耦合CdS量子点与多金属氧酸盐-负载[Re(CO)3]+催化剂的光催化CO2高效还原

IF 4.2 2区化学 Q2 CHEMISTRY, MULTIDISCIPLINARY

Chemical Communications Pub Date : 2025-03-14 DOI:10.1039/d5cc00726g

Yongkang Liu , Yuanyuan Dong , Jiaxin Yang , Yeqin Feng , Mengyun Zhao , Yun Qin , Hongjin Lv

引用次数: 0

摘要

将CdS量子点作为光吸收剂与多金属氧酸负载的[Re(CO)3]+ (POM-Re)催化剂相结合，构建了一个耦合的光催化体系，该体系具有将CO2光还原为HCOOH的高效活性。机理研究表明，Sb2W20Re2具有良好的光生电子迁移能力，使其具有高效的光催化CO2还原活性。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

Coupling CdS quantum dots with polyoxometalate-supported [Re(CO)3]+ catalysts for efficient photocatalytic CO2 reduction†

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Coupling CdS quantum dots with polyoxometalate-supported [Re(CO)3]+ catalysts for efficient photocatalytic CO2 reduction†

A coupled photocatalytic system has been constructed by integrating CdS quantum dots as a light-absorber and polyoxometalate-supported [Re(CO)₃]⁺ (POM-Re) catalysts, which exhibited efficient activity towards photoreduction of CO₂ to HCOOH. Mechanistic studies revealed that the favorable migration of photogenerated electrons endows with efficient photocatalytic CO₂ reduction activity.

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来源期刊

Chemical Communications 化学-化学综合

CiteScore

8.60

自引率

4.10%

发文量

2705

审稿时长

1.4 months

期刊介绍： ChemComm (Chemical Communications) is renowned as the fastest publisher of articles providing information on new avenues of research, drawn from all the world''s major areas of chemical research.