IF 5 Q2 ENERGY & FUELS
Peter Lang , Nils E. Schneider , Franz J.T. Huber , Stefan Will
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引用次数: 0

摘要

喷焰合成(SFS)是生产金属氧化物纳米粒子的一种前景广阔的技术。然而,人们尚未完全了解合成过程中的相关过程。为了给广泛的研究提供一个通用的工作平台,我们引入了标准化的 SpraySyn 燃烧器。本研究对改进型 SpraySyn 2.0 燃烧器进行了深入研究,确定了液滴、燃烧和颗粒的重要特征。采用广角光散射(WALS)技术,在燃烧器(HAB)上方 20 毫米至 45 毫米高度范围内测量了点燃乙醇喷雾产生的液滴尺寸,结果显示液滴比之前的 SpraySyn 1.0 小得多,这最终导致蒸发速度加快。通过对火焰化学发光的高速成像,对火焰波动进行了研究,结果表明与之前的燃烧器相比,火焰波动行为发生了变化。此外,还利用 WALS 对生成的氧化铁和二氧化钛纳米粒子在 30 毫米到 210 毫米的不同 HAB 下进行单次原位尺寸测量,从而观察粒子的生长情况。为了进一步评估所生产颗粒的特性,还对两种颗粒系统进行了广泛的 TEM 测量和评估。最后,通过将化学发光成像与 WALS 相结合,研究了火焰脉动对颗粒大小的影响,结果表明两者之间没有相关性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Characterization of the SpraySyn 2.0 burner: Droplet diameters, flame stability and particle sizes
Spray flame synthesis (SFS) is a promising technique for the production of metal-oxide nanoparticles. However, the processes involved during the synthesis are not yet fully understood. To provide a common workbench for a wide range of investigations, the standardized SpraySyn burners have been introduced. This work presents an in-depth investigation of the improved SpraySyn 2.0 burner, characterizing important droplet, combustion and particle features. The sizes of the droplets produced from an ignited ethanol spray are measured in a range between 20 mm and 45 mm height above the burner (HAB) employing wide-angle light scattering (WALS), revealing much smaller droplets compared to previous SpraySyn 1.0, which eventually leads to faster evaporation. Flame fluctuations are investigated using high-speed imaging of the flame chemiluminescence, indicating a change in fluctuation behaviour compared to the previous burner. WALS is also employed for single-shot in situ size measurements of produced iron-oxide and titanium-dioxide nanoparticles at various HABs ranging from 30 mm to 210 mm, allowing to observe the particle growth. To further assess the properties of the produced particles, extensive TEM measurements for both particle systems are conducted and evaluated. Finally, the influence of flame pulsations on particle size is investigated by coupling chemiluminescence imaging with WALS, yielding no correlation between both.
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CiteScore
4.20
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