工程超快光诱导电荷和碳中间体在界面上的转移打破了甲烷直接转化为甲醇的活性-选择性平衡[j] .能源工程，6/2025。

IF 26 1区材料科学 Q1 CHEMISTRY, PHYSICAL

Advanced Energy Materials Pub Date : 2025-02-11 DOI:10.1002/aenm.202570032

Yuehan Cao, Wang Yu, Yi Li, Jie Meng, Kaibo Zheng, Chuan Huang, Xin Yang, Yuantao Yang, Fan Dong, Ying Zhou

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引用次数: 0

摘要

在文章2404871中，周颖等人介绍了利用BiOI/BN异质结纳米片在光催化甲烷制甲醇方面取得的突破性进展，他们利用界面工程技术增强了超快电荷转移，稳定了中间体生产甲醇的逆向反应。在环境条件下，24小时甲烷转化率为15.5%，甲醇选择性为86.4%。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

Engineering Ultrafast Photo-Induced Charge and Carbon Intermediates Transfer at Interface to Break the Activity-Selectivity Trade-Off in Direct Conversion of Methane to Methanol (Adv. Energy Mater. 6/2025)

查看原文本刊更多论文

Methane Conversion

In article number 2404871, Ying Zhou and co-workers introduce a breakthrough in photocatalytic methane-to-methanol conversion using BiOI/BN heterojunction nanosheets, employing interface engineering to enhance ultrafast charge transfer and stabilize the backtracking of intermediate to produce methanol. This achieves 15.5% methane conversion and 86.4% methanol selectivity under ambient conditions for 24 hours.

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来源期刊

Advanced Energy Materials CHEMISTRY, PHYSICAL-ENERGY & FUELS

CiteScore

41.90

自引率

4.00%

发文量

889

审稿时长

1.4 months

期刊介绍： Established in 2011, Advanced Energy Materials is an international, interdisciplinary, English-language journal that focuses on materials used in energy harvesting, conversion, and storage. It is regarded as a top-quality journal alongside Advanced Materials, Advanced Functional Materials, and Small. With a 2022 Impact Factor of 27.8, Advanced Energy Materials is considered a prime source for the best energy-related research. The journal covers a wide range of topics in energy-related research, including organic and inorganic photovoltaics, batteries and supercapacitors, fuel cells, hydrogen generation and storage, thermoelectrics, water splitting and photocatalysis, solar fuels and thermosolar power, magnetocalorics, and piezoelectronics. The readership of Advanced Energy Materials includes materials scientists, chemists, physicists, and engineers in both academia and industry. The journal is indexed in various databases and collections, such as Advanced Technologies & Aerospace Database, FIZ Karlsruhe, INSPEC (IET), Science Citation Index Expanded, Technology Collection, and Web of Science, among others.