无焰蜡烛并非无污染:有香味的蜡融化为大气纳米粒子的重要来源

IF 8.9 2区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL
Satya S. Patra, Jinglin Jiang, Jianghui Liu, Gerhard Steiner, Nusrat Jung* and Brandon E. Boor*, 
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引用次数: 0

摘要

作为一种更安全、无毒的室内香薰蜡烛和熏香的替代品,香味蜡融化剂正在得到普及。我们在一个住宅测试屋进行了现场测量,以调查使用芳香蜡熔体形成的大气纳米颗粒。采用高分辨率粒子尺寸放大扫描迁移率粒子尺寸仪(PSMPS)和质子转移反应飞行时间质谱仪(PTR-TOF-MS)分别实时监测室内大气纳米颗粒尺寸分布和萜烯混合比。我们的研究结果表明,从芳香蜡熔体中释放的萜烯与室内大气臭氧(O3)发生反应,引发新颗粒形成(NPF)事件,导致室内大气纳米颗粒浓度显著(>106 cm-3),与燃烧型芳香蜡烛、燃气灶、柴油发动机和天然气发动机排放的纳米颗粒浓度相当。我们发现,香味蜡融化引发的NPF事件可导致显著的呼吸道暴露,纳米颗粒呼吸道沉积剂量率与燃烧源的剂量率相似。我们的研究结果挑战了香味蜡融化物作为燃烧芳香疗法更安全替代品的看法,强调需要进一步研究新形成的纳米颗粒的毒理学特性,以更好地了解它们对环境健康的影响。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Flame-Free Candles Are Not Pollution-Free: Scented Wax Melts as a Significant Source of Atmospheric Nanoparticles

Scented wax melts are being popularized as a safer, nontoxic alternative to traditional candles and incense for indoor aromatherapy. We performed field measurements in a residential test house to investigate atmospheric nanoparticle formation from scented wax melt use. We employed a high-resolution particle size magnifier-scanning mobility particle sizer (PSMPS) and a proton transfer reaction time-of-flight mass spectrometer (PTR-TOF-MS) for real-time monitoring of indoor atmospheric nanoparticle size distributions and terpene mixing ratios, respectively. Our findings reveal that terpenes released from scented wax melts react with indoor atmospheric ozone (O3) to initiate new particle formation (NPF) events, resulting in significant indoor atmospheric nanoparticle concentrations (>106 cm–3) comparable to those emitted by combustion-based scented candles, gas stoves, diesel engines, and natural gas engines. We show that scented wax melt-initiated NPF events can result in significant respiratory exposures, with nanoparticle respiratory tract deposited dose rates similar to those determined for combustion-based sources. Our results challenge the perception of scented wax melts as a safer alternative to combustion-based aromatherapy, highlighting the need for further research on the toxicological properties of the newly formed nanoparticles to better understand their environmental health implications.

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来源期刊
Environmental Science & Technology Letters Environ.
Environmental Science & Technology Letters Environ. ENGINEERING, ENVIRONMENTALENVIRONMENTAL SC-ENVIRONMENTAL SCIENCES
CiteScore
17.90
自引率
3.70%
发文量
163
期刊介绍: Environmental Science & Technology Letters serves as an international forum for brief communications on experimental or theoretical results of exceptional timeliness in all aspects of environmental science, both pure and applied. Published as soon as accepted, these communications are summarized in monthly issues. Additionally, the journal features short reviews on emerging topics in environmental science and technology.
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