Yuan Fa, Agata Piacentini, Bart Macco, Holger Kalisch, Michael Heuken, Andrei Vescan, Zhenxing Wang, Max C. Lemme
{"title":"通过反向溅射诱导结构修饰优化MoS2场效应晶体管的接触电阻","authors":"Yuan Fa, Agata Piacentini, Bart Macco, Holger Kalisch, Michael Heuken, Andrei Vescan, Zhenxing Wang, Max C. Lemme","doi":"10.1021/acsami.4c21596","DOIUrl":null,"url":null,"abstract":"Two-dimensional material (2DM)-based field-effect transistors (FETs), such as molybdenum disulfide (MoS<sub>2</sub>)-FETs, have gained significant attention for their potential for ultrashort channels, thereby extending Moore’s law. However, MoS<sub>2</sub>–FETs are prone to the formation of Schottky barriers at the metal-MoS<sub>2</sub> interface, resulting in high contact resistance (<i>R</i><sub>c</sub>) and, consequently, reduced transistor currents in the ON-state. Our study explores the modification of MoS<sub>2</sub> to induce the formation of conductive 1T-MoS<sub>2</sub> at the metal-MoS<sub>2</sub> interface via reverse sputtering. MoS<sub>2</sub>–FETs exposed to optimized reverse sputtering conditions in the contact area show <i>R</i><sub>c</sub> values reduced to less than 50% of their untreated counterparts. This reduction translates into improvements in other electrical characteristics, such as higher ON-state currents. Since reverse sputtering is a standard semiconductor process that enhances the electrical performance of MoS<sub>2</sub>–FETs, it has great potential for broader application scenarios in 2DM-based microelectronic devices and circuits.","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":"4 1","pages":""},"PeriodicalIF":8.2000,"publicationDate":"2025-03-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Contact Resistance Optimization in MoS2 Field-Effect Transistors through Reverse Sputtering-Induced Structural Modifications\",\"authors\":\"Yuan Fa, Agata Piacentini, Bart Macco, Holger Kalisch, Michael Heuken, Andrei Vescan, Zhenxing Wang, Max C. Lemme\",\"doi\":\"10.1021/acsami.4c21596\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Two-dimensional material (2DM)-based field-effect transistors (FETs), such as molybdenum disulfide (MoS<sub>2</sub>)-FETs, have gained significant attention for their potential for ultrashort channels, thereby extending Moore’s law. However, MoS<sub>2</sub>–FETs are prone to the formation of Schottky barriers at the metal-MoS<sub>2</sub> interface, resulting in high contact resistance (<i>R</i><sub>c</sub>) and, consequently, reduced transistor currents in the ON-state. Our study explores the modification of MoS<sub>2</sub> to induce the formation of conductive 1T-MoS<sub>2</sub> at the metal-MoS<sub>2</sub> interface via reverse sputtering. MoS<sub>2</sub>–FETs exposed to optimized reverse sputtering conditions in the contact area show <i>R</i><sub>c</sub> values reduced to less than 50% of their untreated counterparts. This reduction translates into improvements in other electrical characteristics, such as higher ON-state currents. Since reverse sputtering is a standard semiconductor process that enhances the electrical performance of MoS<sub>2</sub>–FETs, it has great potential for broader application scenarios in 2DM-based microelectronic devices and circuits.\",\"PeriodicalId\":5,\"journal\":{\"name\":\"ACS Applied Materials & Interfaces\",\"volume\":\"4 1\",\"pages\":\"\"},\"PeriodicalIF\":8.2000,\"publicationDate\":\"2025-03-11\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Materials & Interfaces\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1021/acsami.4c21596\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Materials & Interfaces","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acsami.4c21596","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Contact Resistance Optimization in MoS2 Field-Effect Transistors through Reverse Sputtering-Induced Structural Modifications
Two-dimensional material (2DM)-based field-effect transistors (FETs), such as molybdenum disulfide (MoS2)-FETs, have gained significant attention for their potential for ultrashort channels, thereby extending Moore’s law. However, MoS2–FETs are prone to the formation of Schottky barriers at the metal-MoS2 interface, resulting in high contact resistance (Rc) and, consequently, reduced transistor currents in the ON-state. Our study explores the modification of MoS2 to induce the formation of conductive 1T-MoS2 at the metal-MoS2 interface via reverse sputtering. MoS2–FETs exposed to optimized reverse sputtering conditions in the contact area show Rc values reduced to less than 50% of their untreated counterparts. This reduction translates into improvements in other electrical characteristics, such as higher ON-state currents. Since reverse sputtering is a standard semiconductor process that enhances the electrical performance of MoS2–FETs, it has great potential for broader application scenarios in 2DM-based microelectronic devices and circuits.
期刊介绍:
ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.