盐湖排放被忽视的贡献——以青藏高原沙尘沉积为例

IF 3.4 2区 地球科学 Q2 METEOROLOGY & ATMOSPHERIC SCIENCES
Haixia Zhu, Wenxia Li, Xiangrui Kong, Xiying Zhang
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引用次数: 0

摘要

青藏高原东北部柴达木盆地盐湖众多,生态系统脆弱,盐尘排放对其影响日益严重。为了评价盐尘对环境的影响,于2020年1月至2023年3月,在6个监测站每月采集尘样,分析尘、盐尘沉积通量(DF)、矿物组成、水溶性离子、微量元素和碳质含量。采用反向轨迹模型、Pearson相关、富集因子(EF)分析和正矩阵分解(PMF)等方法量化盐湖对大气扬尘的贡献。结果表明,盐酸盐和石膏含量在0 ~ 47 wt%之间,盐尘沉积通量(SDF)在0 ~ 2.54 g/m2·30d之间。关键可溶性离子包括非playa盐硫酸盐(nps-SO42−),playa盐氯化物(ps-Cl−)和钠(ps-Na+)。微量元素如铁、铝、硅和钛来源于自然和人为来源。有机碳/元素碳(OC/EC)比和PMF模型指出,车辆排放、煤炭燃烧和生物质燃烧是主要污染源,尤其是在城市地区。PMF分析表明,盐湖占总粉尘质量的5.23% ~ 29.76%,与可溶性离子和盐石膏含量的变化一致。由于该地区是河流系统的主要来源,粉尘中的可溶性盐对冰川和淡水资源构成威胁。这些发现突出了内陆盐气溶胶在干旱内陆地区的重大影响,强调它们对大气过程的贡献是重要的,不应被忽视。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Overlooked Contribution of Salt Lake Emissions: A Case Study of Dust Deposition From the Qinghai-Xizang Plateau

Overlooked Contribution of Salt Lake Emissions: A Case Study of Dust Deposition From the Qinghai-Xizang Plateau

The Qaidam Basin in the Northeastern Qinghai-Xizang Plateau, characterized by its numerous salt lakes and fragile ecosystem, is increasingly impacted by salt dust emissions. To evaluate the impact of salt dust on environment, monthly dust samples were collected from six monitoring stations between January 2020 and March 2023 and analyzed for dust and salt dust deposition flux (DF), mineral composition, water-soluble ions, trace elements, and carbonaceous content. The study used backward trajectory modeling, Pearson correlation, enrichment factor (EF) analysis, and positive matrix factorization (PMF) to quantify salt lake contributions to atmospheric dust. Results revealed that halite and gypsum content ranged from 0 to 47 wt%, with salt dust deposition flux (SDF) varying between 0 and 2.54 g/m2·30d. Key soluble ions included non-playa salt sulfate (nps-SO42−), playa salt chloride (ps-Cl), and sodium (ps-Na+). Trace elements such as iron, aluminum, silicon, and titanium originated from both natural and anthropogenic sources. The organic carbon to element carbon (OC/EC) ratio and PMF model pointed to vehicle emissions, coal combustion, and biomass burning as major pollution sources, particularly in urban areas. PMF analysis showed that salt lakes contributed 5.23%–29.76% of total dust mass, aligning with changes in soluble ion and halite gypsum content. As the region is a key source of river systems, the soluble salts in dust pose risks to glaciers and freshwater resources. These findings highlight the substantial impact of inland salt aerosols in arid inland regions, emphasizing that their contribution to atmospheric processes is significant and should not be overlooked.

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来源期刊
Journal of Geophysical Research: Atmospheres
Journal of Geophysical Research: Atmospheres Earth and Planetary Sciences-Geophysics
CiteScore
7.30
自引率
11.40%
发文量
684
期刊介绍: JGR: Atmospheres publishes articles that advance and improve understanding of atmospheric properties and processes, including the interaction of the atmosphere with other components of the Earth system.
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