α放射性遥测技术中不同环境条件下氮荧光产率的研究

IF 1.4 3区 物理与天体物理 Q3 INSTRUMENTS & INSTRUMENTATION
Quanxiao Wang , Wanlin Li , Xinfeng Pei , Binghua Song , Junliang Chen , Yiqiang Zhong , Lianshun Li , Jian Wang , Tinggui Yang , Shuyao Si , Kaihong Fang
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引用次数: 0

摘要

核燃料循环中的α衰变具有很强的电离能力,对其危害很大,必须进行有效的检测。传统的检测方法需要耗时的扫描或采样,往往不适合极端环境和增加辐射风险。α辐射遥测技术(ARTT)是一种利用二次氮荧光检测的非接触式α辐射检测方法,解决了传统方法的局限性,近年来受到广泛关注。然而,α-诱导的氮荧光在不同条件下的研究有限,影响了环境校正和定量分析,制约了ARTT的应用。本文考察了α-诱导的氮荧光产率对能量、压力、湿度和氮氧比的依赖性,给出了所有主要2P系统发射波段的测量结果。结果表明:(1)在1.5-4 MeV范围内,沉积能量或α-射线能量对荧光产率没有影响;(2)产率对压力和湿度的依赖符合理论预期,但对氮氧比有偏差;(3)温度对荧光产率的影响最小,在25°C左右30°C的变化对荧光产率的影响小于5%。相比之下,在1atm压力下,空气的产量是零压力下的几百倍。在25°C时,干燥空气的产率是100% RH时的1.4倍。纯氮的能量比含20%氮和80%氧的能量高十倍以上。该工作为ARTT应用中的环境校正提供了数据基础。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Study of the nitrogen fluorescence yield under different environmental conditions in alpha radioactivity telemetry technique
α Decay in the nuclear fuel cycle poses significant hazards due to its strong ionizing capability, making effective detection essential. Conventional detection methods require time-consuming scanning or sampling, often unsuitable for extreme environments and increasing radiation risks. Alpha Radioactivity Telemetry Technology (ARTT), a non-contact α radiation detecting method via secondary nitrogen fluorescence detection, addresses the limitations of traditional methods and has gained significant attention in recent years. However, limited research on α-induced nitrogen fluorescence under varying conditions hampers environmental corrections and quantitative analysis, constraining applications of ARTT. This article examines the dependence of α-induced nitrogen fluorescence yield on energy, pressure, humidity, and nitrogen–oxygen ratio, presenting measurements for all major 2P system emission bands. The results indicate that (1) fluorescence yield remains unaffected by deposited energy or α-ray energy within 1.5–4 MeV, (2) yield dependence on pressure and humidity aligns with theoretical expectations, but deviates for nitrogen–oxygen ratios, and (3) temperature has minimal impact, with a 30 °C variation around 25 °C affecting fluorescence yield by less than 5 %. In contrast, at 1 atm pressure, the yield of air is several hundred times greater than at zero pressure. At 25 °C, the yield of dry air is 1.4 times that of air at 100 % RH. And the one of pure nitrogen is over ten times higher than the gas with 20 % nitrogen and 80 % oxygen. This work provides a data foundation for environmental corrections in ARTT applications.
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来源期刊
CiteScore
2.80
自引率
7.70%
发文量
231
审稿时长
1.9 months
期刊介绍: Section B of Nuclear Instruments and Methods in Physics Research covers all aspects of the interaction of energetic beams with atoms, molecules and aggregate forms of matter. This includes ion beam analysis and ion beam modification of materials as well as basic data of importance for these studies. Topics of general interest include: atomic collisions in solids, particle channelling, all aspects of collision cascades, the modification of materials by energetic beams, ion implantation, irradiation - induced changes in materials, the physics and chemistry of beam interactions and the analysis of materials by all forms of energetic radiation. Modification by ion, laser and electron beams for the study of electronic materials, metals, ceramics, insulators, polymers and other important and new materials systems are included. Related studies, such as the application of ion beam analysis to biological, archaeological and geological samples as well as applications to solve problems in planetary science are also welcome. Energetic beams of interest include atomic and molecular ions, neutrons, positrons and muons, plasmas directed at surfaces, electron and photon beams, including laser treated surfaces and studies of solids by photon radiation from rotating anodes, synchrotrons, etc. In addition, the interaction between various forms of radiation and radiation-induced deposition processes are relevant.
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