未来人为土地利用变化对碳质气溶胶的影响及其对气候和空气质量的影响

IF 4.6 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY
Yang Shi, Colette L. Heald, Maria Val Martin
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引用次数: 0

摘要

未来人为土地利用变化(LUC)可能通过扰动生物源和火源排放而改变大气中的碳质气溶胶(黑碳和有机气溶胶)负担。然而,对这种影响的研究很少。我们利用CESM2模式研究了从现在到2100年,在共享社会经济路径预测的再造林和森林砍伐情景下,未来含碳气溶胶的全球演变。与目前相比,未来生物源性挥发性有机化合物排放的变化是随着森林覆盖率的变化而变化的,而在森林砍伐火灾趋势的推动下,这两个预测的火灾排放都有所减少。相关的碳质气溶胶负荷变化在两种情景下均产生中等气溶胶直接辐射强迫(- 0.021至+0.034 W/m2)和PM2.5暴露量的中等平均减少(- 0.11至- 0.23 μg/m3)。我们发现,在确定大气碳质气溶胶负担方面,未来人为的土地利用变化可能比直接的人为排放更重要,这凸显了进一步限制土地利用变化影响的重要性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Future Anthropogenic Land Use Change Impacts on Carbonaceous Aerosol and Implications for Climate and Air Quality

Future Anthropogenic Land Use Change Impacts on Carbonaceous Aerosol and Implications for Climate and Air Quality

Future Anthropogenic Land Use Change Impacts on Carbonaceous Aerosol and Implications for Climate and Air Quality

Future Anthropogenic Land Use Change Impacts on Carbonaceous Aerosol and Implications for Climate and Air Quality

Future Anthropogenic Land Use Change Impacts on Carbonaceous Aerosol and Implications for Climate and Air Quality

Future anthropogenic land use change (LUC) may alter atmospheric carbonaceous aerosol (black carbon and organic aerosol) burden by perturbing biogenic and fire emissions. However, there has been little investigation of this effect. We examine the global evolution of future carbonaceous aerosol under the Shared Socioeconomic Pathways projected reforestation and deforestation scenarios using the CESM2 model from present-day to 2100. Compared to present-day, the change in future biogenic volatile organic compounds emission follows changes in forest coverage, while fire emissions decrease in both projections, driven by trends in deforestation fires. The associated carbonaceous aerosol burden change produces moderate aerosol direct radiative forcing (−0.021 to +0.034 W/m2) and modest mean reduction in PM2.5 exposure (−0.11 μg/m3 to −0.23 μg/m3) in both scenarios. We find that future anthropogenic LUC may be more important in determining atmospheric carbonaceous aerosol burden than direct anthropogenic emissions, highlighting the importance of further constraining the impact of LUC.

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来源期刊
Geophysical Research Letters
Geophysical Research Letters 地学-地球科学综合
CiteScore
9.00
自引率
9.60%
发文量
1588
审稿时长
2.2 months
期刊介绍: Geophysical Research Letters (GRL) publishes high-impact, innovative, and timely research on major scientific advances in all the major geoscience disciplines. Papers are communications-length articles and should have broad and immediate implications in their discipline or across the geosciences. GRLmaintains the fastest turn-around of all high-impact publications in the geosciences and works closely with authors to ensure broad visibility of top papers.
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