IF 9.6 1区 化学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Xichen Hu, Xianhu Liu, Quan Xu, Olli Ikkala and Bo Peng*, 
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引用次数: 0

摘要

生物传感器的特点是适应不同的刺激范围,能比绝对刺激值更早有效地检测到刺激变化,受此启发,我们提出了一种机械传感概念,通过磁场(H)门控来调整分辨率,以检测各种压缩刺激下的微小压力变化。在电压偏置下,通过平面电极之间的软铁磁导电粒子的柱状 H 驱动组件实现电阻式传感。通过对 H 值进行调制,这些柱状物就能以机械适应性灵敏度做出响应。H 值越高,电流分辨率越高,但由于组装中胶体之间的磁结构干扰增加,重复测量的散度也会增加。为了在电流分辨率和散射之间权衡利弊,我们引入了机器学习来搜索最佳 H 门,从而促进有效的压力预测。这种方法为开发自适应刺激响应型机械传感器提出了生物启发路径,通过机器学习提高效率,检测不同刺激水平下的微妙变化。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Mechanosensing of Stimuli Changes with Magnetically Gated Adaptive Sensitivity

Inspired by biological sensors that characteristically adapt to varying stimulus ranges, efficiently detecting stimulus changes sooner than the absolute stimulus values, we propose a mechanosensing concept in which the resolution can be adapted by magnetic field (H) gating to detect small pressure-changes under a wide range of compressive stimuli. This is realized with resistive sensing by pillared H-driven assemblies of soft ferromagnetic electrically conducting particles between planar electrodes under a voltage bias. By modulation of H, the pillars respond with mechanically adaptable sensitivity. Higher H enhances current resolution, while it increases scatter among repeating measurements due to increased magnetic structural jamming between colloids in their assembly. To manage the trade-off between electrical resolution and scatter, machine learning is introduced for searching optimum H gatings, thus facilitating efficient pressure prediction. This approach suggests bioinspired pathways for developing adaptive stimulus-responsive mechanosensors, detecting subtle changes across varying stimuli levels with enhanced effectiveness through machine learning.

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来源期刊
ACS Materials Letters
ACS Materials Letters MATERIALS SCIENCE, MULTIDISCIPLINARY-
CiteScore
14.60
自引率
3.50%
发文量
261
期刊介绍: ACS Materials Letters is a journal that publishes high-quality and urgent papers at the forefront of fundamental and applied research in the field of materials science. It aims to bridge the gap between materials and other disciplines such as chemistry, engineering, and biology. The journal encourages multidisciplinary and innovative research that addresses global challenges. Papers submitted to ACS Materials Letters should clearly demonstrate the need for rapid disclosure of key results. The journal is interested in various areas including the design, synthesis, characterization, and evaluation of emerging materials, understanding the relationships between structure, property, and performance, as well as developing materials for applications in energy, environment, biomedical, electronics, and catalysis. The journal has a 2-year impact factor of 11.4 and is dedicated to publishing transformative materials research with fast processing times. The editors and staff of ACS Materials Letters actively participate in major scientific conferences and engage closely with readers and authors. The journal also maintains an active presence on social media to provide authors with greater visibility.
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