{"title":"透射模式AlGaN纳米阵列光电阴极从光子激发到电子收集四步的三维输运机制","authors":"Xian Wu , Yu Diao , Sihao Xia","doi":"10.1016/j.apsusc.2025.162927","DOIUrl":null,"url":null,"abstract":"<div><div>This study focuses on the photoemission model of transmissive AlGaN nanoarray cathodes. By introducing energy-dependent absorption coefficient and a new calculation method upon escape probability of photoelectrons, we establish a three-dimensional transmissive photoemission model. Based on the photoemission model, the influences of multiple parameters (geometric, surface, environmental, material) on cathode performance are explored. It is found that the quantum efficiency (QE) attains a better response with high-energy photons irradiated. When the height of the nanoarray is 90 nm and the diameter is 60 nm, the QE generates a high response up to 24.6 % and 22.4 %. When the external electric field is less than 1 V/μm, the enhancement of the external electric field can improve the effective quantum efficiency (EQE), especially when low-energy photons less than 4 eV are incident. The increase of Al composition from 0 to 1 lead to an increasing response threshold of EQE from 3.4 eV to 6.3 eV. Al<sub>x</sub>Ga<sub>1-x</sub>N array cathodes with different Al compositions all exhibit the highest EQE near the threshold. This study provides a new theoretical basis and computational idea for development of the transmissive photocathode with nanoarray structure.</div></div>","PeriodicalId":247,"journal":{"name":"Applied Surface Science","volume":"695 ","pages":"Article 162927"},"PeriodicalIF":6.9000,"publicationDate":"2025-03-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Three-dimensional transportation mechanism of transmission-mode AlGaN nanoarray photocathode within four steps from photon excitation to electron collection\",\"authors\":\"Xian Wu , Yu Diao , Sihao Xia\",\"doi\":\"10.1016/j.apsusc.2025.162927\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>This study focuses on the photoemission model of transmissive AlGaN nanoarray cathodes. By introducing energy-dependent absorption coefficient and a new calculation method upon escape probability of photoelectrons, we establish a three-dimensional transmissive photoemission model. Based on the photoemission model, the influences of multiple parameters (geometric, surface, environmental, material) on cathode performance are explored. It is found that the quantum efficiency (QE) attains a better response with high-energy photons irradiated. When the height of the nanoarray is 90 nm and the diameter is 60 nm, the QE generates a high response up to 24.6 % and 22.4 %. When the external electric field is less than 1 V/μm, the enhancement of the external electric field can improve the effective quantum efficiency (EQE), especially when low-energy photons less than 4 eV are incident. The increase of Al composition from 0 to 1 lead to an increasing response threshold of EQE from 3.4 eV to 6.3 eV. Al<sub>x</sub>Ga<sub>1-x</sub>N array cathodes with different Al compositions all exhibit the highest EQE near the threshold. This study provides a new theoretical basis and computational idea for development of the transmissive photocathode with nanoarray structure.</div></div>\",\"PeriodicalId\":247,\"journal\":{\"name\":\"Applied Surface Science\",\"volume\":\"695 \",\"pages\":\"Article 162927\"},\"PeriodicalIF\":6.9000,\"publicationDate\":\"2025-03-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Applied Surface Science\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0169433225006415\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Applied Surface Science","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0169433225006415","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Three-dimensional transportation mechanism of transmission-mode AlGaN nanoarray photocathode within four steps from photon excitation to electron collection
This study focuses on the photoemission model of transmissive AlGaN nanoarray cathodes. By introducing energy-dependent absorption coefficient and a new calculation method upon escape probability of photoelectrons, we establish a three-dimensional transmissive photoemission model. Based on the photoemission model, the influences of multiple parameters (geometric, surface, environmental, material) on cathode performance are explored. It is found that the quantum efficiency (QE) attains a better response with high-energy photons irradiated. When the height of the nanoarray is 90 nm and the diameter is 60 nm, the QE generates a high response up to 24.6 % and 22.4 %. When the external electric field is less than 1 V/μm, the enhancement of the external electric field can improve the effective quantum efficiency (EQE), especially when low-energy photons less than 4 eV are incident. The increase of Al composition from 0 to 1 lead to an increasing response threshold of EQE from 3.4 eV to 6.3 eV. AlxGa1-xN array cathodes with different Al compositions all exhibit the highest EQE near the threshold. This study provides a new theoretical basis and computational idea for development of the transmissive photocathode with nanoarray structure.
期刊介绍:
Applied Surface Science covers topics contributing to a better understanding of surfaces, interfaces, nanostructures and their applications. The journal is concerned with scientific research on the atomic and molecular level of material properties determined with specific surface analytical techniques and/or computational methods, as well as the processing of such structures.