废棕榈油加氢转化为生物喷气燃料用钴分散硫酸氧化锆纳米催化剂的合成

Q1 Environmental Science
Riska Astin Fitria , Niko Prasetyo , Aldino Javier Saviola , Wega Trisunaryanti , Akhmad Syoufian , Amalia Kurnia Amin , Won-Chun Oh , Karna Wijaya
{"title":"废棕榈油加氢转化为生物喷气燃料用钴分散硫酸氧化锆纳米催化剂的合成","authors":"Riska Astin Fitria ,&nbsp;Niko Prasetyo ,&nbsp;Aldino Javier Saviola ,&nbsp;Wega Trisunaryanti ,&nbsp;Akhmad Syoufian ,&nbsp;Amalia Kurnia Amin ,&nbsp;Won-Chun Oh ,&nbsp;Karna Wijaya","doi":"10.1016/j.cscee.2024.101052","DOIUrl":null,"url":null,"abstract":"<div><div>In the past decade, rising demand for air travel has resulted in increased carbon emissions, stimulating research into bio-jet fuel as an eco-friendly aviation alternative. This study examines the synthesis and application of cobalt-dispersed sulfated zirconia nanocatalysts for the hydroconversion of used palm cooking oil into bio-jet fuel under atmospheric conditions. The catalysts were synthesized using the wet impregnation method with varying cobalt loadings (1 %, 3 %, and 5 %) and characterized by FTIR, XRD, NH<sub>3</sub>-TPD, SAA, XRF, SEM-EDX Mapping, TEM-SAED, and XPS analyses. Hydroconversion with the Co-3/SZ catalyst yielded a 63.03 wt% liquid product, with 92.28 % bio-jet fuel selectivity and a yield of 58.17 wt%. Reusability tests for six consecutive runs further indicated that this catalyst maintained a bio-jet fuel selectivity of 56.94 % and a yield of 28.43 %, underscoring its potential as a promising candidate for bio-jet fuel production.</div></div>","PeriodicalId":34388,"journal":{"name":"Case Studies in Chemical and Environmental Engineering","volume":"11 ","pages":"Article 101052"},"PeriodicalIF":0.0000,"publicationDate":"2024-12-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Synthesis of cobalt-dispersed sulfated zirconia nanocatalyst for the hydroconversion of used palm cooking oil into bio-jet fuel\",\"authors\":\"Riska Astin Fitria ,&nbsp;Niko Prasetyo ,&nbsp;Aldino Javier Saviola ,&nbsp;Wega Trisunaryanti ,&nbsp;Akhmad Syoufian ,&nbsp;Amalia Kurnia Amin ,&nbsp;Won-Chun Oh ,&nbsp;Karna Wijaya\",\"doi\":\"10.1016/j.cscee.2024.101052\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>In the past decade, rising demand for air travel has resulted in increased carbon emissions, stimulating research into bio-jet fuel as an eco-friendly aviation alternative. This study examines the synthesis and application of cobalt-dispersed sulfated zirconia nanocatalysts for the hydroconversion of used palm cooking oil into bio-jet fuel under atmospheric conditions. The catalysts were synthesized using the wet impregnation method with varying cobalt loadings (1 %, 3 %, and 5 %) and characterized by FTIR, XRD, NH<sub>3</sub>-TPD, SAA, XRF, SEM-EDX Mapping, TEM-SAED, and XPS analyses. Hydroconversion with the Co-3/SZ catalyst yielded a 63.03 wt% liquid product, with 92.28 % bio-jet fuel selectivity and a yield of 58.17 wt%. Reusability tests for six consecutive runs further indicated that this catalyst maintained a bio-jet fuel selectivity of 56.94 % and a yield of 28.43 %, underscoring its potential as a promising candidate for bio-jet fuel production.</div></div>\",\"PeriodicalId\":34388,\"journal\":{\"name\":\"Case Studies in Chemical and Environmental Engineering\",\"volume\":\"11 \",\"pages\":\"Article 101052\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2024-12-10\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Case Studies in Chemical and Environmental Engineering\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2666016424004468\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"Environmental Science\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Case Studies in Chemical and Environmental Engineering","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2666016424004468","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"Environmental Science","Score":null,"Total":0}
引用次数: 0

摘要

在过去的十年里,航空旅行需求的增长导致了碳排放的增加,刺激了对生物喷气燃料作为环保航空替代品的研究。本研究研究了钴分散硫酸氧化锆纳米催化剂的合成及其在常压条件下将废棕榈油加氢转化为生物喷气燃料的应用。采用湿浸渍法合成了钴含量为1%、3%和5%的催化剂,并通过FTIR、XRD、NH3-TPD、SAA、XRF、SEM-EDX Mapping、TEM-SAED和XPS分析对催化剂进行了表征。在Co-3/SZ催化剂的加氢转化下,液体产物的转化率为63.03 wt%,生物喷气燃料的选择性为92.28%,收率为58.17 wt%。连续6次的重复使用试验进一步表明,该催化剂保持了56.94%的生物喷气燃料选择性和28.43%的产率,突显了其作为生物喷气燃料生产的潜在候选物的潜力。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Synthesis of cobalt-dispersed sulfated zirconia nanocatalyst for the hydroconversion of used palm cooking oil into bio-jet fuel

Synthesis of cobalt-dispersed sulfated zirconia nanocatalyst for the hydroconversion of used palm cooking oil into bio-jet fuel
In the past decade, rising demand for air travel has resulted in increased carbon emissions, stimulating research into bio-jet fuel as an eco-friendly aviation alternative. This study examines the synthesis and application of cobalt-dispersed sulfated zirconia nanocatalysts for the hydroconversion of used palm cooking oil into bio-jet fuel under atmospheric conditions. The catalysts were synthesized using the wet impregnation method with varying cobalt loadings (1 %, 3 %, and 5 %) and characterized by FTIR, XRD, NH3-TPD, SAA, XRF, SEM-EDX Mapping, TEM-SAED, and XPS analyses. Hydroconversion with the Co-3/SZ catalyst yielded a 63.03 wt% liquid product, with 92.28 % bio-jet fuel selectivity and a yield of 58.17 wt%. Reusability tests for six consecutive runs further indicated that this catalyst maintained a bio-jet fuel selectivity of 56.94 % and a yield of 28.43 %, underscoring its potential as a promising candidate for bio-jet fuel production.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Case Studies in Chemical and Environmental Engineering
Case Studies in Chemical and Environmental Engineering Engineering-Engineering (miscellaneous)
CiteScore
9.20
自引率
0.00%
发文量
103
审稿时长
40 days
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信