Runlong Gao, Wuying Ma, Pengying Wan, Ao Liu, Xiao Ouyang, Xue Du, Qiantao Lei, Qi Deng, Linyue Liu, Xiaoping Ouyang
{"title":"基于碳化硅换能器的阿尔法光伏电池实现 2.1% 的效率","authors":"Runlong Gao, Wuying Ma, Pengying Wan, Ao Liu, Xiao Ouyang, Xue Du, Qiantao Lei, Qi Deng, Linyue Liu, Xiaoping Ouyang","doi":"10.1002/eem2.12846","DOIUrl":null,"url":null,"abstract":"<p>Alpha-voltaic cell is a type of micro nuclear battery that provides several decades of reliable power in the nanowatt to microwatt range, supplying for special applications where traditional chemical batteries or solar cells are difficult to operate. However, the power conversion efficiency of the alpha-voltaic cells reported are still far behind the theoretical limit, making the development of alpha-voltaic cell challenging. Developing advanced semiconductor transducers with higher efficiency in converting the energy of alpha particles into electric energy is proving to be necessary for realizing high-power conversion efficiency. Herein, we propose an alpha-voltaic cell based on SiC PIN transducer that includes a sensitive region with an area of 1 cm<sup>2</sup>, a width of 51.2 μm, and a charge collection efficiency of 95.6% at 0 V bias. We find that optimizing the unintentional doping concentration and crystal quality of the SiC epitaxial layer can significantly increase the absorption and utilization of the energy of alpha particles, resulting in a 2.4-fold enhancement in power conversion efficiency compared with that of the previous study. Electrical properties of the SiC alpha-voltaic cell are measured using an He-ion accelerator as the equivalent α-radioisotopes, with the best power conversion efficiency of 2.10% and maximum output power density of 406.66 nW cm<sup>−2</sup> is obtained. Our research makes a big leap in SiC alpha-voltaic cell, bridging the gap between micro nuclear batteries and practical applications in micro-electromechanical systems, micro aerial vehicles, and tiny satellites.</p>","PeriodicalId":11554,"journal":{"name":"Energy & Environmental Materials","volume":"8 2","pages":""},"PeriodicalIF":13.0000,"publicationDate":"2024-11-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/eem2.12846","citationCount":"0","resultStr":"{\"title\":\"Achieving 2.1% Efficiency in Alpha-Voltaic Cell Based on Silicon Carbide Transducer\",\"authors\":\"Runlong Gao, Wuying Ma, Pengying Wan, Ao Liu, Xiao Ouyang, Xue Du, Qiantao Lei, Qi Deng, Linyue Liu, Xiaoping Ouyang\",\"doi\":\"10.1002/eem2.12846\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Alpha-voltaic cell is a type of micro nuclear battery that provides several decades of reliable power in the nanowatt to microwatt range, supplying for special applications where traditional chemical batteries or solar cells are difficult to operate. However, the power conversion efficiency of the alpha-voltaic cells reported are still far behind the theoretical limit, making the development of alpha-voltaic cell challenging. Developing advanced semiconductor transducers with higher efficiency in converting the energy of alpha particles into electric energy is proving to be necessary for realizing high-power conversion efficiency. Herein, we propose an alpha-voltaic cell based on SiC PIN transducer that includes a sensitive region with an area of 1 cm<sup>2</sup>, a width of 51.2 μm, and a charge collection efficiency of 95.6% at 0 V bias. We find that optimizing the unintentional doping concentration and crystal quality of the SiC epitaxial layer can significantly increase the absorption and utilization of the energy of alpha particles, resulting in a 2.4-fold enhancement in power conversion efficiency compared with that of the previous study. Electrical properties of the SiC alpha-voltaic cell are measured using an He-ion accelerator as the equivalent α-radioisotopes, with the best power conversion efficiency of 2.10% and maximum output power density of 406.66 nW cm<sup>−2</sup> is obtained. Our research makes a big leap in SiC alpha-voltaic cell, bridging the gap between micro nuclear batteries and practical applications in micro-electromechanical systems, micro aerial vehicles, and tiny satellites.</p>\",\"PeriodicalId\":11554,\"journal\":{\"name\":\"Energy & Environmental Materials\",\"volume\":\"8 2\",\"pages\":\"\"},\"PeriodicalIF\":13.0000,\"publicationDate\":\"2024-11-27\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://onlinelibrary.wiley.com/doi/epdf/10.1002/eem2.12846\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Energy & Environmental Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://onlinelibrary.wiley.com/doi/10.1002/eem2.12846\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Energy & Environmental Materials","FirstCategoryId":"88","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/eem2.12846","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Achieving 2.1% Efficiency in Alpha-Voltaic Cell Based on Silicon Carbide Transducer
Alpha-voltaic cell is a type of micro nuclear battery that provides several decades of reliable power in the nanowatt to microwatt range, supplying for special applications where traditional chemical batteries or solar cells are difficult to operate. However, the power conversion efficiency of the alpha-voltaic cells reported are still far behind the theoretical limit, making the development of alpha-voltaic cell challenging. Developing advanced semiconductor transducers with higher efficiency in converting the energy of alpha particles into electric energy is proving to be necessary for realizing high-power conversion efficiency. Herein, we propose an alpha-voltaic cell based on SiC PIN transducer that includes a sensitive region with an area of 1 cm2, a width of 51.2 μm, and a charge collection efficiency of 95.6% at 0 V bias. We find that optimizing the unintentional doping concentration and crystal quality of the SiC epitaxial layer can significantly increase the absorption and utilization of the energy of alpha particles, resulting in a 2.4-fold enhancement in power conversion efficiency compared with that of the previous study. Electrical properties of the SiC alpha-voltaic cell are measured using an He-ion accelerator as the equivalent α-radioisotopes, with the best power conversion efficiency of 2.10% and maximum output power density of 406.66 nW cm−2 is obtained. Our research makes a big leap in SiC alpha-voltaic cell, bridging the gap between micro nuclear batteries and practical applications in micro-electromechanical systems, micro aerial vehicles, and tiny satellites.
期刊介绍:
Energy & Environmental Materials (EEM) is an international journal published by Zhengzhou University in collaboration with John Wiley & Sons, Inc. The journal aims to publish high quality research related to materials for energy harvesting, conversion, storage, and transport, as well as for creating a cleaner environment. EEM welcomes research work of significant general interest that has a high impact on society-relevant technological advances. The scope of the journal is intentionally broad, recognizing the complexity of issues and challenges related to energy and environmental materials. Therefore, interdisciplinary work across basic science and engineering disciplines is particularly encouraged. The areas covered by the journal include, but are not limited to, materials and composites for photovoltaics and photoelectrochemistry, bioprocessing, batteries, fuel cells, supercapacitors, clean air, and devices with multifunctionality. The readership of the journal includes chemical, physical, biological, materials, and environmental scientists and engineers from academia, industry, and policy-making.