Chen Qu, Zhuoran Zhang, Jinhua Liu, Peng Zhao, Boyu Jing, Wenhui Li, Chuandong Wu, Jiemin Liu
{"title":"多场景自适应电子鼻检测环境气味污染物","authors":"Chen Qu, Zhuoran Zhang, Jinhua Liu, Peng Zhao, Boyu Jing, Wenhui Li, Chuandong Wu, Jiemin Liu","doi":"10.1016/j.jhazmat.2025.137660","DOIUrl":null,"url":null,"abstract":"With the rapid development of sensing technologies, electronic noses have become an important tool for real-time environmental monitoring, but ensuring their applicability and accuracy across various scenarios remains a key challenge. In this study, an electronic nose system with multi-scenario applicability and enhanced accuracy was developed to measure four common key pollutant concentrations in three typical pollution scenarios: landfills, wastewater treatment plants and livestock farms. A scenario-adaptive strategy was proposed to minimize the impact of interferences on the measurement accuracy by constructing a hierarchically structured qualitative-scenario-specific qualitative sub-network to process the sensor response data. Random Forest and Support Vector Machine algorithms were used and evaluated in scenario classification, with the Random Forest model performing best, achieving 100% classification accuracy for 176 samples across all scenarios. Subsequently, scenario-specific qualitative models and unified model were developed with Random Forest Regression (RFR) and Artificial Neuron Networks (ANNs) after eliminating sensor features affected highly by interferences with feature importance analysis. The scenario-adaptive strategy achieved R² values exceeding 0.88 in target pollutant concentration prediction across all scenarios, with a mean absolute percentage error (MAPE) reduction of at least 15% compared with the unified model for the test set. Furthermore, by flexibly integrating the most applicable algorithms, the scenario-adaptive strategy allows the benefits of different algorithms to be fully utilized in various scenarios. This study highlights the effectiveness of the adaptive strategy in improving electronic nose performance across various scenarios, laying a foundation for robust, adaptive electronic nose systems.","PeriodicalId":361,"journal":{"name":"Journal of Hazardous Materials","volume":"12 1","pages":""},"PeriodicalIF":11.3000,"publicationDate":"2025-02-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Multi-scenario Adaptive Electronic Nose for the Detection of Environmental Odor Pollutants\",\"authors\":\"Chen Qu, Zhuoran Zhang, Jinhua Liu, Peng Zhao, Boyu Jing, Wenhui Li, Chuandong Wu, Jiemin Liu\",\"doi\":\"10.1016/j.jhazmat.2025.137660\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"With the rapid development of sensing technologies, electronic noses have become an important tool for real-time environmental monitoring, but ensuring their applicability and accuracy across various scenarios remains a key challenge. In this study, an electronic nose system with multi-scenario applicability and enhanced accuracy was developed to measure four common key pollutant concentrations in three typical pollution scenarios: landfills, wastewater treatment plants and livestock farms. A scenario-adaptive strategy was proposed to minimize the impact of interferences on the measurement accuracy by constructing a hierarchically structured qualitative-scenario-specific qualitative sub-network to process the sensor response data. Random Forest and Support Vector Machine algorithms were used and evaluated in scenario classification, with the Random Forest model performing best, achieving 100% classification accuracy for 176 samples across all scenarios. Subsequently, scenario-specific qualitative models and unified model were developed with Random Forest Regression (RFR) and Artificial Neuron Networks (ANNs) after eliminating sensor features affected highly by interferences with feature importance analysis. The scenario-adaptive strategy achieved R² values exceeding 0.88 in target pollutant concentration prediction across all scenarios, with a mean absolute percentage error (MAPE) reduction of at least 15% compared with the unified model for the test set. Furthermore, by flexibly integrating the most applicable algorithms, the scenario-adaptive strategy allows the benefits of different algorithms to be fully utilized in various scenarios. This study highlights the effectiveness of the adaptive strategy in improving electronic nose performance across various scenarios, laying a foundation for robust, adaptive electronic nose systems.\",\"PeriodicalId\":361,\"journal\":{\"name\":\"Journal of Hazardous Materials\",\"volume\":\"12 1\",\"pages\":\"\"},\"PeriodicalIF\":11.3000,\"publicationDate\":\"2025-02-18\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Hazardous Materials\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://doi.org/10.1016/j.jhazmat.2025.137660\",\"RegionNum\":1,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, ENVIRONMENTAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Hazardous Materials","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.1016/j.jhazmat.2025.137660","RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
Multi-scenario Adaptive Electronic Nose for the Detection of Environmental Odor Pollutants
With the rapid development of sensing technologies, electronic noses have become an important tool for real-time environmental monitoring, but ensuring their applicability and accuracy across various scenarios remains a key challenge. In this study, an electronic nose system with multi-scenario applicability and enhanced accuracy was developed to measure four common key pollutant concentrations in three typical pollution scenarios: landfills, wastewater treatment plants and livestock farms. A scenario-adaptive strategy was proposed to minimize the impact of interferences on the measurement accuracy by constructing a hierarchically structured qualitative-scenario-specific qualitative sub-network to process the sensor response data. Random Forest and Support Vector Machine algorithms were used and evaluated in scenario classification, with the Random Forest model performing best, achieving 100% classification accuracy for 176 samples across all scenarios. Subsequently, scenario-specific qualitative models and unified model were developed with Random Forest Regression (RFR) and Artificial Neuron Networks (ANNs) after eliminating sensor features affected highly by interferences with feature importance analysis. The scenario-adaptive strategy achieved R² values exceeding 0.88 in target pollutant concentration prediction across all scenarios, with a mean absolute percentage error (MAPE) reduction of at least 15% compared with the unified model for the test set. Furthermore, by flexibly integrating the most applicable algorithms, the scenario-adaptive strategy allows the benefits of different algorithms to be fully utilized in various scenarios. This study highlights the effectiveness of the adaptive strategy in improving electronic nose performance across various scenarios, laying a foundation for robust, adaptive electronic nose systems.
期刊介绍:
The Journal of Hazardous Materials serves as a global platform for promoting cutting-edge research in the field of Environmental Science and Engineering. Our publication features a wide range of articles, including full-length research papers, review articles, and perspectives, with the aim of enhancing our understanding of the dangers and risks associated with various materials concerning public health and the environment. It is important to note that the term "environmental contaminants" refers specifically to substances that pose hazardous effects through contamination, while excluding those that do not have such impacts on the environment or human health. Moreover, we emphasize the distinction between wastes and hazardous materials in order to provide further clarity on the scope of the journal. We have a keen interest in exploring specific compounds and microbial agents that have adverse effects on the environment.