多孔mof衍生过渡金属-氮-碳作为质子交换膜燃料电池氧还原反应催化剂的合理设计研究进展

IF 9.4 2区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Wai Yin Wong, Muhammad Amirul Aiman Abdul Rani, Kee Shyuan Loh, Kean Long Lim, Lorna Jeffery Minggu
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引用次数: 0

摘要

对可持续能源解决方案的追求推动了对氧还原反应(ORR)催化剂的重大研究。金属-有机骨架(MOF)衍生的过渡金属-氮-碳(TM-N-C)催化剂由于其丰富度、高表面积和单原子催化剂形成的潜力而成为铂的有前途的替代品。然而,与内在活动和耐久性相关的挑战阻碍了它们的广泛采用。这篇综述重点介绍了mof衍生的TM-N-C催化剂的最新进展,包括调制电子性能、创建开放孔结构和引入支撑材料的策略。这些方法旨在提高质子交换膜燃料电池的活性和稳定性。重点介绍近年来在质子交换膜燃料电池性能和稳定性方面取得的最新进展。提出了未来的研究方向,以提高燃料电池在各种环境下的可持续性和最佳性能。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Current progress on rational design of porous MOF-derived transition metal–nitrogen–carbon as oxygen reduction reaction catalysts for proton exchange membrane fuel cells
The pursuit of sustainable energy solutions has driven significant research into oxygen reduction reaction (ORR) catalysts. metal–organic framework (MOF)-derived transition metal–nitrogen–carbon (TM-N-C) catalysts emerge as a promising alternative to platinum due to their abundance, high surface area, and potential for single-atom catalyst formation. However, challenges related to intrinsic activity and durability hinder their widespread adoption. This mini-review highlights current advancements in MOF-derived TM-N-C catalyst development, including strategies to modulate electronic properties, create open pore structures, and introduce supportive materials. These approaches aim to enhance both activity and stability for proton exchange membrane fuel cell applications. The recent works with highest proton exchange membrane fuel cell performance and stability will be highlighted. Future research direction is proposed to achieve improved sustainability and optimal performance in various fuel cell environments.
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来源期刊
CiteScore
16.00
自引率
2.20%
发文量
140
审稿时长
103 days
期刊介绍: The Current Opinion journals address the challenge specialists face in keeping up with the expanding information in their fields. In Current Opinion in Green and Sustainable Chemistry, experts present views on recent advances in a clear and readable form. The journal also provides evaluations of the most noteworthy papers, annotated by experts, from the extensive pool of original publications in Green and Sustainable Chemistry.
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