成渝地区臭氧形成敏感性时空特征及其影响因素[j]。

Q2 Environmental Science
Wen Xu, Hao Yang, Min He, Zhen Yang, Yang Zhang, Zhi-Hong Liu, Yu-Ming He
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引用次数: 0

摘要

为研究成渝地区夏季臭氧形成敏感性变化特征,利用OMI对流层HCHO和NO2柱浓度卫星观测资料,分析了夏季臭氧形成敏感性(OFS)。此外,利用大地探测器确定了气象因子、源排放及其相互作用对OFS的影响。结果表明:成渝地区夏季OFS分区以过渡区为主,占42.42%;vocs限制较少,主要分布在成都市和重庆市市区,面积占比为16.37%。nox限制区主要分布在雅安市、乐山市、宜宾市、泸州市和重庆市东部,面积占41.21%。6 - 8月vocs限制区面积逐渐减少,8月达到最低值,仅占3.53%,9月vocs限制区面积显著增加。污染物排放(CO、PM2.5、NMVOC和NOx)是影响成渝地区夏季OFS的主要因素。随着排放量的增加,FNR逐渐减小,OFS趋于vocs限制状态。SP、T2和TCW是影响成渝地区夏季OFS变化的3个主要气象因子。3个因子均与FNR呈负相关,SP、T2和TCW值越大,OFS越容易转变为vocs限制状态。各因子间的相互作用加剧了成渝地区夏季OFS的变化,是其时空变化的主要驱动因素。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
[Spatial and Temporal Characteristics of Ozone Formation Sensitivity and Its Influencing Factors in Chengdu-Chongqing Area].

To study the characteristics of ozone formation sensitivity changes in the Chengdu-Chongqing area, the summer ozone formation sensitivity (OFS) was analyzed using satellite observation of the OMI tropospheric column concentration of HCHO and NO2. Additionally, the effects of meteorological factors, source emissions, and their interactions on OFS were identified with the geodetic detector. The results showed that the summer OFS zoning in the Chengdu-Chongqing area was dominated by a transitional regime, with an area share of 42.42%. Less VOCs-limited regime was observed, which was mainly distributed in the urban areas of Chengdu City and Chongqing Municipality, with an area share of 16.37%. The NOx-limited regime was mainly located in Ya'an City, Leshan City, Yibin City, Luzhou City, and the eastern part of Chongqing Municipality, with an area share of 41.21%. The area of the VOCs-limited regime gradually decreased from June to August and reached the lowest value in August, accounting for only 3.53%, and the area of the VOCs-limited regime increased significantly in September. Pollutant emissions (CO, PM2.5, NMVOC, and NOx) were the main factors affecting summer OFS in the Chengdu-Chongqing area. With the increase in emissions, the FNR gradually decreased, and the OFS tended to be the VOCs-limited regime. SP, T2, and TCW were the three main meteorological factors that affected the change in summer OFS in the Chengdu-Chongqing area. All three factors were negatively correlated with FNR; the larger the values of SP, T2, and TCW, the more easily OFS changed to a VOCs-limited regime. Interactions between factors exacerbated OFS changes and were the main drivers of spatial and temporal variations for summer OFS in the Chengdu-Chongqing area.

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来源期刊
环境科学
环境科学 Environmental Science-Environmental Science (all)
CiteScore
4.40
自引率
0.00%
发文量
15329
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