基于稳定同位素的青藏高原典型高寒湖泊水化学过程与水平衡趋势

IF 3.4 2区 地球科学 Q1 GEOCHEMISTRY & GEOPHYSICS
Changchang Fu , Xiangquan Li , Xu Cheng , Cong Liu , Zhanxue Bai , Jinqiu Li
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引用次数: 0

摘要

由于气候变暖,青藏高原水循环加速,导致高寒湖泊持续增长。一旦溢流,会对下游水质和资源造成重大威胁。然而,对青藏高原湖泊的化学成分和水分平衡缺乏全面的研究。研究了位于青藏高原中部的盐湖盆地高寒湖泊的演化机制。研究了稳定同位素(δ18O和δD)和水化学,并利用同位素平衡模型确定了湖泊水的蒸发流入比(E/I)。结果表明,湖泊水体具有ClNa型水化学特征,富集总溶解固体(TDS)、硼(B)和锂(Li)元素。在δD- δ18O图上,湖水在当地大气水位线(LMWL)下方呈右向倾斜,斜率为4.75,截距为11.83,显示出明显的蒸发特征。更多的正同位素信号和主要离子之间的比值表明,蒸发过程主要控制着湖水的水化学。模拟的E/I比值在0.19 ~ 0.65之间,表明湖水量正平衡,有利于湖面面积的持续扩大。因此,地方政府需要加大监测力度,密切观察堰湖水位波动,加快实施湖泊引水工程,并对其对当地生态环境的潜在影响进行综合评估。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Hydrochemical processes and water balance trends based on stable isotopes of typical alpine lakes in the Qinghai-Tibet Plateau
Due to the warming climate, the hydrological cycle of the Qinghai-Tibet Plateau (QTP) is accelerating, leading to continuous growth of alpine lakes. In case of overflow, this can pose significant risks to downstream water quality and resources. However, there is a lack of comprehensive investigations on the chemical composition and water balance of lakes in QTP. This study examines the evolutionary mechanisms of alpine lakes in the Yanhu Lake Basin (YHB) located in central QTP. It investigates stable isotopes (δ18O and δD), hydrochemistry, and utilizes the isotope balance model to determine the evaporation to inflow (E/I) ratio of lake water. The findings reveal that lake water exhibits a ClNa hydrochemical type with enrichment in total dissolved solids (TDS), boron (B), and lithium (Li) elements. On the δD- δ18O plot, lake water falls below the Local Meteoric Water Line (LMWL) towards rightward direction with a slope of 4.75 and an intercept of 11.83, indicating pronounced evaporation characteristics. The presence of more positive isotope signals and ratios among major ions suggests that evaporation processes primarily govern lake water's hydrochemistry. The modeled E/I ratio ranges from 0.19 to 0.65 across YHB, implying a positive lake water balance which contributes to consistent expansion in surface area. This highlights the need for local government to enhance monitoring efforts, closely observe fluctuations in Yanhu Lake's water level, expedite implementation of lake water diversion projects, and conduct comprehensive assessment on their potential impact on local ecological environment.
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来源期刊
Journal of Geochemical Exploration
Journal of Geochemical Exploration 地学-地球化学与地球物理
CiteScore
7.40
自引率
7.70%
发文量
148
审稿时长
8.1 months
期刊介绍: Journal of Geochemical Exploration is mostly dedicated to publication of original studies in exploration and environmental geochemistry and related topics. Contributions considered of prevalent interest for the journal include researches based on the application of innovative methods to: define the genesis and the evolution of mineral deposits including transfer of elements in large-scale mineralized areas. analyze complex systems at the boundaries between bio-geochemistry, metal transport and mineral accumulation. evaluate effects of historical mining activities on the surface environment. trace pollutant sources and define their fate and transport models in the near-surface and surface environments involving solid, fluid and aerial matrices. assess and quantify natural and technogenic radioactivity in the environment. determine geochemical anomalies and set baseline reference values using compositional data analysis, multivariate statistics and geo-spatial analysis. assess the impacts of anthropogenic contamination on ecosystems and human health at local and regional scale to prioritize and classify risks through deterministic and stochastic approaches. Papers dedicated to the presentation of newly developed methods in analytical geochemistry to be applied in the field or in laboratory are also within the topics of interest for the journal.
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