{"title":"HiGee 辅助气泡柱反应器中的微气泡群:尺寸、气体容纳量和有效界面面积","authors":"Li-Hua Wang, Hai-Long Liao, Liang Zheng, Zhi-Xuan Fan, Hai-Kui Zou, Yong Luo","doi":"10.1002/aic.18804","DOIUrl":null,"url":null,"abstract":"Microbubble technology is promising for intensifying gas–liquid mass transfer in the bubble column reactor (BCR). The HiGee microbubble generator (HMG), flexibly controlling the microbubble size by adjusting the rotational speed, was developed for the BCR with obvious advantages. However, the hydrodynamics and mass transfer performance of the microbubble swarm generated by HMG in the bubble column were not clear, which hinders its industrial application process. In this work, a HiGee-aided bubble column reactor (HBCR), including an HMG and a bubble column, was proposed and designed. The effects of operating conditions on flow behavior, Sauter mean diameter (<i>d</i><sub>32</sub>), and gas holdup (<i>φ</i><sub><i>G</i></sub>) were studied. A prediction model for gas holdup was established, and the deviation between the predicted and experimental values was within ±15%. Based on <i>d</i><sub>32</sub> and <i>φ</i><sub><i>G</i></sub>, the effective interfacial area in HBCR was calculated as 500–3800 m<sup>2</sup>/m<sup>3</sup>. This study provided fundamental data for the design and scale-up of HBCR.","PeriodicalId":120,"journal":{"name":"AIChE Journal","volume":"34 1","pages":""},"PeriodicalIF":3.5000,"publicationDate":"2025-03-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Microbubble swarm in a HiGee-aided bubble column reactor: Size, gas holdup, and effective interfacial area\",\"authors\":\"Li-Hua Wang, Hai-Long Liao, Liang Zheng, Zhi-Xuan Fan, Hai-Kui Zou, Yong Luo\",\"doi\":\"10.1002/aic.18804\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Microbubble technology is promising for intensifying gas–liquid mass transfer in the bubble column reactor (BCR). The HiGee microbubble generator (HMG), flexibly controlling the microbubble size by adjusting the rotational speed, was developed for the BCR with obvious advantages. However, the hydrodynamics and mass transfer performance of the microbubble swarm generated by HMG in the bubble column were not clear, which hinders its industrial application process. In this work, a HiGee-aided bubble column reactor (HBCR), including an HMG and a bubble column, was proposed and designed. The effects of operating conditions on flow behavior, Sauter mean diameter (<i>d</i><sub>32</sub>), and gas holdup (<i>φ</i><sub><i>G</i></sub>) were studied. A prediction model for gas holdup was established, and the deviation between the predicted and experimental values was within ±15%. Based on <i>d</i><sub>32</sub> and <i>φ</i><sub><i>G</i></sub>, the effective interfacial area in HBCR was calculated as 500–3800 m<sup>2</sup>/m<sup>3</sup>. This study provided fundamental data for the design and scale-up of HBCR.\",\"PeriodicalId\":120,\"journal\":{\"name\":\"AIChE Journal\",\"volume\":\"34 1\",\"pages\":\"\"},\"PeriodicalIF\":3.5000,\"publicationDate\":\"2025-03-03\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"AIChE Journal\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://doi.org/10.1002/aic.18804\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"AIChE Journal","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1002/aic.18804","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
Microbubble swarm in a HiGee-aided bubble column reactor: Size, gas holdup, and effective interfacial area
Microbubble technology is promising for intensifying gas–liquid mass transfer in the bubble column reactor (BCR). The HiGee microbubble generator (HMG), flexibly controlling the microbubble size by adjusting the rotational speed, was developed for the BCR with obvious advantages. However, the hydrodynamics and mass transfer performance of the microbubble swarm generated by HMG in the bubble column were not clear, which hinders its industrial application process. In this work, a HiGee-aided bubble column reactor (HBCR), including an HMG and a bubble column, was proposed and designed. The effects of operating conditions on flow behavior, Sauter mean diameter (d32), and gas holdup (φG) were studied. A prediction model for gas holdup was established, and the deviation between the predicted and experimental values was within ±15%. Based on d32 and φG, the effective interfacial area in HBCR was calculated as 500–3800 m2/m3. This study provided fundamental data for the design and scale-up of HBCR.
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