胶体现象反映了界面溶液结构、粒子间作用力和动力学响应之间的相互作用

IF 7 2区 化学 Q1 CHEMISTRY, PHYSICAL
Jaeyoung Heo , Pravalika Butreddy , Gregory K. Schenter , Christopher J. Mundy , James J. De Yoreo , Elias Nakouzi , Jaewon Lee , Jaehun Chun
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引用次数: 0

摘要

胶体系统的物理和化学性质是自然和合成过程的核心,可以实现广泛的能源和环境应用。这些性质是胶体系统在电学、范德华、水合作用和系统固有波动耦合的空间力的相互作用下所采用的结构的紧急结果。在这里,我们回顾了这些力的性质,并展示了它们的相对重要性的变化如何导致不同的自由能景观和随之而来的动态行为,例如胶体分散,纳米晶超晶格和通过定向附着形成的单晶。最后,我们讨论了由于需要从分子到粒子到集合尺度无缝耦合而产生的未来进展的挑战。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Colloidal phenomena reflect the interplay between interfacial solution structure, interparticle forces, and dynamical response

Colloidal phenomena reflect the interplay between interfacial solution structure, interparticle forces, and dynamical response
The physical and chemical properties of colloidal systems are central to both natural and synthetic processes that enable a wide range of energy and environmental applications. These properties are an emergent outcome of the structure that colloidal systems adopt in response to the interplay of electrical, van der Waals, hydration, and steric forces coupled to the inherent fluctuations of the system. Here we review the nature of those forces and show how variations in their relative importance lead to distinct free energy landscapes and consequent dynamic behaviors, illustrated for colloidal dispersions, nanocrystal superlattices, and single crystals formed through oriented attachment. We end by discussing the challenges to future progress arising from the need to seamlessly couple from molecular to particle to ensemble scales.
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来源期刊
CiteScore
16.50
自引率
1.10%
发文量
74
审稿时长
11.3 weeks
期刊介绍: Current Opinion in Colloid and Interface Science (COCIS) is an international journal that focuses on the molecular and nanoscopic aspects of colloidal systems and interfaces in various scientific and technological fields. These include materials science, biologically-relevant systems, energy and environmental technologies, and industrial applications. Unlike primary journals, COCIS primarily serves as a guide for researchers, helping them navigate through the vast landscape of recently published literature. It critically analyzes the state of the art, identifies bottlenecks and unsolved issues, and proposes future developments. Moreover, COCIS emphasizes certain areas and papers that are considered particularly interesting and significant by the Editors and Section Editors. Its goal is to provide valuable insights and updates to the research community in these specialized areas.
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