燃料和技术对生物质炉灶颗粒排放的影响──物理和化学性质的详细表征

IF 4.3 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Robert Lindgren, Natxo García-López, Karin Lovén, Lisa Lundin, Joakim Pagels and Christoffer Boman*, 
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引用次数: 0

摘要

在全球范围内,30亿人依靠固体生物质燃料进行日常烹饪,其中大多数人使用效率低下的烹饪方法,导致家庭空气污染程度很高。这随后与负面的健康和气候影响联系在一起。此外,生物质燃料的低效使用给天然林带来压力,导致森林砍伐、生物多样性丧失和土壤退化。正在推广改进的炉灶技术和生物质燃料,以减轻这些问题。然而,关于炉子技术和新燃料之间的相互作用如何影响颗粒排放的物理和化学性质的知识有限。在本研究中,在实验室设置中评估了四种炉灶技术与五种燃料相结合的排放性能,采用改进的水沸腾试验和罩式稀释系统进行烟气采样。采用过滤器取样来确定细颗粒物(PM1)的排放,并对多环芳香族化合物(PAC)、有机碳和元素碳以及无机成分进行后续分析。采用13级低压级联冲击器测定颗粒粒径分布。使用在线仪器来确定气体排放(例如CO, CH4和BTX)以及颗粒数大小分布。结果表明,炉体设计和燃料性能对总排放和PM的理化特性都有影响。进一步发现,燃料对PM性能的影响在不同炉具技术之间并不是线性转化的。这意味着每个炉子都应该用不同的燃料进行测试,以确定总排放量和燃料的适用性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Influence of Fuel and Technology on Particle Emissions from Biomass Cookstoves─Detailed Characterization of Physical and Chemical Properties

Globally, 3 billion people rely on solid biomass fuel for their everyday cooking, most often using inefficient cooking practices, leading to high exposure levels of household air pollution. This is subsequently associated with negative health and climate impact. Further, the inefficient use of biomass fuels applies pressure on natural forests, resulting in deforestation, loss of biodiversity, and soil degradation. Improved cookstove technologies and biomass fuels are being promoted to mitigate these issues. However, limited knowledge exists about how the interaction between stove technology and new fuels affects the physical and chemical properties of particulate emissions. In this study, the emission performance of four cookstove technologies in combination with five fuels was evaluated in a laboratory setup, applying a modified water boiling test with a hood dilution system for flue gas sampling. Filter sampling was applied to determine the emissions of fine particulate matter (PM1) and for subsequent analysis of polycyclic aromatic compounds (PAC), organic- and elemental carbon, and inorganic composition. Particle mass size distribution was determined by using a 13-stage low-pressure cascade impactor. Online instruments were used to determine gaseous emissions (e.g., CO, CH4, and BTX) as well as particle number size distribution. The results show that both the stove design and fuel properties influence the total emissions as well as the physiochemical PM characteristics. It was further seen that the impact of fuel on the PM properties did not translate linearly among the different stove technologies. This implies that each stove should be tested with various fuels to determine both the total emissions and fuel suitability.

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来源期刊
ACS Omega
ACS Omega Chemical Engineering-General Chemical Engineering
CiteScore
6.60
自引率
4.90%
发文量
3945
审稿时长
2.4 months
期刊介绍: ACS Omega is an open-access global publication for scientific articles that describe new findings in chemistry and interfacing areas of science, without any perceived evaluation of immediate impact.
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