{"title":"非磁性二阶拓扑绝缘体中高陈氏数的工程量子反常霍尔效应","authors":"Xiaoran Feng, Yingxi Bai, Zhiqi Chen, Ying Dai, Baibiao Huang, Chengwang Niu","doi":"10.1002/adfm.202501934","DOIUrl":null,"url":null,"abstract":"Quantum anomalous Hall effect (QAHE) with a high Chern number hosts multiple dissipationless edge states, which is of significant fundamental and technological importance in low-dissipation spintronics. Here, in contrast to generally reported QAHE in 2D ferromagnets, the emergence of high-Chern-number QAHE in 2D nonmagnets is theoretically demonstrated. Remarkably, tight-binding model analyses and calculations show that Floquet engineering offers a fertile strategy to achieve the QAHE in 2D nonmagnetic second-order topological insulators (SOTIs), with the Chern number reaching as much as <span data-altimg=\"/cms/asset/c4c92865-2669-4f24-bbf6-21a776b1bcfd/adfm202501934-math-0001.png\"></span><mjx-container ctxtmenu_counter=\"1\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" role=\"application\" sre-explorer- style=\"font-size: 103%; position: relative;\" tabindex=\"0\"><mjx-math aria-hidden=\"true\" location=\"graphic/adfm202501934-math-0001.png\"><mjx-semantics><mjx-mrow data-semantic-children=\"0,4\" data-semantic-content=\"1\" data-semantic- data-semantic-role=\"equality\" data-semantic-speech=\"upper C equals plus or minus 6\" data-semantic-type=\"relseq\"><mjx-mi data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"latinletter\" data-semantic-type=\"identifier\"><mjx-c></mjx-c></mjx-mi><mjx-mo data-semantic- data-semantic-operator=\"relseq,=\" data-semantic-parent=\"5\" data-semantic-role=\"equality\" data-semantic-type=\"relation\" rspace=\"5\" space=\"5\"><mjx-c></mjx-c></mjx-mo><mjx-mrow data-semantic-children=\"3\" data-semantic-content=\"2\" data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"addition\" data-semantic-type=\"prefixop\"><mjx-mo data-semantic- data-semantic-operator=\"prefixop,±\" data-semantic-parent=\"4\" data-semantic-role=\"addition\" data-semantic-type=\"operator\" rspace=\"1\" style=\"margin-left: 0.056em;\"><mjx-c></mjx-c></mjx-mo><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"4\" data-semantic-role=\"integer\" data-semantic-type=\"number\"><mjx-c></mjx-c></mjx-mn></mjx-mrow></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\"inline\" unselectable=\"on\"><math altimg=\"urn:x-wiley:1616301X:media:adfm202501934:adfm202501934-math-0001\" display=\"inline\" location=\"graphic/adfm202501934-math-0001.png\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><semantics><mrow data-semantic-=\"\" data-semantic-children=\"0,4\" data-semantic-content=\"1\" data-semantic-role=\"equality\" data-semantic-speech=\"upper C equals plus or minus 6\" data-semantic-type=\"relseq\"><mi data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic-parent=\"5\" data-semantic-role=\"latinletter\" data-semantic-type=\"identifier\">C</mi><mo data-semantic-=\"\" data-semantic-operator=\"relseq,=\" data-semantic-parent=\"5\" data-semantic-role=\"equality\" data-semantic-type=\"relation\">=</mo><mrow data-semantic-=\"\" data-semantic-children=\"3\" data-semantic-content=\"2\" data-semantic-parent=\"5\" data-semantic-role=\"addition\" data-semantic-type=\"prefixop\"><mo data-semantic-=\"\" data-semantic-operator=\"prefixop,±\" data-semantic-parent=\"4\" data-semantic-role=\"addition\" data-semantic-type=\"operator\">±</mo><mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"4\" data-semantic-role=\"integer\" data-semantic-type=\"number\">6</mn></mrow></mrow>$C=\\pm 6$</annotation></semantics></math></mjx-assistive-mml></mjx-container>. Moreover, based on the Chern number, corner states, and edge states analyses, the SMoSiN<sub>2</sub> monolayer is identified as an experimentally feasible candidate of the proposed mechanism of Floquet QAHE, where a topological phase transition from the 2D nonmagnetic SOTI to QAHE emerges. These findings pave a technological avenue to bridge the higher-order topology and exotic QAH physics with high feasibility of applications in topological spintronics.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"8 1","pages":""},"PeriodicalIF":19.0000,"publicationDate":"2025-03-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Engineering Quantum Anomalous Hall Effect with a High Chern Number in Nonmagnetic Second-Order Topological Insulator\",\"authors\":\"Xiaoran Feng, Yingxi Bai, Zhiqi Chen, Ying Dai, Baibiao Huang, Chengwang Niu\",\"doi\":\"10.1002/adfm.202501934\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Quantum anomalous Hall effect (QAHE) with a high Chern number hosts multiple dissipationless edge states, which is of significant fundamental and technological importance in low-dissipation spintronics. Here, in contrast to generally reported QAHE in 2D ferromagnets, the emergence of high-Chern-number QAHE in 2D nonmagnets is theoretically demonstrated. Remarkably, tight-binding model analyses and calculations show that Floquet engineering offers a fertile strategy to achieve the QAHE in 2D nonmagnetic second-order topological insulators (SOTIs), with the Chern number reaching as much as <span data-altimg=\\\"/cms/asset/c4c92865-2669-4f24-bbf6-21a776b1bcfd/adfm202501934-math-0001.png\\\"></span><mjx-container ctxtmenu_counter=\\\"1\\\" ctxtmenu_oldtabindex=\\\"1\\\" jax=\\\"CHTML\\\" role=\\\"application\\\" sre-explorer- style=\\\"font-size: 103%; position: relative;\\\" tabindex=\\\"0\\\"><mjx-math aria-hidden=\\\"true\\\" location=\\\"graphic/adfm202501934-math-0001.png\\\"><mjx-semantics><mjx-mrow data-semantic-children=\\\"0,4\\\" data-semantic-content=\\\"1\\\" data-semantic- data-semantic-role=\\\"equality\\\" data-semantic-speech=\\\"upper C equals plus or minus 6\\\" data-semantic-type=\\\"relseq\\\"><mjx-mi data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"italic\\\" data-semantic- data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"latinletter\\\" data-semantic-type=\\\"identifier\\\"><mjx-c></mjx-c></mjx-mi><mjx-mo data-semantic- data-semantic-operator=\\\"relseq,=\\\" data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"equality\\\" data-semantic-type=\\\"relation\\\" rspace=\\\"5\\\" space=\\\"5\\\"><mjx-c></mjx-c></mjx-mo><mjx-mrow data-semantic-children=\\\"3\\\" data-semantic-content=\\\"2\\\" data-semantic- data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"addition\\\" data-semantic-type=\\\"prefixop\\\"><mjx-mo data-semantic- data-semantic-operator=\\\"prefixop,±\\\" data-semantic-parent=\\\"4\\\" data-semantic-role=\\\"addition\\\" data-semantic-type=\\\"operator\\\" rspace=\\\"1\\\" style=\\\"margin-left: 0.056em;\\\"><mjx-c></mjx-c></mjx-mo><mjx-mn data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic- data-semantic-parent=\\\"4\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\"><mjx-c></mjx-c></mjx-mn></mjx-mrow></mjx-mrow></mjx-semantics></mjx-math><mjx-assistive-mml display=\\\"inline\\\" unselectable=\\\"on\\\"><math altimg=\\\"urn:x-wiley:1616301X:media:adfm202501934:adfm202501934-math-0001\\\" display=\\\"inline\\\" location=\\\"graphic/adfm202501934-math-0001.png\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><semantics><mrow data-semantic-=\\\"\\\" data-semantic-children=\\\"0,4\\\" data-semantic-content=\\\"1\\\" data-semantic-role=\\\"equality\\\" data-semantic-speech=\\\"upper C equals plus or minus 6\\\" data-semantic-type=\\\"relseq\\\"><mi data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"italic\\\" data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"latinletter\\\" data-semantic-type=\\\"identifier\\\">C</mi><mo data-semantic-=\\\"\\\" data-semantic-operator=\\\"relseq,=\\\" data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"equality\\\" data-semantic-type=\\\"relation\\\">=</mo><mrow data-semantic-=\\\"\\\" data-semantic-children=\\\"3\\\" data-semantic-content=\\\"2\\\" data-semantic-parent=\\\"5\\\" data-semantic-role=\\\"addition\\\" data-semantic-type=\\\"prefixop\\\"><mo data-semantic-=\\\"\\\" data-semantic-operator=\\\"prefixop,±\\\" data-semantic-parent=\\\"4\\\" data-semantic-role=\\\"addition\\\" data-semantic-type=\\\"operator\\\">±</mo><mn data-semantic-=\\\"\\\" data-semantic-annotation=\\\"clearspeak:simple\\\" data-semantic-font=\\\"normal\\\" data-semantic-parent=\\\"4\\\" data-semantic-role=\\\"integer\\\" data-semantic-type=\\\"number\\\">6</mn></mrow></mrow>$C=\\\\pm 6$</annotation></semantics></math></mjx-assistive-mml></mjx-container>. Moreover, based on the Chern number, corner states, and edge states analyses, the SMoSiN<sub>2</sub> monolayer is identified as an experimentally feasible candidate of the proposed mechanism of Floquet QAHE, where a topological phase transition from the 2D nonmagnetic SOTI to QAHE emerges. These findings pave a technological avenue to bridge the higher-order topology and exotic QAH physics with high feasibility of applications in topological spintronics.\",\"PeriodicalId\":112,\"journal\":{\"name\":\"Advanced Functional Materials\",\"volume\":\"8 1\",\"pages\":\"\"},\"PeriodicalIF\":19.0000,\"publicationDate\":\"2025-03-12\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advanced Functional Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1002/adfm.202501934\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Functional Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1002/adfm.202501934","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Engineering Quantum Anomalous Hall Effect with a High Chern Number in Nonmagnetic Second-Order Topological Insulator
Quantum anomalous Hall effect (QAHE) with a high Chern number hosts multiple dissipationless edge states, which is of significant fundamental and technological importance in low-dissipation spintronics. Here, in contrast to generally reported QAHE in 2D ferromagnets, the emergence of high-Chern-number QAHE in 2D nonmagnets is theoretically demonstrated. Remarkably, tight-binding model analyses and calculations show that Floquet engineering offers a fertile strategy to achieve the QAHE in 2D nonmagnetic second-order topological insulators (SOTIs), with the Chern number reaching as much as . Moreover, based on the Chern number, corner states, and edge states analyses, the SMoSiN2 monolayer is identified as an experimentally feasible candidate of the proposed mechanism of Floquet QAHE, where a topological phase transition from the 2D nonmagnetic SOTI to QAHE emerges. These findings pave a technological avenue to bridge the higher-order topology and exotic QAH physics with high feasibility of applications in topological spintronics.
期刊介绍:
Firmly established as a top-tier materials science journal, Advanced Functional Materials reports breakthrough research in all aspects of materials science, including nanotechnology, chemistry, physics, and biology every week.
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