations corresponding to large OAM values in these vortex beams, leads to a high sensitivity to small variations in the driving field. However, a study of the generation dynamics via an accurate reconstruction of multiwavelength OAM beams is challenging. Here we show full complex field measurements of multiple individual harmonics of the HHG vortex beams. By using spectrally resolved ptychographic wavefront sensing, we retrieve the high-resolution amplitude and phase profiles for harmonics 23 to 29 in parallel, enabling detailed multiwavelength beam reconstructions. We study the influence of generation conditions and drive laser aberrations on the resulting vortex fields by comparing measured fields to numerical simulations and retrieving the propagation conditions around the focus and the OAM content of the beams. Specifically, we find that the multimodal content of such vortex beams can significantly influence the propagation and field distributions in the focal region. Such a beam propagation analysis allows a prediction of the resulting attosecond pulse trains and associated attosecond light springs that can be generated under realistic driving conditions.</p>","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"12 3","pages":"1638–1649 1638–1649"},"PeriodicalIF":6.7000,"publicationDate":"2025-02-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acsphotonics.4c02516","citationCount":"0","resultStr":"{\"title\":\"Generation Dynamics of Broadband Extreme Ultraviolet Vortex Beams\",\"authors\":\"Antonios Pelekanidis,&nbsp;Fengling Zhang,&nbsp;Kjeld S. E. Eikema and Stefan Witte*,&nbsp;\",\"doi\":\"10.1021/acsphotonics.4c0251610.1021/acsphotonics.4c02516\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Light beams carrying orbital angular momentum (OAM) can be generated in the extreme ultraviolet and soft X-ray spectra by means of high harmonic generation (HHG). In HHG, phase properties of the drive laser, such as curvature, aberrations, and topological charge, are upconverted to the harmonic beams and coherently added to the inherent dipole phase. The strong nonlinearity of the HHG process, combined with the rapid phase variations corresponding to large OAM values in these vortex beams, leads to a high sensitivity to small variations in the driving field. However, a study of the generation dynamics via an accurate reconstruction of multiwavelength OAM beams is challenging. Here we show full complex field measurements of multiple individual harmonics of the HHG vortex beams. By using spectrally resolved ptychographic wavefront sensing, we retrieve the high-resolution amplitude and phase profiles for harmonics 23 to 29 in parallel, enabling detailed multiwavelength beam reconstructions. We study the influence of generation conditions and drive laser aberrations on the resulting vortex fields by comparing measured fields to numerical simulations and retrieving the propagation conditions around the focus and the OAM content of the beams. Specifically, we find that the multimodal content of such vortex beams can significantly influence the propagation and field distributions in the focal region. Such a beam propagation analysis allows a prediction of the resulting attosecond pulse trains and associated attosecond light springs that can be generated under realistic driving conditions.</p>\",\"PeriodicalId\":23,\"journal\":{\"name\":\"ACS Photonics\",\"volume\":\"12 3\",\"pages\":\"1638–1649 1638–1649\"},\"PeriodicalIF\":6.7000,\"publicationDate\":\"2025-02-28\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://pubs.acs.org/doi/epdf/10.1021/acsphotonics.4c02516\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Photonics\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acsphotonics.4c02516\",\"RegionNum\":1,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Photonics","FirstCategoryId":"101","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsphotonics.4c02516","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

在极紫外和软x射线光谱中,利用高谐波产生(HHG)可以产生携带轨道角动量(OAM)的光束。在HHG中,驱动激光的相位特性,如曲率、像差和拓扑电荷,被上转换为谐波光束,并相干地添加到固有偶极子相位中。HHG过程的强非线性,加上涡旋光束中较大OAM值对应的快速相位变化,导致对驱动场的微小变化具有很高的灵敏度。然而,通过精确重建多波长OAM光束的产生动力学研究是具有挑战性的。在这里,我们展示了HHG涡旋光束的多个单独谐波的完整复杂场测量。通过使用光谱分辨型波前传感技术,我们获得了23至29次谐波的高分辨率振幅和相位曲线,从而实现了详细的多波长波束重建。通过将实测场与数值模拟结果进行比较,并获取焦点周围的传播条件和光束的OAM含量,研究了产生条件和驱动激光像差对涡旋场的影响。具体而言,我们发现涡旋光束的多模态含量会显著影响其在焦点区域的传播和场分布。这样的光束传播分析可以预测在现实驾驶条件下产生的阿秒脉冲序列和相关的阿秒光弹簧。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Generation Dynamics of Broadband Extreme Ultraviolet Vortex Beams

Light beams carrying orbital angular momentum (OAM) can be generated in the extreme ultraviolet and soft X-ray spectra by means of high harmonic generation (HHG). In HHG, phase properties of the drive laser, such as curvature, aberrations, and topological charge, are upconverted to the harmonic beams and coherently added to the inherent dipole phase. The strong nonlinearity of the HHG process, combined with the rapid phase variations corresponding to large OAM values in these vortex beams, leads to a high sensitivity to small variations in the driving field. However, a study of the generation dynamics via an accurate reconstruction of multiwavelength OAM beams is challenging. Here we show full complex field measurements of multiple individual harmonics of the HHG vortex beams. By using spectrally resolved ptychographic wavefront sensing, we retrieve the high-resolution amplitude and phase profiles for harmonics 23 to 29 in parallel, enabling detailed multiwavelength beam reconstructions. We study the influence of generation conditions and drive laser aberrations on the resulting vortex fields by comparing measured fields to numerical simulations and retrieving the propagation conditions around the focus and the OAM content of the beams. Specifically, we find that the multimodal content of such vortex beams can significantly influence the propagation and field distributions in the focal region. Such a beam propagation analysis allows a prediction of the resulting attosecond pulse trains and associated attosecond light springs that can be generated under realistic driving conditions.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
ACS Photonics
ACS Photonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
11.90
自引率
5.70%
发文量
438
审稿时长
2.3 months
期刊介绍: Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信