Xintao Lai, Tongyu Li, Xiaoyu Hou, Florian Vogelbacher, Jiajun Wang, Yanlin Song, Lei Shi, Mingzhu Li
{"title":"手性结构颜色来自微圆顶","authors":"Xintao Lai, Tongyu Li, Xiaoyu Hou, Florian Vogelbacher, Jiajun Wang, Yanlin Song, Lei Shi, Mingzhu Li","doi":"10.1073/pnas.2419113122","DOIUrl":null,"url":null,"abstract":"Artificial chiral-structural-color materials can carry high-dimensional information based on multiple optical degrees of freedom, providing possibilities for advanced optical security and information storage. However, current artificial chiral-structural-color materials are hindered by their specific compositions, fine nanostructures, and single polarization modulation. Here, we found that microdomes made from common polymers have chiral structural colors with broadband tunability and multiple polarization-modulated chirality. The microdome patterns are easily fabricated by ordinary printing techniques and have inhomogeneous spatial distributions of full polarization states and customizable colors. Our chiral-structural-color microdomes (CSCMs) provide a promising roadmap for high-capacity information encryption and high-security anti-counterfeiting. We developed multidimensional tunable structural color displays and achieved encryption with high information capacity. To further highlight the application potential, we constructed contact lenses integrated with CSCMs for identity authentication with 2 <jats:sup>32</jats:sup> distinctive cryptograms.","PeriodicalId":20548,"journal":{"name":"Proceedings of the National Academy of Sciences of the United States of America","volume":"51 1","pages":""},"PeriodicalIF":9.1000,"publicationDate":"2025-02-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Chiral structural color from microdomes\",\"authors\":\"Xintao Lai, Tongyu Li, Xiaoyu Hou, Florian Vogelbacher, Jiajun Wang, Yanlin Song, Lei Shi, Mingzhu Li\",\"doi\":\"10.1073/pnas.2419113122\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Artificial chiral-structural-color materials can carry high-dimensional information based on multiple optical degrees of freedom, providing possibilities for advanced optical security and information storage. However, current artificial chiral-structural-color materials are hindered by their specific compositions, fine nanostructures, and single polarization modulation. Here, we found that microdomes made from common polymers have chiral structural colors with broadband tunability and multiple polarization-modulated chirality. The microdome patterns are easily fabricated by ordinary printing techniques and have inhomogeneous spatial distributions of full polarization states and customizable colors. Our chiral-structural-color microdomes (CSCMs) provide a promising roadmap for high-capacity information encryption and high-security anti-counterfeiting. We developed multidimensional tunable structural color displays and achieved encryption with high information capacity. To further highlight the application potential, we constructed contact lenses integrated with CSCMs for identity authentication with 2 <jats:sup>32</jats:sup> distinctive cryptograms.\",\"PeriodicalId\":20548,\"journal\":{\"name\":\"Proceedings of the National Academy of Sciences of the United States of America\",\"volume\":\"51 1\",\"pages\":\"\"},\"PeriodicalIF\":9.1000,\"publicationDate\":\"2025-02-25\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Proceedings of the National Academy of Sciences of the United States of America\",\"FirstCategoryId\":\"103\",\"ListUrlMain\":\"https://doi.org/10.1073/pnas.2419113122\",\"RegionNum\":1,\"RegionCategory\":\"综合性期刊\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MULTIDISCIPLINARY SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Proceedings of the National Academy of Sciences of the United States of America","FirstCategoryId":"103","ListUrlMain":"https://doi.org/10.1073/pnas.2419113122","RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MULTIDISCIPLINARY SCIENCES","Score":null,"Total":0}
Artificial chiral-structural-color materials can carry high-dimensional information based on multiple optical degrees of freedom, providing possibilities for advanced optical security and information storage. However, current artificial chiral-structural-color materials are hindered by their specific compositions, fine nanostructures, and single polarization modulation. Here, we found that microdomes made from common polymers have chiral structural colors with broadband tunability and multiple polarization-modulated chirality. The microdome patterns are easily fabricated by ordinary printing techniques and have inhomogeneous spatial distributions of full polarization states and customizable colors. Our chiral-structural-color microdomes (CSCMs) provide a promising roadmap for high-capacity information encryption and high-security anti-counterfeiting. We developed multidimensional tunable structural color displays and achieved encryption with high information capacity. To further highlight the application potential, we constructed contact lenses integrated with CSCMs for identity authentication with 2 32 distinctive cryptograms.
期刊介绍:
The Proceedings of the National Academy of Sciences (PNAS), a peer-reviewed journal of the National Academy of Sciences (NAS), serves as an authoritative source for high-impact, original research across the biological, physical, and social sciences. With a global scope, the journal welcomes submissions from researchers worldwide, making it an inclusive platform for advancing scientific knowledge.