甘蔗渣基多孔花状MoS2/碳复合材料的高效微波吸收

IF 5.5 3区 材料科学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Yingxiu Zhang, Lihui Xu, Jiahao Wang, Hong Pan, Meiran Dou, Yi Teng, Xueqiang Fu, Zhangyong Liu, Xinzhe Huang, Meng Wang
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引用次数: 0

摘要

生物质碳材料以其成本低、重量轻、可持续性等优点在电磁波吸收领域受到广泛关注。以天然废甘蔗渣为原料,采用正化活化法制备甘蔗渣基多孔炭(BPC)。采用水热法制备了多孔花状MoS2/BPC复合材料,并在BPC的多孔结构中原位形成花状MoS2,成功制备了具有高效微波吸收性能的多孔花状MoS2/BPC复合材料。考察了水热时间和水热温度对制备样品表面形貌、石墨化程度、表面化学成分和阻抗匹配的影响。结果表明,当水热温度为220℃,水热时间为24 h时,得到的MoS2/BPC样品(称为MoS2/BPC-220℃)在8.96 GHz处的最小反射损耗值(RL)为- 41.6 dB,在相对较薄的1.5 mm厚度处的有效微波吸收带宽(EAB)为4.32 GHz。这项工作为制备具有强宽带电磁吸收性能的新型生物质衍生多孔碳提供了一条有前途的途径。图形抽象
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Bagasse-based porous flower-like MoS2/carbon composites for efficient microwave absorption

Biomass-derived carbon materials have attracted considerable attention in electromagnetic wave (EMW) absorption applications due to their advantages of low cost, light weight, and sustainability. Herein, bagasse-based porous carbon (BPC) was prepared by canonization and activation process from natural waste bagasse. The porous flower-like MoS2/BPC composites were successfully prepared for efficient microwave absorption via hydrothermal process by in-situ formation of flower-like MoS2 into the porous structure of BPC. The effect of hydrothermal time and hydrothermal temperature on surface morphology, degree of graphitization, surface chemical composition and impedance matching of the prepared samples was investigated. Results demonstrated that when the hydrothermal temperature was 220 °C, and the hydrothermal time was 24 h, the obtained MoS2/BPC sample (named as MoS2/BPC-220 ℃) showed the minimum reflection loss value (RL) of − 41.6 dB at 8.96 GHz and exhibited effective microwave absorption bandwidth (EAB) of 4.32 GHz at a relatively thin thickness of 1.5 mm. This work provides a promising way to prepare novel biomass-derived porous carbon for strong broadband electromagnetic absorption.

Graphical abstract

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来源期刊
Carbon Letters
Carbon Letters CHEMISTRY, MULTIDISCIPLINARY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
7.30
自引率
20.00%
发文量
118
期刊介绍: Carbon Letters aims to be a comprehensive journal with complete coverage of carbon materials and carbon-rich molecules. These materials range from, but are not limited to, diamond and graphite through chars, semicokes, mesophase substances, carbon fibers, carbon nanotubes, graphenes, carbon blacks, activated carbons, pyrolytic carbons, glass-like carbons, etc. Papers on the secondary production of new carbon and composite materials from the above mentioned various carbons are within the scope of the journal. Papers on organic substances, including coals, will be considered only if the research has close relation to the resulting carbon materials. Carbon Letters also seeks to keep abreast of new developments in their specialist fields and to unite in finding alternative energy solutions to current issues such as the greenhouse effect and the depletion of the ozone layer. The renewable energy basics, energy storage and conversion, solar energy, wind energy, water energy, nuclear energy, biomass energy, hydrogen production technology, and other clean energy technologies are also within the scope of the journal. Carbon Letters invites original reports of fundamental research in all branches of the theory and practice of carbon science and technology.
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