基于神经网络的清洁能源煤层气稳定同位素地球化学预测应用

IF 10 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL
Mohammad Asif , Keka Ojha , D.C. Panigrahi , Fidelis Suorineni
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引用次数: 0

摘要

对煤层气含量、气体组成及稳定同位素地球化学特征进行了研究,探讨了煤层气的生成机理。煤层气样品干气含量在2 ~ 10 m3/t之间。煤层气由甲烷(~ 52% ~ ~ 99%)、高碳氢化合物(0% ~ ~ 12%)和微量CO2组成。该手稿旨在使用机器学习方法识别煤层气样品的稳定同位素,然后对Jharia煤田的天然气来源进行批判性审查。为此构建了人工神经网络(ANN),其中6个参数作为输入,3个参数作为模型的输出。利用该模型预测了Jharia煤田煤层气样品的稳定同位素范围:-59.86‰≤≤-19.31‰,-19.93‰≤≤-7.95‰,-275.74‰≤≤-138.64‰。广泛的同位素数据反映了煤层气复杂的生成机制;煤层气中既有热成因甲烷,也有生物成因甲烷。通过测定二氧化碳和甲烷指数(CDMI)、碳氢化合物指数(HI)和气体干燥指数(DI)来描述伯纳德图和CD图(碳-氢图或怀特卡尔图),推断Jharia煤田煤层气的成因。同时进行了煤层气稳定同位素分析实验,提供了强相关性(R2>0.99),增强了基于神经网络的稳定同位素预测。Van Krevelen图解认为煤样落在III型气源窗口。该研究为清洁能源煤层气的生成机理提供了基础性的认识。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Application of ANN-based prediction insights into the stable isotope geochemistry of the clean energy coalbed gas
The coalbed gas content, gas composition and stable isotope geochemistry of coalbed gas were investigated to study the generation mechanism of coalbed gas. The dry gas content of coalbed gas samples ranges from 2 to 10 m3/t. The composition of coalbed gas reveals that it consists of methane (∼52 %–∼99 %) with higher hydrocarbon (0 %–∼12 %) and traces of CO2. The manuscript is designed to recognise the stable isotopes of coalbed gas samples using machine learning approaches and then provide a critical review of the gas origin from Jharia Coalfield. The artificial neural network (ANN) was constructed for this purpose, consisting of six parameters as the input and three as the model's output. The stable isotopes of coalbed gas samples from Jharia Coalfield were predicted by the model with the following ranges: −59.86‰≤ δC13CH4 ≤-19.31‰, −19.93‰≤ δ13CCO2 ≤-7.95‰, while −275.74‰≤ δDCH4 ≤-138.64‰. The wide range of isotope data imitates the complicated generation mechanism of coalbed gas; both thermogenic and biogenic methane are present in the coalbed gas. The carbon dioxide and methane index (CDMI), hydrocarbon index (HI), and gas dryness index (DI) were determined for the description of the Bernard and CD diagram (carbon-hydrogen diagram or Whiticar-style plot) to infer the origin of coalbed gas from the Jharia Coalfield. The experiment of the stable isotope analysis of the coalbed gas was also performed, which augmented the ANN-based prediction of stable isotopes by providing a strong correlation (R2>0.99). Van Krevelen's diagram concludes that the coal samples fall in the window of type III gas origin. This research provides fundamental insights into the generation mechanism of clean energy coalbed gas.
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来源期刊
Journal of Cleaner Production
Journal of Cleaner Production 环境科学-工程:环境
CiteScore
20.40
自引率
9.00%
发文量
4720
审稿时长
111 days
期刊介绍: The Journal of Cleaner Production is an international, transdisciplinary journal that addresses and discusses theoretical and practical Cleaner Production, Environmental, and Sustainability issues. It aims to help societies become more sustainable by focusing on the concept of 'Cleaner Production', which aims at preventing waste production and increasing efficiencies in energy, water, resources, and human capital use. The journal serves as a platform for corporations, governments, education institutions, regions, and societies to engage in discussions and research related to Cleaner Production, environmental, and sustainability practices.
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