根据水位动态确定水质变化的关键阶段、污染物和驱动机制

IF 3.8 4区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES
Xuefeng Wu, Yan Jiang, Yiping Chen, Yucong Hu, Zhenfang Huang
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引用次数: 0

摘要

区分水质对水位的响应对改善水库水质和生态系统稳定性具有重要意义。目前的研究主要从整体角度研究水位与水质之间的关系,对高水位、低水位、水位下降、水位上升等各种状态的区分并不频繁。本文以密云水库为例,研究了过去 31 年水库水质、水位和营养物质输入的变化趋势。论文采用层次划分分析法研究了营养物质输入和水位对水库水质的相对影响,并确定了水位影响水质的主要阶段、污染物和驱动机制。研究结果表明,在任何情况下,总磷都主要受营养物质输入的制约。在高水位时,营养物质的输入会对水质产生重大影响。相反,在其他阶段,水位是影响含氮物质变化的主要因素。通过分析硝态氮比例、水力停留时间以及氨化、硝化和反硝化过程之间的关系,确定水位影响氮浓度变化的机制在三个阶段有所不同。在水位下降阶段,水库缺氧抑制了硝化过程,导致氨氮积累。在低水位阶段,反硝化率在水位下降后继续下降,导致总氮和硝态氮浓度增加。在水位上升阶段,波动带向水中释放了大量氨氮,导致总氮和氨氮浓度上升。这些发现为加强水环境管理策略提供了一个基础框架,旨在通过调节水位改善水质。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Identifying the Key Stages, Pollutants, and Driving Mechanisms of Water Quality Variation in Relation to Water Level Dynamics

Distinguishing the response of water quality to water level is of great significance for improving reservoir water quality and ecosystems stability. Present research primarily examines the relationship between water level and water quality from a holistic perspective, with infrequent differentiation among various states such as high water level, low water level, water level decline, and water level rise. The paper focused on Miyun Reservoir as a case study, examining the trends in reservoir water quality, water level, and nutrient input over the past 31 years. It employed hierarchical partitioning analysis to investigate the relative impacts of nutrient input and water level on reservoir water quality and identify the main stages, pollutants, and driving mechanisms by which water level influences water quality. The findings indicated that, in every instance, total phosphorus was predominantly constrained by nutrient input. At high water levels, nutrient input significantly impacted water quality. Conversely, during other stages, water level was the primary factor that affecting the variations in nitrogen-containing substances. Through the analysis of relationships among nitrate nitrogen proportions, hydraulic retention time, and the processes of ammonification, nitrification, and denitrification, the mechanisms by which water levels influence nitrogen concentration variations were determined to differ across the three stages. During the drop of water level, the hypoxia in the reservoir inhibited the nitrification process, leading to the accumulation of ammonia nitrogen. In the low water level stage, the denitrification rate continued to decline after the water level dropped, resulting in increased concentrations of total nitrogen and nitrate nitrogen. During the water level rise stage, the fluctuation zone released significant amounts of ammonia nitrogen into the water, causing a rise in total nitrogen and ammonia nitrogen concentrations. These findings could offer a foundational framework for enhancing water environment management strategies aimed at improving water quality through the regulation of water levels.

Graphical abstract

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来源期刊
Water, Air, & Soil Pollution
Water, Air, & Soil Pollution 环境科学-环境科学
CiteScore
4.50
自引率
6.90%
发文量
448
审稿时长
2.6 months
期刊介绍: Water, Air, & Soil Pollution is an international, interdisciplinary journal on all aspects of pollution and solutions to pollution in the biosphere. This includes chemical, physical and biological processes affecting flora, fauna, water, air and soil in relation to environmental pollution. Because of its scope, the subject areas are diverse and include all aspects of pollution sources, transport, deposition, accumulation, acid precipitation, atmospheric pollution, metals, aquatic pollution including marine pollution and ground water, waste water, pesticides, soil pollution, sewage, sediment pollution, forestry pollution, effects of pollutants on humans, vegetation, fish, aquatic species, micro-organisms, and animals, environmental and molecular toxicology applied to pollution research, biosensors, global and climate change, ecological implications of pollution and pollution models. Water, Air, & Soil Pollution also publishes manuscripts on novel methods used in the study of environmental pollutants, environmental toxicology, environmental biology, novel environmental engineering related to pollution, biodiversity as influenced by pollution, novel environmental biotechnology as applied to pollution (e.g. bioremediation), environmental modelling and biorestoration of polluted environments. Articles should not be submitted that are of local interest only and do not advance international knowledge in environmental pollution and solutions to pollution. Articles that simply replicate known knowledge or techniques while researching a local pollution problem will normally be rejected without review. Submitted articles must have up-to-date references, employ the correct experimental replication and statistical analysis, where needed and contain a significant contribution to new knowledge. The publishing and editorial team sincerely appreciate your cooperation. Water, Air, & Soil Pollution publishes research papers; review articles; mini-reviews; and book reviews.
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