多场景自适应电子鼻检测环境气味污染物

IF 11.3 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL
Chen Qu, Zhuoran Zhang, Jinhua Liu, Peng Zhao, Boyu Jing, Wenhui Li, Chuandong Wu, Jiemin Liu
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引用次数: 0

摘要

随着传感技术的快速发展,电子鼻已成为实时环境监测的重要工具,但如何保证其在各种场景下的适用性和准确性仍然是一个关键挑战。在本研究中,开发了一种具有多场景适用性和更高精度的电子鼻系统,用于测量三种典型污染场景(垃圾填埋场、污水处理厂和牲畜养殖场)中的四种常见关键污染物浓度。通过构建分层结构的定性-特定场景的定性子网络来处理传感器响应数据,提出了一种场景自适应策略,以最大限度地减少干扰对测量精度的影响。在场景分类中使用随机森林和支持向量机算法并进行了评估,其中随机森林模型表现最好,在所有场景中对176个样本实现了100%的分类准确率。随后,通过特征重要性分析剔除受干扰较大的传感器特征,利用随机森林回归(RFR)和人工神经元网络(ann)建立场景化定性模型和统一模型。场景自适应策略在所有场景下的目标污染物浓度预测的R²值均超过0.88,与测试集的统一模型相比,平均绝对百分比误差(MAPE)至少降低了15%。此外,通过灵活集成最适用的算法,场景自适应策略可以在各种场景中充分利用不同算法的优势。本研究强调了自适应策略在各种场景下提高电子鼻性能的有效性,为鲁棒、自适应电子鼻系统奠定了基础。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Multi-scenario Adaptive Electronic Nose for the Detection of Environmental Odor Pollutants

Multi-scenario Adaptive Electronic Nose for the Detection of Environmental Odor Pollutants
With the rapid development of sensing technologies, electronic noses have become an important tool for real-time environmental monitoring, but ensuring their applicability and accuracy across various scenarios remains a key challenge. In this study, an electronic nose system with multi-scenario applicability and enhanced accuracy was developed to measure four common key pollutant concentrations in three typical pollution scenarios: landfills, wastewater treatment plants and livestock farms. A scenario-adaptive strategy was proposed to minimize the impact of interferences on the measurement accuracy by constructing a hierarchically structured qualitative-scenario-specific qualitative sub-network to process the sensor response data. Random Forest and Support Vector Machine algorithms were used and evaluated in scenario classification, with the Random Forest model performing best, achieving 100% classification accuracy for 176 samples across all scenarios. Subsequently, scenario-specific qualitative models and unified model were developed with Random Forest Regression (RFR) and Artificial Neuron Networks (ANNs) after eliminating sensor features affected highly by interferences with feature importance analysis. The scenario-adaptive strategy achieved R² values exceeding 0.88 in target pollutant concentration prediction across all scenarios, with a mean absolute percentage error (MAPE) reduction of at least 15% compared with the unified model for the test set. Furthermore, by flexibly integrating the most applicable algorithms, the scenario-adaptive strategy allows the benefits of different algorithms to be fully utilized in various scenarios. This study highlights the effectiveness of the adaptive strategy in improving electronic nose performance across various scenarios, laying a foundation for robust, adaptive electronic nose systems.
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来源期刊
Journal of Hazardous Materials
Journal of Hazardous Materials 工程技术-工程:环境
CiteScore
25.40
自引率
5.90%
发文量
3059
审稿时长
58 days
期刊介绍: The Journal of Hazardous Materials serves as a global platform for promoting cutting-edge research in the field of Environmental Science and Engineering. Our publication features a wide range of articles, including full-length research papers, review articles, and perspectives, with the aim of enhancing our understanding of the dangers and risks associated with various materials concerning public health and the environment. It is important to note that the term "environmental contaminants" refers specifically to substances that pose hazardous effects through contamination, while excluding those that do not have such impacts on the environment or human health. Moreover, we emphasize the distinction between wastes and hazardous materials in order to provide further clarity on the scope of the journal. We have a keen interest in exploring specific compounds and microbial agents that have adverse effects on the environment.
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